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Manuscripts and documents collected by and created by John Roberts Hughes, 1727-1961, including, papers relating to the Quakers, including transcribed extracts from records, collected volumes and items of Quaker interest, and notes on the Quakers by J. R. Hughes; various papers collected and written by J. R. Hughes relating to folk-lore and local histories; notes for addresses and lectures; papers and documents created by others, acquired or purchased by J. R. Hughes; deeds relating mainly to Glamorgan and Monmouthshire, and other miscellaneous deeds; together with personal memoranda by J. R. Hughes and family papers.

Deeds collect by J. Augusta Berry, mainly relating to properties in Glamorgan, Pembrokeshire and Carmarthenshire, 1753-1865.

Collection of deeds acquire by D. Gethin Williams, relating to properties in Carmarthenshire and Glamorgan, 1687-1889.

A volume containing the petition of William Hurst, formerly of Gabalfa and Dinas Powys, to the Court of Exchequer concerning his claims in Dinas Powys, Rumney, Llandough, Highlight, Cibwr, St Andrews Major, Merthyr Dyfan, Cogan, Roath, St Brides-super-Ely, Llanedern, Llandaf, Ystradyfodwg, Peterston-super-Ely and Cardiff. Also included are: a sale bill, 1825, from the Roath estate; a promissory note, 1821, from Harford's ironworks, Machen; the probate record, 1845, of Noah Morgan, Cymer; and an election address, 1851, from General Sir George Tyler to the voters of Glamorgan, with manuscript notes on the contents by Ifan Kyrle Fletcher.

Literary, editorial and personal correspondence, draft and unpublished poetry, short stories and other works, and miscellaneous papers, 1955-1995; unpublished short stories and articles, articles and essays, reviews, lectures, plays, broadcasts, ghost-writing, miscellaneous prose, and editorials.

An additional consignment of papers, 2004-7, of Dannie Abse. This group remains uncatalogued.

A further tranch of papers, being letters, loose manuscripts, workbooks and miscellaneous papers, 2008-2013. This group remains uncatalogued.