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A register of the overseers and parish constables of the hundreds of Kemes, Dewsland, Roose, and Dungleddy, 1864-1879.

Sermons preached at Newport, Maenclochog, Brynberian and elsewhere in Pembrokeshire, 1817-1819 [? by Thomas Jones].

The so-called Llwynwormwood MS, containing legal precedents, many of them of Carmarthenshire and Pembrokeshire interest, medical and culinary recipes, etc.

Lists of the sheriffs of Pembrokeshire from 1540 to 1867, the Queen's Lieutenants of Pembrokeshire, 1867, and the Mayors and Sheriffs of Haverfordwest from 1563 to 1857.

A draft by Morgan James Rees of a scheme for hospital inquiries, together with notes of an inquiry, 30 July 1911, relating to hospital service in Pembrokeshire.

A memorandum book containing notes of land and financial transactions, together with surveys of land in Pembrokeshire and Carmarthenshire, recorded by several owners in connection with those counties, etc.

'Short Pedegrees of Divers, Noble-Men, Knights, Esquires, Gentlemen and Women of Pembrook-shire; containing All, or most of the Eight Ancestors from whom they are Descended. Together With the Armes of most of them', being a transcript, made by John Tinkler in 1888, of Chetham Library (Manchester) MS. 6715.

A property rating book covering parishes in north Pembrokeshire and kept by Griffith Davies, Cardigan.

Copies of memorial inscriptions, etc., mainly in Pembrokeshire.

One of four Pembrokeshire parliamentary election polling books. NLW MS 6418 is for the hundred of Roose (Rhos), the election held May-June 1807.

One of four Pembrokeshire parliamentary election polling books. NLW MS 6419E is for the hundred of Roose (Rhos), the election held October 1812.

One of four Pembrokeshire parliamentary election polling books. NLW MS 6420E is for the hundred of Narberth, the election held October 1812.

One of four Pembrokeshire parliamentary election polling books. NLW MS 6421E is for the hundred of Castlemartin, the election held October 1812.

A collection of inscriptions and notes by John Rowland (Giraldus), 19 cent., in pencil, from churches in Pembrokeshire.

Holograph sermon notes by the Reverend Simon Evans, minister of the Congregational churches of Pen-y-groes, parish of Whitchurch-in-Cemais, co. Pembroke, and of Hebron, parish of Llanglydwen, and Nebo, parish of Cilymaenllwyd, both in co. Carmarthen. NLW MS 11689A ('9fed Bregeth Lyfr Cymreig') was compiled at Tyddyn, parish of Whitchurch-in-Cemais, during the period 1852-1854, and NLW MS 11690A ('18 Bregeth Lyfr Cymreig') at Caeraeron, parish of Llanfyrnach, co. Pembroke, during 1873-1876.

Miscellaneous manuscript and printed material, 1775-1870, relating to Captain John Phillips of Liverpool, his heirs, and the Smalls Lighthouse on the Pembrokeshire coast, the building of which he instigated, including two broadsides, articles of agreement, legal opinions, autograph letters and the signed document by which Phillips transferred the management of the lighthouse to Trinity House.

Correspondence, 1990-1991, of Nia Rhosier including letters relating to PARC (Pembrokeshire Against Radar Campaign).

A list of the sheriffs of Pembrokeshire, 1540-1668. Stitch marks at the foot of the roll suggest that the list was once longer. There are also columns for their deputies and the recorders or county clerks, but these are empty.

The file contains a description of Hengwm, which includes the weather, landscape and intrusion of modern forestry; brief notes of plants, birds and mammals recorded at various sites in Cardiganshire and Pembrokeshire; geology and vegetation of the Sugar Loaf and other sandstone or limestone hills, topography of mountainous areas in Breconshire and fungus list for Bont Ddu.