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Small numbers of title deeds relating to the town and immediate locality of Harlech, 1327-1649, the Faenol estate near Bangor belonging to Sir William Williams and Sir Thomas Williams, 1596-1645, the Irish estates of William Ormsby, Owen Ormsby, and William Gore, 1606-1799, the township of Dolbenmaen in Caernarfonshire purchased by William Owen (3), 1721-1737, and miscellaneous deeds for properties in Anglesey, Caernarfonshire, Cardiganshire, Denbighshire, Merionethshire, Montgomeryshire, Radnorshire and parts of England, 1298-1773. It has been difficult to establish the provenance of some of the deeds. The group also contains a number of unplaced bonds and general releases, the purpose of which has not been established, 1599-1780.

Title deeds and other documents concerning properties purchased or leased by the Brogyntyn estate in the county of Merioneth, 1706-1961. They include a lease and arbitration award for Ty Cerrig, Talsarnau, in the parish of Llanfihangel-y-traethau, 1920-1961; miscellaneous properties in Llandanwg, Llanfihangel-y-traethau, Barmouth, Beddgelert, Harlech and other locations in Merioneth, 1706-1912; and mining and quarrying leases, 1837-1947.

Title deeds and other documents relating to property owned by the Brogyntyn estate in Montgomeryshire, 1647-1902. One series concerns properties of the Penrhos and Cemmes (Cemais) estates, formerly belonging to John Owen, which descended to Mary Jane Ormsby Gore, 1647-1899; another series comprises records of the manors of Broniarth and Deuddwr, 1773-1894. Other deeds concern properties in the township of Broniarth in the parish of Guilsfield, 1740-1885, and at Sarnau in the parish of Meifod, 1828-1902.

Original and copy wills, administration bonds, occasional inventories and other documents associated with probate belonging to the main families of Maurice of Clenennau, Owen of Clenennau and Brogyntyn (Porkington) and Ormsby-Gore of Brogyntyn, 1621-1829, and those who were connected with them by marriage, namely Anwyl of Park, 1600-1700, Godolphin of Abertanat, 1725-[c. 1862], Vaughan of Corsygedol, 1606, 1636, and Wynn of Glyn, Sylfaen and Ystumcegid, 1563-1682.

Original, draft and copy marriage settlements, other family settlements and trusts of the families of Maurice, Owen and Ormsby-Gore of Clenennau and Brogyntyn, 1485-1839 and other families related to them by marriage, namely Wynn of Glyn, Sylfaen and Ystumcegid, 1516-1683, Clayton (incorporating Griffith), 1704-1709, Godolphin, 1733, Hanmer, 1620-1656, and Lyster (incorporating Derwas), 1665-1703, with related deeds and documents of the type normally associated with disentailment and resettlement.

Papers comprising deeds, abstracts, agreements, bonds, rentals, accounts, legal opinons and correspondence relating to several family and non-family trusts administered by members of the Maurice and Owen families, 1584, 1636-1666, [1698], 1725-1773. The family trusts here are specific and separate from those incorporated into the family settlements (section PBF).

Private correspondence of the main Clenennau and Brogyntyn families of Maurice and Owen, 1587-1801, and their descendants, the Ormsbys and Ormsby-Gores, 1777-1950, together with two smaller groups of letters of their relatives, the Owens/Lysters of Penrhos, 1703-1823, and the Owens/Claytons of Brymbo, 1714-1739.

Private letters exchanged between Margaret Godolphin, [c. 1698]-1764, and various members of the Godolphin family of Abertanat, Eton and Thames Ditton, 1698-1763, including her parents, Sydney and Susanna, her sisters, Ellen and Mary, her nephew, Francis, their Hoblyn and Pendarves relatives, and others; together with letters from friends, solicitors and other professionals. The contents reflect in great detail the personal, domestic and social circumstances of an eighteenth century upper class family, against the background of the Jacobite Wars. Recurrent topics include the management of the Abertanat estate, especially the exploitation of timber, the death of Master Henry Godolphin, 1722, physical ailments, financial investments, family settlements and inheritance. The correspondence of Ellen, Margaret and Mary Godolphin from 1728 to 1730 shows a preoccupation with the reluctance of Miss Mary Godolphin to marry William Owen of Porkington!

