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Papurau'r Coleg Cymraeg Cenedlaethol, 2001-2011, gan gynnwys cofnodion grwpiau pwyllgor, ffeiliau yn ymwneud a phrosiectau, gohebiaeth, papurau marchnata a phapurau amrywiol eraill.

Some sixty letters, 1886-1913, to Alfred Thomas, 1st baron Pontypridd, relating mainly to national and local politics and to secondary and university education in Wales. The correspondents include Sir Edward Anwyl (1) 1905, Henry Austin Bruce, Lord Aberdare (1) 1886, Sir D. Brynmor Jones (2) 1900, J. Viriamu Jones (3) 1900, Sir Isambard Owen (1) 1893, Robert Threshie Reid, Lord Loreburn (4) 1908-1911, Lord Rendel (2) 1899, 1902, and Charles Vaughan, dean of Llandaf (6) 1888-1897.

Administrative records of the University of Wales from its establishment in 1893 comprising papers relating to the foundation of the University; records of the University Court, Guild of Graduates, the Senate, Academic Board, University Council, Board of Celtic Studies, University of Wales Press Board, The Committee of Principals, Registrar's papers; records of committees, sub-committees and ad hoc committees created by, or answerable to, the Court, the Council, the Academic Board, etc., and printed materials. The archive is a fundamental source for the history of the University and for University education in Wales; to the development and provision of bilingual education in higher education in Wales, and, to a lesser extent to education in general in twentieth-century Wales.