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Mae'r fonds yn cynnwys dwy gyfrol, 1937-1961, yn cofnodi'r niferoedd a oedd yn bresennol yn nosbarthiadau'r Ysgol Sul, Capel Hermon, Llanfachreth, manylion am eu gweithgareddau yno a chyfanswm y casgliadau; nifer o 'lyfrau'r athro' a gedwid gan athrawon yr Ysgol Sul, 1959-1968, yn rhestri enwau'r plant o fewn y dosbarthiadau unigol a manylion am eu presenoldeb; ynghyd â llyfr cyfrifon, 1912-1927, yn cofnodi cyfraniadau'r aelodau at wahanol gasgliadau a chyfres o holiaduron, 1916-1929, yn rhoi manylion am y capel a'r aelodau.

The manuscripts of J. Gwyndud Jones, comprising mostly religious literature, sermons and hymns.

A collection of hymn-tunes and other pieces composed in the second half of the nineteenth century by William Evans Alaw Afan.

Deeds and documents, 1508-1706, relating to the parishes of Llanbedr and Llandecwyn, Merionethshire.

Records of Siop y Jones, Llandysul, 1823-1862, consisting of day books, 1823-1841; ledger, 1845-1862; and index of customers, 1845-1862.

Records of the Cardiganshire Association for the Blind, 1920-1975, including record books of registered blind, 1920-1938; minutes of the executive committee, 1933-1974; minutes of the Annual General Meetings, 1940-1973; and annual reports, 1921-1975.

Seven deeds, 1675-1721, relating to properties in Ystrad, Cilcennin, Llanbadarn Trefeglwys, Llanddewi Aberarth, Dihewyd, Ciliau Aeron, Llannarth, Llansanffraid, Henfynyw, Llanbadarn Fawr and Aberystwyth, co. Cardigan, and Harplesmore and Folkeston, Pembrokeshire.

Deeds, 1728-1825, relating to properties in the parish of Llywel, Brecknockshire.

Charter of incorporation of the borough of New Radnor, Radnorshire, 1562, and charter of re-incorporation, 1739.

Deeds and documents, 1740-1856, relating to properties in the parishes of Henllanfallteg, Llanboidy, Llanwinio, and Laugharne, Carmarthenshire, and St. Davids, Pembrokeshire; miscellaneous papers, 1876 - c. 1960, relating to St. Davids; and a pedigree, compiled by Major Francis Jones, of the Devonald and Morse families of Llanfyrnach and the associated family of Skeel of Trewilym, Pembrokeshire, 1886-1905.

Deeds, plans, wills, marriage settlements and other papers, 1709-1940, relating to the Ffrwdgrech estate, Llanfaes, Brecknockshire, and to lands in neighbouring parishes.

Research papers of Professor T. V. Davies, 1981-[c. 1991], into the farms and farmers of Senghenydd Supra in the parishes of Gelligaer and Merthyr Tydfil including photocopies of documents in the Public Record Office, National Library of Wales, Glamorgan County Record Office, and Gwent County Record Office; miscellaneous research notes and transcripts; draft chapters; papers relating to the Llantrisant and District Local History Society, 1981-1990; letters to T. V. Davies, [c.1984]-1990; and typescripts of his lectures to history societies, 1988-1989.

The fonds comprises research material relating to drovers and drove roads in Wales, and in other parts of Britain and Ireland, reflecting R. G. Avent's interest in the subject. The papers include manuscript notes, notebooks and offprints from journals and magazines, together with some related publications. Also included is a card index containing references to relevant printed sources, some of which are cross-referenced with the notes.

Ratebooks of the parish of St Athan for 1880-1905.

The collection comprises the UCW Agricultural Debating Society minute books, 1920-1963, and a file of correspondence, 1960-1973; agricultural club minute books, 1929-1939; and the rustics' club minute book, 1933-1940.

Deeds and documents, 1769-1891, relating to Penpistyll and other properties in the parish of Llangeler, Carmarthenshire.

Deeds, wills and documents, 1718-1767, relating to people and properties in the parish of Llanrhidian, Glamorgan.

Papers, 1976-1996, of political interest, including copies of speeches of various politicians, 1976-1996; miscellaneous papers, 1981-1994, including interview notes, drafts of newspaper articles, television news scripts, notes from Rhodri Morgan MP and Sir Bernard Braine MP; press releases, 1982-1995; miscellaneous papers, [c. 1980]-1992, concerning Welsh matters, including the Welsh language, Welsh language broadcasting, parliamentary constituency boundaries in Gwent, the Welsh Office, road tolls, the National Museum of Wales, the distribution of a political newspaper, Y Glorian, in Rhondda schools, devolution, Labour Party Young Socialists; printed parliamentary debates, 1977-1994; House of Commons reports, 1986-1992; and miscellaneous printed material, 1993-1995. Additional Papers of political interest, from the late 1980s to 2007, accumulated by the donor as Lobby Correspondent for the Community News Service, at the House of Commons. This additional group remains uncatalogued.