Private letters, 1582-1933, written to, by or about individuals connected to the families of Maurice, Owen, Ormsby-Gore and Godolphin through marriage, friendship or business and a small number of items where neither the author nor the recipient can be identified. The group also contains several letters (mainly copies) by eminent figures of the Stuart period concerning matters of political and religious significance, which must reflect the interests of the Owen family and their associates.

Personal papers of the Owen and Godolphin families and various members of the Ormsby-Gore family, comprising almanacks and pocket books, 1676-1765, and miscellaneous papers relating to personal interests, physical statistics, training, education and careers, 1672-(Watermark 1860), 1893-[1900].

Personal papers associated with the career and interests of William Ormsby-Gore, 1822-1860.

Personal papers of William Richard Ormsby-Gore, second Baron Harlech, consisting of diaries, 1837-1893, and papers relating to his career and interests, 1836-1894. They cover aspects of his travels in Europe, his army career and participation in the Crimean War, official business as an Irish MP, involvement in local institutions and his membership of the freemasons in North Wales and Ireland.

Personal papers, being journals and diaries of Emily Charlotte Seymour (married name Ormsby-Gore, second Lady Harlech), 1844-1849, 1890, some of which describe travels with her family to Chile and elsewhere in South America, and including a diary of her mother, Georgiana Mary Seymour, 1869-1870.

Personal papers, comprising diaries and army papers of George Ralph Charles Ormsby-Gore, third Baron Harlech, 1873-1883, and diaries of his wife Margaret Ethel, 1914-1937.

Personal papers of William George Arthur Ormsby-Gore, fourth Baron Harlech, comprising notes on church architecture and art, 1903-1927; addresses and essays deriving from both his professional career and his personal interest in (mainly) European art, 1925-1945; and miscellaneous papers relating to his education, personal life and work abroad, 1904-1943.

The group contains pedigrees in handwritten and printed forms, extracts from original and published sources, notes and correspondence on the genealogy of Ormsby-Gore and the families from whom they were descended, such as Gore and Gorges, 1794-[c. 1906], Owen of Brogyntyn, Wynn of Glyn, and other families who were related to them by marriage or who were relevant to the history of the estate, 1698-1951.

Large volumes, notebooks and folders, containing mainly poetry and prose compositions accumulated by various members of the Owen and Ormsby-Gore families, 1624-1868, and in particular by Frances Morres Gore, 1809-1832. The great majority are in English, but they include some works in French, Welsh, Latin and Italian by published and unpublished authors, including members of the Gore family. They broadly cover contemporary national events and politics of the Stuart period, the Hanoverian monarchy and the Napoleonic Wars, together with matters of local interest, and various romantic and moralistic themes.

A play and miscellaneous other papers relating to drama, [1684]-(Watermark 1812), together with papers relating to music and art, [1731]-1888.

Manuscript and printed papers of academic and general interest collected or researched by the family, comprising original documents [14 cent.], 1590, sermons [early 17 cent. x mid 18 cent.], epitaphs, [c. 1686], 1736, prophecies, [c. 1694], [19 cent.], catalogues of books and documents, including Brogyntyn library, 1702-1946, various academic exercises, notes, articles and other literature relating to religion, historical and antiquarian subjects, literature, natural history and topography, philosophical and moralistic themes, money and other subjects of general interest, [1656]-1940.

Complete editions, cuttings and pages of newspapers, 1685-1887; printed newsletters, broadsides, advertisements and general information leaflets, 1666-1861; and manuscript newsletters, 1676-1710.