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Miscellaneous holograph letters and documents including letters, 18 January, 1667/8 and 15 August, 1668, relating to an action on behalf of [John] Morris and [Robert] Clayton for the recovery of iron at Pembroke; two letters, 16 May - 1 June, 1668, to [John] Morris or [Robert] Clayton relating to the lading of cinders; a covenant, 30 September, 1679, for the observance of an award of Sir Edward Mansell, bart, and Bussy Mansell concerning the purchase of properties in Ewenny, Colwinston, and Llangan, Glamorgan; two recommendations, 18 May-26 June, 1687, signed by Henry Somerset, 1st duke of Beaufort, of persons fit to be put into the commission of the peace for the counties of Gloucester, Monmouth, Denbigh, Caernarvon, Anglesey, and Brecknock; a letter, 7 June, 1687, from William Herbert, 1st marquis of Powis, to [George Jeffreys, 1st baron Jeffreys of Wem] (recommending the appointment of a Clerk of the Peace for Montgomeryshire); a letter, 16 September, 1688, from [Sir] Wi[lliam] Williams ['Speaker Williams'] from Glascoed, 'near Oswestry', to [George Jeffreys, 1st baron Jeffreys of Wem] (the forthcoming parliamentary elections for Anglesey, Wallingford, etc.); papers, 1736, 1745, 1756, relating to the Lloyd family of Alltycadno, Carmarthenshire; an attested copy of the will, 15 June, 1782, of George Philipps of Coedgaing, Carmarthenshire; etc.

Papers of Sir William Williams, mainly legal papers, 1685-1693; political papers, 1680-1698; and papers relating to, or collected by his ancestors or descendants, 1567-1812. The legal papers include papers relating to the trials of the Earl of Shaftesbury, 1677, Algernon Sidney, 1683, his own trials for a scandalum magnatum brought by James II and the Earl of Peterborough, 1685-1686, and the trial of the Seven Bishops, 1688.

Estate and family records, 1183-1957, of the Wynn and Williams Wynn family of Wynnstay, Denbighshire. The archive includes a group of architectural drawings, c. 1770, by James Byres; a group of early charters and deeds, 1183-1676, from the Cistercian Abbey of Strata Marcella (Ystrad Marchell) near Welshpool, Montgomeryshire, and elsewhere; antiquarian, legal and literary manuscripts; account rolls of Sir Richard Wynn, Treasurer to Queen Henrietta Maria, 1627-1649; manorial records relating to manors and boroughs in Denbighshire, Montgomeryshire and Shropshire, 1364-1895 (1934-40 and 1952 deposits); parliamentary election papers for Anglesey, Cardigan (county and borough), Denbighshire, Flintshire and Montgomeryshire, 1621-1883; family and estate correspondence, including part of that of Sir William Williams (1634-1700), Speaker of the House of Commons; rentals and account books, 1300-1925 (preserved in an almost unbroken series from the time of Sir William Williams); over 5000 title deeds and documents, [pre-1290]-[c. 1910], mainly relating to properties in the six North Wales counties and Shropshire, including records for Glascoed and Llanforda, Llwydiarth, Llangedwyn and Glanllyn, Plas-y-Ward, Rhiwgoch and Mathafarn, estates acquired either by marriage or purchase in the seventeenth and eighteenth centuries; together with papers relating to administration of the estates, 1573-1946; family papers, 1499-1913, county and central government administration papers, 1608-1880; two discrete groups of Much Wenlock estate records, 1534-1860, and Nantcriba estate records, 1381-1680; and various maps. There is an additional group of papers relating to the Wynnstay estate which came from the office of Longueville Gittins solicitors, Oswestry, dated 1582-1957.