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The catalogued material comprises two groups of deeds and other documents relating to lands of the Bodwenni and Syrior estates in Merionethshire, Denbighshire and Montgomeryshire, and to the Roberts, Williams and Evans families of Bodwenni and Syrior, [13th century]-1833; miscellaneous literary manuscripts, [16th century]-[19th cenury]; and printed material. Uncatalogued material includes deeds, family papers and correspondence, 1609-1953.

A late seventeenth century notebook of William Roberts, Bodwenni, Llandderfel, co. Merioneth, containing transcripts of Latin texts (Greek and Roman biographies, 'Dictamen de bonis moribus', etc.), with English translations, written in 1681; notes of sermons by Mr. Jenkin Thomas (once at Llanvilling), Mr. H. Owens [of Bronyclydwr, Llanegryn], and Mr. Morg[an] Tho[mas] (once at Hendre), 1695-1696; miscellaneous memoranda (payment for wheat at Corwen fair, payment of Bodwenni tithe, the tenancies of tenements in Llandderfel, etc.), 1694/5-1696; 'Phrases ex Erasmo'; extracts from Ovid's Metamorphosis; a Greek-Latin vocabulary; etc.