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Letters, 1855-1904, of miscellaneous provenance, including letters, 1871-1894, to and from Welsh emigrants to Australia and the United States of America (ff. 11-24, 49-50, 69-70, 108-123); a letter, 1855, from the artist Penry Williams relating to a proposed visit by Lady Charlotte Guest to the Vatican; and a letter, 1857, from the Rev. Calvert Richard Jones, photographic pioneer, to his friend Christopher Rice Mansel Talbot of Margam, written from Nice. Other correspondents include Owen M. Edwards (1) 1891, Thomas E. Ellis (1) 1892, David Lloyd George (5) 1879-1892, William E. Gladstone (3) 1857-1875, Sir Lewis Morris (2) 1890-1895, Daniel Owen (1) 1885 and John Thomas (Pencerdd Gwalia) (4) 1891-1904.

Papers, 1715-1985, of miscellaneous provenance, including a brief memoir [watermark 1794] of Richard Wilson by Joseph Farington, apparently unpublished (ff. 5-7); a transcript of the regulations, 1795, regarding the charges for crossing the ferry at Llandeilo (ff. 174-5); scenario and cast, [c. 1807], of 'Miller of Mansfield', a play, apparently unpublished, for performance in the theatre at Wynnstay by members of the Wynn family and their friends (ff. 179-84); autograph fragments of 'De Chatillon' and of the original manuscript of The Vespers of Palermo by Felicia Hemans (ff. 9, 178); a copy of the fourth Report, 1832, of the Anglesey branch of the Royal National Institution for the Preservation of Life from Shipwreck (see also NLW MS 1600E and Anglesey Antiquarian Society and Field Club Transactions 1957, 20-5) (ff. 53-4); draft lecture notes, [c. 1846]-1847, of the Rev. Calvert Richard Jones, photographic pioneer, describing his visit to Malta during the winter of 1845-1846 and containing his observations on evidence in favour of St Paul's shipwreck having occurred in Malta (ff. 98-101); and a copy of a special typescript issue of the North Wales Chronicle, 6 May 1926, outlining the state of the country during the general strike of 1926 (ff. 102-3).