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Janet Jones was selected from 1099 other female applicants to embark on a tour of the USA to spread awareness Wales and Welsh culture. Leather bound scrapbook entitled, 'National Hostess of Wales Goodwill Tour 1955'. A typed paper pasted to a page at the beginning of the volume reads "Prepared for: Miss Janet Jones as a memento of her successful Goodwill Tour by the Public Relations Department, British Travel Association, 336 Madison Avenue, New York 17, N.Y.". The scrapbook contains newspaper cuttings of articles and photographs, telegrams, letters, typed daily schedules, and interviews.

Nine letters, 1963-83, addressed to William Robert (Bill) Carrick, including seven from the novelist Richard Vaughan, dated 1963-9 and 1981.

A dissertation by Elsie M. Price, entitled 'The Welsh Woollen Industry', submitted in 1969 as part of a course at C F Mott Teacher's Training College (Liverpool) during the 1960s. The work is typed and bound, and includes photographs together with samples of wool and weave for blankets and clothing.

Some ninety-nine letters and postcards, 1975-2013, from the poet and local historian Ruth Bidgood, Abergwesyn and later Beulah, Powys, addressed to the Rev. James Coutts, and frequently also to his wife Stevie, discussing her poetry, publications and public readings, her daily life and her family, containing frequent references to friends including Anne Cluysenaar, Angela Morton and A. M. (Donald) Allchin (ff. 1-188, 191-214).
Also included are typescript copies of eighteen of Bidgood's poems and sequences of poems, published and unpublished, [c. 1979]-2014, notably 'Hymn to Sant Ffraed' (ff. 215-225), most given by her to Coutts and a few re-typed by him, and cuttings and photocopies of a further fifteen poems from periodicals, 1983-2002 (ff. 25, 37-38, 52-53, 70, 116, 120, 215-265); typescript drafts, cuttings and photocopies of articles, interviews and reviews, [1978]-2006 (ff. 266-299), including two typescript articles by Donald Allchin (ff. 279-293); and a letter from Bidgood's friend Mary [MacGregor], of Myddfai, to James Coutts, 2 June 2009 (ff. 189-190). Many of the letters were written on the backs of sixty-three of Bidgood's own photographs, so as to resemble postcards; besides these a further twenty-nine of her photographs are also included amongst the letters.

Miscellaneous papers, 1981-96, belonging to Professor David Blamires, author of David Jones: Artist and Writer (1971), who established the David Jones Society in 1975. The collection includes exhibition notes, research papers, conference programmes, postcards, and correspondence. A separate file within the box contains a set of David Jones Society Newsletters, nos.1-38 (1976-84).

Sgript y ffilm Un Nos Ola Leuad (1991), addasiad Gwenlyn Parry ac Endaf Emlyn o nofel Caradog Prichard. Mae'r sgript yn cynnwys nodiadau a darluniau o waith y cyfarwyddwr, Endaf Emlyn, sy'n ymwneud â'r cynhyrchiad.

A visitors' book, 1990-1995, of the exhibition 'New Traditions: contemporary Welsh craft / Traddodiadau Newydd: crefftau Cymreig cyfoes' by Charles and Patricia Aithie, which accompanied the Welsh-Yemeni Festival held in Sana, Yemen. Most entries are in Arabic; a typescript containing an English translation is included in the front of the volume. The visitors' book was transferred to NLW among the Charles and Patricia Aithie photographic collection.

A typescript précis of the text of NLW MS 24191B, a journal of an 1816 tour of New York State and the Niagara Peninsula, Upper Canada (ff. 1-7 verso), together with endnotes (ff. 7 verso-8). The typescript contains annotations, corrections and underlinings throughout. The folio numbers and quotes given are not always entirely accurate.

Two volumes, [2015], comprising ‘A millennium of Clement ancestry’ by Dillwyn Clement bearing the Clement coat of arms with the motto ‘I's gorau ein gorau’. The first file contains the ancestry of the Clement family especially in Wales and the second file is an appendix to the study.

Six scripts, 2016, of the television programme 'Adrian's Election Bites', being interviews between Adrian Masters, political editor at ITV Wales, and leaders of the political parties in Wales, broadcast on ITV Cymru Wales prior to the 2016 Welsh Assembly elections. The leaders interviewed were Alice Hooker-Stroud (Wales Green Party), Nathan Gill (UKIP), Kirsty Williams (Liberal Democrats), Leanne Wood (Plaid Cymru), Andrew R. T. Davies (Conservatives) and Carwyn Jones (Labour).

A file of correspondence, 30 March-7 May 2017, between Valerie Wynne-Williams and her solicitors Kuits on the one hand and Thomas Dilworth and his publishers Penguin Random House UK on the other, relating to the contents of Dilworth's biography David Jones: Engraver, Soldier, Painter, Poet (London, 2017). The correspondence resulted in a number of amendments being made to subsequent editions of the book.

A dissertation, by the donor, submitted in partial fulfillment of the requirements for the BA History degree at the University of Southampton (13/5/2021), entitled 'You can't make an omelette without breaking eggs: an investigation into the role of Western correspondents and governments in the cover-up of the Ukrainian Famine, 1932-33'. The contribution of the journalist Gareth Jones in uncovering the Holodomor is covered in this study.

Script of a lecture given by Ted Harrison, at the National Library of Wales in December 2022 entitled 'The boy from Barry who became a Fleet Street legend', on the cartoonist Leslie Gilbert Illingworth. Also included are photocopies of the slides used in the lecture.

A volume, 1681-2, in the hand of Huw Morys ('Eos Ceiriog', 1622-1709), poet, Llansilin, co. Denbigh, containing mainly holograph Welsh poetry in strict and free metres, including a poem dated 1681 (ff. 10-11), together with a cywydd by Siôn Tudur (f. 16 verso), prophetic verses, some attributed to Taliesin (ff. 12 verso, 25 verso), and anonymous englynion (ff. 36 verso-37, 42); the original parchment cover, preserved at the beginning, contains copies by H.M. of 'Diarhebion o waith Taliessin', 'Cynghorion Taliessin' (f. i verso) and 'Tri Thlws ar ddeg o Ynys Brydaine' (f. ii). The manuscript was probably written for the poet's brother John Maurice (d. 1699), Bodlith, Llansilin, whose name appears on f. 1; other signatures in the volume suggest it to have remained in the possession of the family until the [mid-18 cent.].

Notes by T. Ivor Davies and T. Charles Jones, from contemporary sources including the Coroner's Court records, a public meeting at Beaumaris and service at Bangor Cathedral, relating to the sinking of the 'Rothsay Castle' steam packet on 17th August 1831, on its journey from Liverpool to Beaumaris, during which over a hundred and forty lives were lost.