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The collection comprises correspondence, including general correspondence to Sir J. Herbert Lewis, 1886-1933, drafts and copies of correspondence from Sir J. Herbert Lewis, 1887-1933, letters from Sir J. Herbert Lewis to Adelaide, his first wife, 1891-1893, letters from Sir J. Herbert Lewis to Ruth, his second wife, 1902-1933, letters from Sir J. Herbert Lewis to his daughter Kitty, 1915-1925, letters from Lady Lewis to Sir J. Herbert Lewis, 1899-1930, letters to Lady Lewis, 1901-1939, and miscellaneous correspondence, 1890-1920; diaries, 1872-1933; Liberal Party in Wales, 1889-1896; subject files (including correspondence), 1865-1933; press cuttings, 1879-1933; deeds and documents, 1442-1864; miscellaneous papers, 1750-1949; and photographs, c. 1890-1929.

Article by Ruth Lewis - 'Early Memories'; letters between Saunders Lewis and Sir Herbert Lewis and other letters; article by Kitty Idwal Jones - 'Early Memories'; article by Olwen Foreman - ''Wartime and College Memories', deposited by Mrs Olwen Foreman, February 2008.

Papers of and relating to Sir Daniel Lleufer Thomas, 1599-1941, comprising general correspondence of Sir Daniel Lleufer Thomas, 1893-1919 and 1922-1940; general correspondence of Lady Thomas, 1895-1941; American letters from descendants of relatives who emigrated, 1873-1931; letters of Welsh interest mainly concerning localities and place-names, 1892-1919; letters relating to T.E. Ellis, 1898-1935; personal letters and cards from Daniel Lleufer Thomas to his wife, 1902; political letters, 1906-1933; papers relating to Daniel Lleufer Thomas's legal career and interests, 1891-1938; subject files relating to his public offices, including his appointment to the Welsh Land Commission, 1887-1941, societies and institutions to which he belonged, 1886-1940, Llandovery School, 1880-1935, the translator and poet Richard Morris Lewis, 1866-1933, general literary and historical interests, 1889-1940, and miscellaneous subjects, 1915-1933; and personal papers which include deeds of Brynmaen, once the family home, 1599-1885, and diaries of Daniel Lleufer Thomas and Lady Thomas, 1892-1899.

Papers of David Robert Daniel, comprising, material relating to Thomas Edward Ellis, MP, including diaries, exercise books, speeches and election addresses, correspondence of Thomas Edward Ellis, including correspondence with D. R. Daniel, papers of his political career, copies of diaries and letters, memoirs by others and papers relating to the death of T. E. Ellis, [c. 1854x1934]; material relating to David Robert Daniel, [c. 1869x1931], including diaries, manuscript volumes and notes on places, his family and various individuals, some being eminent Welshmen, school and college papers, letters and cards to and from D. R. Daniel, including some from public men and women, relations and his wife, and miscellaneous and family papers; material relating to the North Wales Quarrymen's Union and the Penrhyn Quarry Strikes, [1878xc.1903], including reports, pamphlets, cuttings, correspondence, discussions, resolutions, and newspaper cuttings; together with material relating to David Lloyd George, including letters and cards to D. R. Daniel and to Mrs S. E. Daniel, some of which are from David Lloyd George and Megan Lloyd George [c. 1890x1966].