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Manuscripts, estate records and papers of the Wynne family of Bodewryd, Anglesey, including records of the Bodowyr estate (Bodedern), Anglesey, and Plas Einion estate, Denbighshire, and papers of the Owen family of Penrhos, Anglesey; important Welsh literary manuscripts, legal manuscripts relating to civil and ecclesiastical law; the antiquarian collections of Edward Wynne, chancellor of Hereford, relating to Wales and to the diocese of Hereford, and part of the collection of Humphrey Humphreys, bishop of Bangor and later of Hereford; letters to Humphrey Humphreys, 1691-1709 (mainly 1705-1709); Wynne family correspondence, 1613-1816; legal papers, [17 cent.]-[18 cent.], especially relating to a lengthy action between Chancellor Edward Wynne and the Mostyn estate following the purchase by Wynne of the Bodowyr estate, 1721-1746; estate, personal and household accounts, 1603-1753; and title deeds, [13 cent.]-1864.

Estate records, mainly title deeds, of the Carreg-lwyd and Berw estates, Anglesey, and family papers, mainly correspondence, of the Griffith family of Carreg-lwyd and the Holland family of Berw, 1329-1864, including valuable early 17th century papers relating to affairs of state, accumulated by John Griffith, secretary to Henry Howard (1540-1614), 1st earl of Northampton, Keeper of the Privy Seal, 1608-1614, and First Commissioner of the Treasury, 1612-1614; accounts and papers relating to the administration of the county of Anglesey, including muster rolls, 1602-1656, mainly for the hundreds of Tindaethwy, Menai and Talybolion; mise, window, house and land tax assessments, 1653-1764, mainly for the hundreds of Tindaethwy, Menai and Talybolion; rentals of Crown lands in the same hundreds; 1503-1737; papers of Dr William Griffith (1597-1648), successively chancellor of the dioceses ofSt Asaph and Bangor, and Commissioner of North Wales from 1633; account of the funerals of Elizabeth I and James I, [1625], and a census of the inhabitants of the parish of Llanfaethlu, Anglesey, August 1690.

Family and estate records of Griffith of Porthamal, Anglesey, and Llanfair, Caernarfonshire, Griffith of Brynodol, Caernarfonshire, and the associated families of Rowlands of Nant, Caernarfonshire, and Wynn of Taltreuddyn, Merionethshire. The estate records include rentals of the Llanfair estate, 1516-1669, the Brynodol estate, 1581-1751, the Cefnamwlch estate, 1630-1717, the Nant estate, 1702-1719, the Taltreuddyn estate, 1744-1848, the Llanfair and Brynodol estate, 1761-1832, and rentals from various other estates, 1615-1816; and deeds of the Porthamal and Llanfair estate, 1435-1673, the Brynodol (and later Llanfair and Brynodol) estate, 1564-1864, and the Taltreuddyn estate, 1664-1751. -- The archive also includes rentals of Crown rents in Anglesey, Caernarfonshire, Denbighshire, Flintshire and Merionethshire, 1558-1798, and ministers' accounts, 1365-1825; Caernarfon borough records, 1545-1783, including rentals of corporation property, lists of burgesses, and notes on the constitution of the borough and the appointment of officers; and a number of literary and historical manuscripts.

Estate records of the Edwards family of Nanhoron, Caernarfonshire, and associated families, including the Vaughan of Bronheulog, Denbighshire, Lloyd of Rhosbeiro, Hirdrefaig, Angelsey, and Jones of Gelliwig, Caernarfonshire, comprising mainly title deeds, 1476-1880, relating to lands in Anglesey, Caernarfonshire, Denbighshire, Flintshire and Merionethshire, and estate correspondence, mainly 1781-1857.

Deeds, relating to the Plas Tregayan estate in Anglesey and Merioneth, 1810-1926, and associated estates, namely Llwyn Onn in Denbighshire, [late 13 cent.]-1879, Madryn estate in Caernarfonshire, 1638-1831, Aberdunant estate, Anglesey, Caernarfonshire and Merioneth, 1845-1902, and Cesailgyfarch estate, Caernarfonshire, 1638-1897.