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A volume, compiled [19 cent., first half], containing a number of homilies on moral and religious topics by an unidentified Quaker (inside front cover-f. 19); together with extracts from the manuscripts of John Kelsall, Dolobran, Montgomeryshire, comprising brief accounts, 1701-1712, of meetings of the Society of Friends, including those held at Dolobran and yearly meetings of the Society in Wales (ff. 19 verso-27).

Letters, 1847-1873 and n.d., from Henry Griffiths of Brecon, Liverpool and Bowden, mainly relating to education in Wales and to the proposed Normal School at Brecon. One letter, 1854, contains adjudications in both Welsh and English by Griffiths on essays submitted for competition at an eisteddfod (see also a letter, 1854, relating to the adjudications), while another, 1862, to William Roberts, tutor at Brecon Independent College, relates to Griffiths's application for the Theological Chair at Carmarthen Presbyterian College.
Also included is a letter, 1889, from Samuel Job of Illinois; a letter, 1906, from Hugh Williams ('Hywel Cernyw') at Pontypridd; and a letter, 1928, from Caleb Lewis at Blaina, Monmouthshire. The last two letters relate to the Welsh periodicals of the time.

A copy of the publication given to James Ifano Jones by its author William Williams, Keeper of Printed Books at the National Library of Wales, and annotated by the recipient who was a Welsh Librarian at Cardiff City Library.

Papers of Rev. Daniel Rowland Thomas, pacifist and scholar, including order of services for his induction as minister at Aberdare, 1939 and Merthyr Tydfil, 1945; radio scripts of services conducted by him which were transmitted by the BBC; a programme for his lecture tour in the United States as a visiting lecturer in Biblical Studies in 1967; his poem written for CND Cymru, 1999; press cuttings of articles by him and a leaflet for a Peace festival held in Ammanford in 1990, when he was one of the guest speakers. = Papurau'r Parch. Dr Daniel Rowland Thomas, heddychwr ac ysgolhaig, gan gynnwys taflenni trefn gwasanaeth ei odeinio'n weinidog yn Aberdâr, 1939 ac yn Merthyr Tudful yn 1945; sgriptau o wasanaethau yn ei ofal a ddarlledwyd gan y BBC; rhaglen ei daith ddarlithio i'r Unol Daleithiau fel darlithydd gwadd ar astudiaethau Beiblaidd yn 1967; cerdd a luniodd i CND Cymru, 1999; torion o'r wasg yn cynnwys erthyglau ganddo a thaflen Gŵyl heddwch, Rhydaman, 1990, pan oedd yn un o'r siaradwyr gwadd.

An essay, written about 1913, by Dr. Hugh Jones, Liverpool, entitled 'A Scheme for the Diffusion of Knowledge of First Aid, Home Nursing, and Domestic Hygiene in Wales'.

A composite volume written after 1818 and containing sermons by, and in the hand of, the Reverend Christmas Evans, Baptist minister, of Llangefni, etc.

Antiphonal, known as the 'Pen-pont MS'.

A volume containing offprints and articles relating to Welsh Gypsy folk-tales, mainly from the Journal of the Gypsy Lore Society, collected and edited by John Sampson.

Research papers of the botanist Richard Henry Roberts, [1953]-[2002], a county recorder for the Botanical Society of the British Isles. The papers including field notes on plants in Anglesey, together with a copy of The flowering plant and ferns of Anglesey (Cardiff, 1982) by him and heavily annotated, and offprints of articles relating to his research.

Legal files relating to the court cases of members of the Welsh Language Society, [1968]-[1971]. = Ffeiliau cyfreithiol yn ymwneud ag achosion llys aelodau Cymdeithas yr Iaith Gymraeg, [1968]-[1971].

Diaries, 1967-2010, of Iona Trefor Jones (1925-2011), relating mainly to her work with flowers, together with her reminiscences: ‘Cofio’ (in Welsh), and a scrapbook chronicling her contribution to flower festivals held in Chester Cathedral, Bangor Cathedral, Holyhead Parish Church and others.

Press-cuttings relating to Welsh Hospital Board, 1951-1974.

Papers of Frank H. Cleaver, 1924-1985, mainly accounts, including personal, family and household expenses, 1924-1985; expenses for his work in Argentina, 1929-1931; and summaries of accounts, 1949-1968.

Papers relating to the work of E. D. Jones as Chairman of the Multiple Sclerosis Research Fund, comprising correspondence, 1961-1979; articles of association of the Multiple Sclerosis Research Fund Ltd, 1964; annual reports and accounts, 1965-6, 1971-2; notes on multiple sclerosis, [1961x1979]; and publicity material, newspaper cuttings and other printed material, [1961x1979].

A copy of Edward Jones, Musical and Poetical Relicks of the Welsh Bards ... (London, 1794), with a few annotations by John Dovaston. Among items tipped in are transcripts by Edward Jones of Welsh, English and Irish airs (ff. 1, 73, 106) and a letter from him to Dovaston, 16 January 1817, concerning Welsh folk-tunes and other national airs (ff. 74-75). The letter is in answer to Dovaston's letter of 25 December 1816, which is part of Cardiff MS 4.130.

Miscellaneous music, including part-songs and hymn-tunes, composed by 'Alaw Afan'.

Tune book containing hymn-tunes and anthems.

A volume containing recipes, household and medicinal but mainly relating to the craft of bookbinding (ff. 5-10); a list of books lent, 1827-1837, from an unspecified library, with observations on their condition (inverted text ff. 44 verso-7 verso); notes on the rudiments of music (ff. 2-4, originally pasted together onto f. 1); with late nineteenth and early twentieth-century additions by William Morris, Cydweli.

Papers, 1976-1996, of political interest, including copies of speeches of various politicians, 1976-1996; miscellaneous papers, 1981-1994, including interview notes, drafts of newspaper articles, television news scripts, notes from Rhodri Morgan MP and Sir Bernard Braine MP; press releases, 1982-1995; miscellaneous papers, [c. 1980]-1992, concerning Welsh matters, including the Welsh language, Welsh language broadcasting, parliamentary constituency boundaries in Gwent, the Welsh Office, road tolls, the National Museum of Wales, the distribution of a political newspaper, Y Glorian, in Rhondda schools, devolution, Labour Party Young Socialists; printed parliamentary debates, 1977-1994; House of Commons reports, 1986-1992; and miscellaneous printed material, 1993-1995. Additional Papers of political interest, from the late 1980s to 2007, accumulated by the donor as Lobby Correspondent for the Community News Service, at the House of Commons. This additional group remains uncatalogued.

Records accumulated by Dr John Herbert, 1968-1984, comprising Welsh Secondary Schools Association records, minutes and papers, 1968-1984; and Headmasters' Association and Secondary Heads Association minutes, correspondence, discussion papers and related material, 1969-1984.