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Genealogical material compiled for Lord Howard de Walden during the early years of his tenancy of Chirk Castle, comprising transcripts of manuscripts containing Welsh genealogies compiled under the supervision of Arthur Owen Vaughan ('Owen Rhoscomyl'); letters, 1906-1921, mainly addressed to Arthur Owen Vaughan, relating to antiquarian and genealogical matters, academic research, etc.; genealogical notes, pedigrees, transcripts of wills, etc.; and an account book, 1870-1872, of the Chirk Castle Estate.

Papers of J. Glyn Davies, mainly letters, many relating to antiquarian, academic and library interests, including 400 from Robert Scourfield Mills ('Owen Rhoscomyl'), 1903-1919, almost 200 from Jennie Thomas relating to Llyfr mawr y plant, 1920-1950, and 150 from T. Gwynn Jones, 1908-1947; papers of his family, including the Tanycastell Collection, 1821-1858; and manuscripts collected by him, including the Henblas manuscript (Welsh poems by various authors, 1664-1685) and the Gwallter Mechain manuscripts.