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Papers, 1889-1988, of Ben G. Jones, including academic notes, 1932-1935; personal letters, 1942-1968; political papers, 1935-1985; correspondence relating to politics in Merionethshire, 1963-1967; press cuttings, 1958-1963, printed material relating to the four main political parties in Wales, 1949-1966; papers relating to the Honourable Society of Cymmrodorion, 1939-1988; minute book, 1889-1909, of the London Welsh Mutual Improvement Societies' Union; papers deriving from the compilation and publication of the Dictionary of Welsh Biography, 1953-1986; papers relating to his public life, 1968-1984, including the Kilbrandon Commission, 1936-1969, the BBC, 1968-1978, UCW Aberystwyth, 1968-1985, and the Agricultural Land Tribunal, 1980-1984; minute book, 1889-1909, of the London Welsh Mutual Improvement Societies' Union; and papers relating to the status of the Welsh language and to teaching and broadcasting through the medium of Welsh, 1965-1987.

Papers of Stuart Rendel and family members, including papers relating to the University College of Wales, Aberystwyth, and the proposal to establish the National Library of Wales and its development during the early years of its existence, 1883-1916; speeches, addresses and political papers relating to disestablishment of the church in Wales and the 1889 Intermediate Education Act, 1882-1909; press cuttings, 1881-1913; photographs, 1892; miscellaneous letters, 1878-1912; letters to Stuart Rendel, 1853-1912, including letters from A. C. Humphreys Owen, 1877-1905, family letters, 1853-1902, and letters from prominent political figures and Welsh public figures; letters and copies of letters from Rendel, 1880-1912; diaries, mainly recording details of Stuart Rendel's business activities, 1863-1869; notes of conversations with W. E. Gladstone, John Morley and H. H. Asquith, 1888-1910; papers relating to Chinese affairs and French and Chinese peace talks, 1884-1886; papers of James Meadows Rendel, including letters, 1828-1856, and papers relating to his estate, 1856-1859; letters of Catherine Jane Rendel, 1845-1855; letters and papers of George Wightwick Rendel, 1871-1902; papers relating to Rendel's other brothers, 1841-1889, and his daughters, 1882-1910; letters and papers of Harry Stuart Goodhart-Rendel, 1898-1959, and other papers concerning him, 1963-1977; papers, mainly letters, of the Goodhart family, 1819-1957; papers of Miss Rosemary Rendel, 1986-1996; papers of Sir George William Rendel, including: Foreign Office papers, 1917-1967, correspondence, 1912-1973, papers relating to the Catholic Union of Great Britain, 1942-1979, lectures, diaries and notes, 1915-1954, personal and family papers, 1908-1980, and material relating to the book The Sword and the Olive (1957), 1954-1986.