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Papers of Stuart Rendel and family members, including papers relating to the University College of Wales, Aberystwyth, and the proposal to establish the National Library of Wales and its development during the early years of its existence, 1883-1916; speeches, addresses and political papers relating to disestablishment of the church in Wales and the 1889 Intermediate Education Act, 1882-1909; press cuttings, 1881-1913; photographs, 1892; miscellaneous letters, 1878-1912; letters to Stuart Rendel, 1853-1912, including letters from A. C. Humphreys Owen, 1877-1905, family letters, 1853-1902, and letters from prominent political figures and Welsh public figures; letters and copies of letters from Rendel, 1880-1912; diaries, mainly recording details of Stuart Rendel's business activities, 1863-1869; notes of conversations with W. E. Gladstone, John Morley and H. H. Asquith, 1888-1910; papers relating to Chinese affairs and French and Chinese peace talks, 1884-1886; papers of James Meadows Rendel, including letters, 1828-1856, and papers relating to his estate, 1856-1859; letters of Catherine Jane Rendel, 1845-1855; letters and papers of George Wightwick Rendel, 1871-1902; papers relating to Rendel's other brothers, 1841-1889, and his daughters, 1882-1910; letters and papers of Harry Stuart Goodhart-Rendel, 1898-1959, and other papers concerning him, 1963-1977; papers, mainly letters, of the Goodhart family, 1819-1957; papers of Miss Rosemary Rendel, 1986-1996; papers of Sir George William Rendel, including: Foreign Office papers, 1917-1967, correspondence, 1912-1973, papers relating to the Catholic Union of Great Britain, 1942-1979, lectures, diaries and notes, 1915-1954, personal and family papers, 1908-1980, and material relating to the book The Sword and the Olive (1957), 1954-1986.

Papers of D. A. Thomas, Viscount Rhondda, including letters to D. A. Thomas on political matters such as working conditions in the mining industry, education, church disestablishment, and the temperance movement, 1891-1910 (mainly 1891-1895); drafts and copies of letters from D. A. Thomas on similar subjects, 1891-1895; miscellaneous letters, 1893-1895; subject files, 1874-1917, on the coal industry, including the Cambrian Navigation Collieries, the Mining Association of Great Britain, the South Wales Liberal Federation, temperance and disestablishment; scrapbooks of press cuttings, 1894-1927, relating to Cymru Fydd, D.A Thomas, Merthyr politics and Keir Hardie, the Lusitania, and Lady Rhondda; miscellaneous items, 1897-1934, including genealogical material and congratulatory addresses to D.A.T.; circulars and memoranda.

Papers of Tom Owen, HMI, of Aberystwyth, Cardiganshire, 1898-1966, mainly relating to his career in education, including inspector's reports on schools in Montgomeryshire, 1946-1950; reports on St. David's College, Lampeter, Cardiganshire, 1907-1945; and personal papers, 1898-1966.

Records accumulated by Dr John Herbert, 1968-1984, comprising Welsh Secondary Schools Association records, minutes and papers, 1968-1984; and Headmasters' Association and Secondary Heads Association minutes, correspondence, discussion papers and related material, 1969-1984.

Records of the Association of Welsh Local Authorities, 1928-1976, including minutes of annual meetings, 1952-1973; minutes of council meetings, 1952-1973; cash books, 1958-1973; administration papers, 1953-1976, papers relating to the withdrawal of railway services in Wales, 1962-1970; and subject files, 1952-1974, relating the interests and activities of the Association, such as water resources, transport, education, and the Welsh economy.

Papers of Sir Evan Vincent Evans, 1880-1933, including correspondence, 1881-1927 (comprising general correspondence to Sir E. Vincent Evans, 1881-1927, letters relating to the Ignatius Williams manuscripts, 1906-1922, drafts and copies of letters from Vincent Evans, 1893-1927, letters addressed to others, 1892-1923; and miscellaneous letters, 1894-1927, mainly those with unrecognisable signatures); bibliography of Welsh printed books, 1701-1807; minutes of the Board of Celtic Studies, 1933; records of the Diphwys Slate Quarry, 1924-1927; papers relating to education in Wales, 1887-1888; the London Committee of the Cardiff Medical Society, 1890; the National Eisteddfod of Wales, 1887-1926; the National Library of Wales, 1924-1927; the National Museum of Wales, c. 1900-1928; the Royal Commission on Ancient Monuments in Wales, 1911-1933; Royal Commission on Public Records, 1914-1916; the Society for the Promotion of Nature Reserves, 1914; the University Board of Celtic Studies, 1922-1927; the University of Wales, c. 1893-1927; the Vincent Evans Testimonial Fund, 1898-1899; and the Welsh Club, 1893-1913; together with copies of speeches and addresses delivered by Vincent Evans; and miscellaneous papers, [c. 1880]-[1930].

