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Autograph letters from a large number of people to Thomas and others, mainly relating to archaeology, Welsh history, literature and ecclesiastical affairs. The correspondents include B. Beedham, William Buckland, W. Boyd Dawkins, Walter Davies ('Gwallter Mechain'), J. P. Earwaker, D. Silvan Evans, R. W. Eyton, E. A. Freeman, Margaret Gatty, Reginald Heber, Felicia Hemans, H. Longueville Jones, John Keble, Sir Theodore Martin, Sydney (Lady) Morgan, Lord Mostyn, Samuel Rogers, W. F. Skene, Sir Arthur Sullivan, John Williams ('Ab Ithel'), Morris Williams ('Nicander') and Robert Williams (Rhydycroesau); an English poem entitled 'The Sixth Centenary of Dante's Beatrice 1890' by T. Tudno Jones; and a number of 'cut-out' autographs.

An armorial drawn and compiled by Thomas, mainly of North Wales families.

A notebook containing 'collectanea' of Thomas relating to the diocese of St Asaph, the Church and Nonconformity in Wales, archaeology, pedigrees, poetry, place names, autograph signatures, etc.

A copy, with a few manuscript corrections in the hand of Thomas, of the 'Index' to 'Llyfr Coch Asaph', printed in Archaeologia Cambrensis, 1868.

A copy of pp. 1-268 of the first (1874) edition of David Richard Thomas, A History of the Diocese of St. Asaph ... (London & St Asaph, 1874), with a few corrections by the author.