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Papers, correspondence and printed items, 1872-1926, relating to the University College of Wales, Aberystwyth. They include copies of the college's early registers, 1872-1877, copies of the conveyance of the college and its hereditaments, 1875, copies of the deed of settlement of the college, and of the charter of incorporation and statutes, both dated 1892, papers concerning the administration of the college's restoration fund, the revised constitution of the college, and the old students' scholarship fund. Other matters include the charter of the federal University of Wales in 1893, the college's building fund, Alexandra Hall, the finance and general purposes committee, the estate of Sir John Williams, the proposed revision of the college's charter and statutes, and museum grants for Wales. The correspondents include Thomas Charles Edwards (3), 1885-1886, Lewis Morris, 1886, and Stuart Rendel, 1889.

Manuscripts and papers of the families of Charles and Edwards, dated between [c. 1600] and 1922; they include letters from Thomas Charles Edwards to his wife, and their son Lewis Charles, 1876-1896; letters to Thomas Charles Edwards, 1885-1899; copies of letters, 1859-1898, including correspondence relating to University College of Wales, Aberystwyth; letters to and from Mary Roberts, 1867-[1893]; letters to their daughter, Elizabeth Alicia Edwards, 1887-1900; Edwards family letters, 1895-1900; and newspapers and press cuttings, [c. 1820]-1922.