Papers of Victor Hampson-Jones, 1881-1975, comprising lectures and speeches, 1966-1973, teaching notes, radio scripts, 1966-1975, material relating to lawsuits and tribunals involving trades union members, 1960-1975, material relating to Undeb Cenedlaethol Athrawon Cymru, 1953-1972, and personal and family papers, 1881-1973.

Press cuttings relating to Wales and Welsh culture, such as religion, politics, literature, music, education, St. David's Day celebrations and the Eisteddfod Genedlaethol, individuals, and the National Library of Wales [1895]-[1939].

Papers of Sir Ben Bowen Thomas (1899-1977), educationalist and public servant, comprising autobiographical material on his career, interests and family, 1954-1972; biographical articles and an interview, 1964-1966; letters to his wife and daughter with references to his work with UNESCO and Welsh educational matters, 1947-1960; letters from Dr Thomas Jones and Sir Percy E. Watkins relating to educational issues and Coleg Harlech, 1926-1955; correspondence concerning BBT's work with UNESCO, 1954-1962; miscellaneous correspondence, 1948-1976; addresses and speech notes, 1949-1977; pamphlets, offprints and articles, 1941-1973; research notes on regions and towns of Wales during the 18th and 19th centuries; circulars, articles, reports, etc. relating to education and educational bodies in Wales, 1942-1975, to UNESCO, 1946-1958, and to public and cultural bodies such as the Welsh Language Council, ITA and the Rural Development Board, 1965-1973; McNair Report on the Training of Teachers, 1942-3; memorials, tributes and obituaries of other educationalists; and miscellaneous press cuttings and notes. The archive also includes a collection of sermon notes and exercise books of his grandfather, the Rev. Benjamin Thomas, (1838-1913), a Baptist minister in Ystrad Rhondda, Glamorgan.

Records accumulated by John Clement as a civil servant, 1942-1958, including records of the Welsh Reconstruction Advisory Council, 1942-1945; records relating to education and hill sheep farming, 1942-1943; papers relating to the Welsh woollen industry, 1954-1958; and records relating to the Council for Wales and Monmouthshire, 1954-1958.

A further box of papers was received August 2007. This group remains uncatalogued.

Records of the National Curriculum History Committee for Wales, 1978-1995, including papers relating to the establishment and subsequent meetings of the National Curriculum History Committee for Wales, 1989-90; minutes, agenda, reports and articles for discussion at various meetings of the National Curriculum History Working Group, 1989, the History Development Group, 1990, The Historical Association, 1986-89, and the Association of History Teachers in Wales, 1988-9; copies of a WJEC report and examination papers, 1986-93; papers relating to assessment by the School Examinations and Assessment Council, 1989; correspondence from MPs and others, 1988-91; miscellaneous articles, reports, press cuttings and papers relating to teachers' conferences, 1978-93; and printed material on the teaching of history in Welsh schools, 1979-95.

