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The 1939 deposit consists of deeds and documents, 1549-1887, relating to properties in Montgomeryshire, Merionethshire, Breconshire and Shropshire. The 1973 deposit mainly contains deeds and documents, 1564-1932, relating to properties in Montgomeryshire, many relating to the Lloyd family of Montgomery. The 1979 deposit comprises materials gathered by J. D. K. Lloyd for a History of Montgomery; a bundle of deeds and documents, [19 cent.]-[20 cent.], relating to the family of Lloyd of Plas Trefaldwyn, Montgomery, and Castell Forwyn, Abermule; photographic albums, 1898-1978, comprising mainly family photographs; a collection of over 1000 postcards and photographs of historic buildings throughout Europe; and seven manuscript maps of land in Montgomeryshire, 1772-1858.

Deeds, 1554-1915, relating to the Neuadd-fawr estates in Breconshire, Carmarthenshire, Cardiganshire and Radnorshire; together with some papers relating to the development of Llanwrtyd Wells, Breconshire, as a spa in the nineteenth century.

Deeds, estate correspondence and legal papers, 1361-1874, relating to the Skreen and Velin Newydd estates, in Radnorshire, Breconshire, and, to a lesser extent, in Monmouthshire, 1361-1874.