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Letters written to T. E. Ellis, 1876-1899, from correspondents including A. H. D. Acland, D. R. Daniel, Ellis Jones Griffith, Lord Rosebery and others; drafts and copies of letters by T. E. Ellis, [c. 1879]-1899; miscellaneous correspondence and papers concerning T. E. Ellis, 1886-1929; diaries, 1889-1897; newspaper cuttings, printed matter, notes, petitions and papers on political matters, 1877-1910; and family papers, consisting mainly of letters to Mrs T. E. Ellis, 1897-1929.

Papers of Arthur John Williams, 1881-1943, including political papers comprising letters, 1868-1911; papers relating to legal, electoral and land reforms, 1867-1911; papers relating to his parliamentary elections in Birkenhead and Glamorgan, 1880-1895; papers relating to South Glamorgan politics, 1886-1924; material concerning the National Liberal Club, 1883-1951; diaries, 1864-1911; diaries of Rose Harriette Thompson Crawshay 1868-1943; and family and financial papers, 1767-1943.

Papers, 1844-1941, of the Williams family of Acre House, Acrefair, mainly comprising letters, including family correspondence and letters received from relatives in Glamorgan, from the Pugh family, and from relatives in the USA, [late 19th cent.]-[early 20th cent.]; letters to the Rev. Ebenezer John Williams, mostly relating to his duties as minister and the chapel and water works in Llanwddyn, 1882-1889; and letters to John Williams, [late 19th cent.], mostly relating to the iron industry. The archive also includes diaries of John Williams, 1844-1897; notebooks, accounts and other documents, 1856-1893, relating to the ironworks in Ruabon and South Wales; diaries and notebooks of the Rev. Ebenezer John Williams, 1869-1935 (including chapel committee notes, accounts, Sunday School registers, and sermon notes); diaries and notebooks of Rev. John Pugh, 1849-1890, (including one containing his autobiography); papers relating to Liberal Party election campaigns in Montgomeryshire and Denbighshire, [late 19th cent.]; deeds, 1842-1921, mostly relating to property in Dowlais; papers relating to schools, [late 19th cent.]-[early 20th cent.], including school notebooks, prospectuses of schools including Holt Academy, and papers relating to the founding of British schools in the Cefn Mawr district and elsewhere.