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Manuscripts and papers relating to the Lloyd family of Bronwydd, Cardiganshire, and their ancestors, the Owen family of Henllys, Pembrokeshire, and records relating to the Bronwydd estate, including an early 17th century book of South Wales pedigrees, the literary, genealogical and historical manuscripts of George Owen of Henllys (c.1552-1613), including his Vairdre Book and a copy of his Description of Pembrokeshire; estate records including manorial records of Pembrokeshire manors including the barony of Cemais, including court rolls, 1381-1771, estreat rolls, 1474-1748, and court leet presentments, 1660-1885; records relating to the borough of Newport, Pembrokeshire, 1434-1847; toll books of Eglwyswrw and Newport fairs, 1599-1603; title deeds, 1241-1933, but mostly 16-18 cent.; rentals, 1682-1873; and estate correspondence, mainly [late 19]-[early 20 cent.].

Records of the Lloyd family of Cefn, Denbighshire, and of their estates in Caernarfonshire, Denbighshire and Flintshire, mainly comprising deeds, 1422-1900, including deeds relating to lead and coal mines in Flintshire and copper mines in Caernarfonshire, 18-19 cent.; papers relating to ecclesiastical affairs, 1562-1864; and important papers of Humphrey Humphreys (1648-1712), cleric and antiquarian, and bishop of Bangor, 1689-1701, and Hereford, 1701-12, relating to his period as bishop of Hereford.