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Welsh School, Ashford, and British Charity School, Board of Governors and trustees minutes, 1718-1848; House Committee minutes, 1830-1905; cash books and financial records, 1792-1905; applicants books, 1826-1844; correspondence and papers, 1760-1904; correspondence and records of the Society for the Diffusion of Useful Knowledge in Wales, 1849-1851; correspondence relating to Llandaff Diocesan Commitee, 1849; and deeds and legal correspondence relating to lands in Ashford, Middlesex, 1845-1893; minute books of the Society of Ancient Britons, 1823-1856, and of the Cymmrodorion, 1828-1849.

A further deposit of papers comprising committee minute books (5), 1905-1987; household wages books (4), 1949-1958; accounts books (3), 1846-1974; receipts and payments books (7), 1813-1963; apprenticeship book, 1852-1853; letters book, 1839-1849; Schoolmistress report book, 1868-1882; attendance and fee register, 1923-1940; confirmation book, 1916-1964; school reports, 1848-1873; house mark book, 1941-1956; House Committees visiting book, 1880-1891; cash books (3), 1932-1956; general fund book, 1949-1958; inventory and valuation book, 1946; school numbers book, 1945-1957; and an investments book, 1940-1949.

Papers, [1939]-2007, pertaining to the school, accumulated by Jacqueline Flindall, a former pupil of the Welsh Girls' School, including letters and items relating to the 150th anniversary celebrations in 2007.

Papers of Trevor Lloyd Williams, 1859-1946, comprising scrapbooks of press-cuttings, letters, notebooks and ephemera relating mainly to his family, in particular to Rev. John Morris, Rev. John Lloyd Williams, Rev. Thomas Nicholson, Rev. W. Pedr Williams, and Ivor Percy Nicholson; also included are notebooks of Trevor Lloyd Williams containing transcripts of documents and notes relating to Welsh history.

Papers of and collected by T. J. Evans, 1843-[c. 1950] , comprising materials of Welsh interest, such as press cuttings, notebooks and research notes, relating to subjects such as various eminent Welshmen, London Welsh, the establishment and early development of the National Library of Wales and Welsh orthography; and including volumes containing poetry and papers relating to poetry, composed by T. J. Evans and other poets; and correspondence.

Papers mainly relating to the published work of Herbert Stanley Jevons, 1895-1963, correspondence on overseas development, coal and economics, 1909-1949; correspondence on housing in Wales, 1912-1914; papers relating to Ethiopia, 1935-1955, including correspondence with Emperor Haile Selassie I, 1937-1953; letters between Herbert Stanley Jevons and John Maynard Keynes, 1930-1936.

Deeds (mainly drafts) and estate correspondence, 1849-1862, relating to the Burghill estate, and papers (apparently unrelated to the Chirk Castle estate) of Mary Coats of Crompton Street, St Anne, Westminster, 1768-1782.