The collection comprises John Owen's diaries, 1889-1926; notebooks containing press cuttings, accounts, extracts from the Bible and historical notes; and an address book (box 1); the memoirs of John Owen entitled 'College Friends', letters, 1872-1894, including many letters concerning the tithe rent charge, papers on the 1889 Welsh Intermediate Education Bill (box 2); a catalogue of the books in the library of Bishop John Owen, 1908, speeches, draft speeches and sermons, letters and papers relating to the disestablishment and disendowment of the church in Wales, papers concerning educational matters, 1891-1895 (box 3); letters, 1893-1897, many on religious matters, including issues of church reform, some of family interest, some congratulating John Owen as Bishop of St Davids in 1897 (box 4); an incomplete manuscript, the final printers' copy and the typescript text of 'The Early Life of Bishop Owen' (box 5); letters, 1898-1905, some relating to sermons and prayers following the death of Gladstone, the 1902 Education Bill, church defence, the fire at the Bishop's Palace at Abergwili in 1903, the new Bishop of Llandaff in 1905, and matters of diocesan interest, and there are also papers, 1904-1905, concerning education, Lloyd George and the Western Mail (box 6); letters, 1897-1914, some relating to the proceedings of the Welsh Church Commission, diocesan matters, church defence etc. (box 7); correspondence and papers, 1914-1917, many relating to the disestablishment and disendowment of the Church in Wales, the Welsh Church Act, 1914, and related matters (box 8); letters, 1906-1915, some relating to the role of the church in politics, education, church defence, the Welsh Church Bill etc. (box 9); correspondence and printed material, 1914-1919, concerning disestablishment, the Welsh Church Act, the Postponement Bill and the war, the tithe and disendowment (box 10); letters and papers, 1910-1926, concerning the tithe and the Welsh Church Bill, the Welsh Church Act, the Church Commissioners, matters relating to the diocese of St Davids (box 11); bundles of letters, 1922-1926, relating to church and diocesan matters, disestablishment and finance (box 12); correspondence and papers, 1914-1926, relating to disendowment, the government of the Church in Wales, the constitutions of the Governing Body and the Representative Body of the Church in Wales, drafts, notes and correspondence concerning 'The Later Life of Bishop Owen' (box 13); papers, 1907-1918, concerning Bishop Owen's life and work, including the typescript draft of 'The Early Life of Bishop Owen' (box 14); typescript drafts of 'The early Life of Bishop Owen' (box 15); manuscript texts of 'The Later Life of Bishop Owen', and miscellaneous source materials relating to Bishop Owen's life and work (box 16); papers concerning church matters, 1889-1925, including material relating to the Ecclesiastical Commissioners, the Representative Body of the Church in Wales, the 'Diocesan Board of Finance', the 'Million Pound Fund' appeal, commutation capital, the St Davids Board of Finance etc., together with the correspondence of Miss Eluned Owen, 1954-1965 (box 17); papers relating to voluntary and parochial contributions, 1905-1908, together with an extensive collection of press cuttings (box 18).
Additional papers (boxes 19-21) comprising the letters of Bishop John Owen, his wife Amelia Owen and their family, together with the recollections of their daughter, Gwenonwy Davies, and of her husband the Very Reverend J. T. Davies, Dean of Bangor, were received in August 2017.

Papers, 1889-1988, of Ben G. Jones, including academic notes, 1932-1935; personal letters, 1942-1968; political papers, 1935-1985; correspondence relating to politics in Merionethshire, 1963-1967; press cuttings, 1958-1963, printed material relating to the four main political parties in Wales, 1949-1966; papers relating to the Honourable Society of Cymmrodorion, 1939-1988; minute book, 1889-1909, of the London Welsh Mutual Improvement Societies' Union; papers deriving from the compilation and publication of the Dictionary of Welsh Biography, 1953-1986; papers relating to his public life, 1968-1984, including the Kilbrandon Commission, 1936-1969, the BBC, 1968-1978, UCW Aberystwyth, 1968-1985, and the Agricultural Land Tribunal, 1980-1984; minute book, 1889-1909, of the London Welsh Mutual Improvement Societies' Union; and papers relating to the status of the Welsh language and to teaching and broadcasting through the medium of Welsh, 1965-1987.

Papers of Trevor Lovett, 1943-1980, relating mainly to secondary education, including personal papers 1944-1970; papers relating to Holyhead County Secondary School, 1949-1971; papers relating to secondary education in Anglesey, 1959-1980; press cuttings relating mainly to comprehensive education, 1945-1975; together with other papers relating to comprehensive education in England and Wales, 1962-1976, and miscellaneous papers, 1943-1969.

Diaries etc, 1903-1930; sermons; addresses and articles, 1916-1948; correspondence, notes and articles relating to penal reform, 1907-1917, Ireland, 1920-1924, education, 1925-1931, reparations, 1926-1931, Tom Nefyn Williams, 1926-1931, and the Fellowship of Reconciliation, 1916-1947; poetry, 1900-1947; genealogical and miscellaneous notes and family papers, 1884-1926; articles and addresses by various authors, 1903-1949; letters to and from George M. Ll. Davies, other members of the family and others, 1826-1964.