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The collection comprises volumes of primary records, 1922-1950, (including executive committee minutes, north Wales committee minutes, finance committee minutes, cash books, ledgers, campaign committee minutes, general purposes committee minutes); the records of the Welsh National Council of the League of Nations Union, 1920-1945; minutes of the committees of the League of Nations Union, 1925-1939; minutes of the sub-committees of the League of Nations Union, 1927-1942. Secondary records of the League of Nations Union: general meetings, 1928-1938; national meetings, 1928-1937; conferences, 1922-1937; committees, 1922-1938; financial records, 1925-1938; educational records, 1922-1946; publications, 1923-1932; publicity, 1929-1947; personal files, 1922-1939; enquiries, 1922-1938; formation of branches, 1923-1938; reports, 1924-1938; London headquarters, 1923-1938; general files, 1922-1951. Branch files, 1922-1940; weekly returns relating to membership etc., 1922-1934; membership, county files etc., 1930-1938; Headway notes, correspondence, press cuttings etc., 1922-1938; League of Nations Union miscellaneous papers, 1923-1939. United Nations Association general files, 1943-1954; United Nations Association committees, 1943-1965; United Nations Association sub-committees, 1947-1952; UNA finance, 1940-1961; UNA membership, 1946-1964; UNA accounts, 1951-1960; UNA 'Files from a series designated letter/number', 1961-1967; UNA branches, 1943-1950; League of Nations Union/UNA meetings, 1944-1964; Temple, 1939-1957; personal files, 1943-1950s; educational themes, 1944-1950; Newsletters, 1961; UNA conferences, 1962-1967; UNA campaigns, 1964-1966; Youth against Humger/Council for Education in World Citizenship Competitions, 1965-1967. Goodwill message: replies to children's wireless message (CWM), 1925-1929; replies to CWM, 1930-1938; CWM related material, 1935-1938; material relating to World Children's Message up to 1939, arranged by countries, 1927-1938; replies to CWM, 1939, arranged by countries; CWM lists of replies, 1928-1939; WCM, copies of replies, correspondence etc., 1938-1959.

Personal correspondence, 1916-1954; study notes, 1902-1952; biographical material, 1903-1954; notebooks entitled 'Tennyson Biography'; sermons and addresses, 1932-1952; orders of service for Victory, 1945, the United Nations 1946, Human Rights Day, 1951-1954, the Coronation and other occasions, 1931-1954; religious and international affairs, 1944-1945; Welsh Book Festivals, 1935-1938; Welsh School of Social Service, 1911-1940; The Gregynog Conferences on International Education, 1922-1937; Advisory Education Committee minutes, 1926-1929; international co-operation, 1933-1937; Welsh nationalism, 1910-1943, including nationalists' attitudes towards World War II, 1939-1941; broadcasting materials mostly of Marconi and Kemp, 1931-1953; Welsh broadcasting, 1923-1948; the Welsh Children's Peace Message, Pageant, and Wales and the Peace Movement, 1923-1955; BBC staff changes and administration in Wales, 1934-1952; the League of Nations, 1923-1952; the Welsh National Council of the League of Nations Union, 1923-1945; United Nations, 1942-1954; UNESCO, 1925-1947; addresses, radio talks and notebooks on the international situation, 1930-1954; Council for Education in World Citizenship, 1940-1950; London International Assembly, 1941-1944; Welsh Committee of the UNESCO, 1949-1953 and human rights materials, 1945-1953.

Papers relating to the Welsh National Council of the League of Nations received by Mr J. R. Thomas, including an appreciation of his services and support to the Peace Ballot, 1934-35.