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A manuscript volume, [1747x1748], written by an unidentified scribe, entitled 'A Catalogue of the Representatives in Parliament for the Counties & Boroughs In Wales From the first returns of them A[nn]o 1542 to this present Parliament Conven[e]d A[nn]o 1747' (f. 4), listing the Members of Parliament of all county and borough seats in Wales, with the exception of Monmouthshire and Monmouth (ff. 5-62).
The seats are listed alphabetically by county with MPs then listed chronologically by monarch and regnal year; the Parliaments of the Commonwealth and Protectorate periods are omitted.

Papers, 1889-1988, of Ben G. Jones, including academic notes, 1932-1935; personal letters, 1942-1968; political papers, 1935-1985; correspondence relating to politics in Merionethshire, 1963-1967; press cuttings, 1958-1963, printed material relating to the four main political parties in Wales, 1949-1966; papers relating to the Honourable Society of Cymmrodorion, 1939-1988; minute book, 1889-1909, of the London Welsh Mutual Improvement Societies' Union; papers deriving from the compilation and publication of the Dictionary of Welsh Biography, 1953-1986; papers relating to his public life, 1968-1984, including the Kilbrandon Commission, 1936-1969, the BBC, 1968-1978, UCW Aberystwyth, 1968-1985, and the Agricultural Land Tribunal, 1980-1984; minute book, 1889-1909, of the London Welsh Mutual Improvement Societies' Union; and papers relating to the status of the Welsh language and to teaching and broadcasting through the medium of Welsh, 1965-1987.

One hundred and twenty-four autograph letters, 1959-1974, from painter-poet David ('Dafydd') Jones, all addressed to Valerie ('Elri') Wynne-Williams (née Price), with the exception of two to her husband Michael ('Mihangel') (ff. 54, 112-113) and one to them both (ff. 55-56), discussing a variety of topics including his, and her, health and living conditions, his work, his friends, the Welsh language and Welsh history and politics. Some letters are illustrated with coloured pencil, pen and ink drawings, mainly of animals and flowers (ff. 8, 32, 33, 45 verso, 46 verso-47, 48 verso, 76, 103, 104 verso, 152), inscriptions (ff. 9, 34, 124 verso, 128, 136 verso) and sketch maps of Harrow (ff. 143, 144).
There are references throughout to friends and correspondents including Saunders Lewis (ff. 2-11 passim, 42-188 passim), Harman Grisewood (ff. 4-192 verso passim), René Hague (ff. 42 verso-187 passim), David Blamires (ff. 160, 186, 190 verso, 192), Louis Bonnerot (ff. 123, 186 verso), Tom Burns (ff. 13, 14 verso, 48, 64 verso, 68 verso, 77, 85 verso, 86 verso, 89 verso, 110, 116, 140 recto-verso, 188 verso), Douglas Cleverdon (ff. 68 verso, 160 verso, 162, 163 verso, 187), Aneirin Talfan Davies (ff. 9 verso, 11, 14 verso, 16, 33 verso, 63 verso, 71 verso, 123, 124, 128, 129 verso, 154 verso, 162), Clarissa Eden (f. 107 verso), T. S. Eliot (ff. 51 recto-verso, 62 verso, 67 verso, 69 verso, 71, 73, 74, 85), Gwynfor Evans (ff. 29 verso, 31, 131-192 verso passim), Illtud Evans (f. 6, 11 recto-verso, 37, 46 verso, 57, 61), Arthur Giardelli (ff. 150, 151 verso, 171 verso, 186), Eric Gill (ff. 45 verso, 66, 67 verso, 68 verso, 121), Stanley Honeyman (ff. 84, 140, 154 verso, 159 verso), Morag Owen (ff. 59, 98, 140), Catherine Rousseau (née Ivainer) (ff. 36 verso-127 passim), Stephen Spender (ff. 81 verso-82, 83 verso, 91), Bill Stevenson (f. 158 verso) and Helen Sutherland (ff. 68, 97 verso, 157). There are also occasional references to Desmond Chute (f. 120 verso), Idris Foster (ff. 60 verso, 63 verso), Philip Jones Griffiths (ff. 1, 131), David Lloyd George (ff. 108 verso-109, 127 verso), Megan Lloyd George (ff. 18 verso, 20, 21-22), J. D. Innes (f. 49 verso), Augustus John (f. 85 verso), Alun Oldfield-Davies (ff. 37, 77), Tristram Powell (ff. 142 recto-verso, 144), Caradog Prichard (ff. 19 verso, 77, 108), Kathleen Raine (f. 59 verso), Keidrych Rhys (ff. 6 verso, 8, 9, 16, 30 verso, 36 verso), Meic Stephens (ff. 171, 175), Vernon Watkins (ff. 47, 128 verso), D. J. Williams (f. 106 recto-verso), Kyffin Williams (ff. 49, 63, 77) and R. O. F. Wynne and his family (ff. 61, 62, 63, 64 verso, 67 verso, 81, 94 verso, 96 verso¸ 98, 130 verso), and brief reminiscences of his experiences during the First World War (ff. 70 recto-verso, 76, 79 recto-verso, 108 verso-109, 130 recto-verso, 151 verso, 164). Also included is a copy of his letter, dated 10 August 1959, to Megan Lloyd George (f. 21; for her reply see NLW, David Jones (Artist and Writer) Papers CT3/3, f. 247); cuttings of letters to the Times by David Jones, Valerie Price and others, 1958 (ff. 193-196); and a copy of a 1959 photograph of the two by Philip Jones Griffiths (f. 197). The letter of 23 September 1973 (ff. 178-179 verso) was published under the title 'Yr Iaith' in Planet, 21 (January 1974), 3-5.

Papers, 1968-2006, of the Reverend David Morris relating to his interests in political and social issues, his career as MEP for Mid and West Wales, and later MEP for South Wales West, and his work as a Presbyterian minister.

Papers, correspondence and press cuttings relating to Ireland, 1926-1978; Plaid Cymru, 1929-1965; Welsh political, economic and social affairs, 1931-1962; Pantybeiliau Folk School, 1933-1938; world economics, socialism and communism, 1934-1951; and Brittany, 1946; and personal papers, including correspondence, 1924-1978, diaries, 1921-1979, and academic papers, 1922-1946.

Letters, newspaper cuttings, notes, pamphlets and periodicals, typescripts, reports, volumes of parliamentary debates, and other papers of James Griffiths relating to the following: the coal industry and the South Wales Miners' Federation, 1912-1967; the Labour Party, 1919-1975; the Central Labour College, 1919-1922; National Insurance, 1931-1954; the Colonies, 1939-1972; his work as Secretary of State for Wales, 1964-1966; papers relating to Welsh affairs including devolution, the Welsh Reconstruction Advisory Council, education and local government reorganization, 1935-1975; constituency affairs, 1937-1969; overseas visits, 1936-1968; the Nigeria-Biafra War, 1968-1970; papers relating to his autobiography Pages from Memory, including letters from Gwilym Prys Davies and others, 1961-1969, notebooks, [1960s], typescripts, [1964]-1969, and cuttings of reviews, 1969; unpublished reminiscences, 1955-1974; notes and typescripts for lectures and speeches, 1940-1971; typescripts of broadcasts by Griffiths, 1937-1967; typescripts of articles and reviews, 1940-1974; newspaper cuttings, 1919-1974; and other miscellaneous personal matter, [1930s]-1975; and papers relating to Mrs Silyn Roberts, 1897-1954.