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Records of the Vale of Neath Brewery, 1844-1913, including ledgers, 1894-1897; pay books, 1882-1912; purchase abstract books, 1896-1908; beer sales books, 1896-1913; spirit sales books, 1897-1912; and printed books, 1863-1913.

A manuscript containing the names of all rectories 'in the kingdom of England and Calais and the Marches thereof' of the annual value of over £10, arranged in dioceses, deaneries and counties, followed by the names of all vicarages in England, Wales and the Marches of the annual value of over £10, similarly arranged, all having been transcribed from the Liber Regis in the First Fruits and Tenths Office.

A vesting assent dated 17 December 1953, bound in book form, relating to the Llysnewydd Estate in the counties of Carmarthen and Cardigan, 1953-1981, including an estate map.

A collection of photographs (290 colour, 35 b&w), mainly by Ian Campbell covering a range of protest movements and associated organisational banners including a march in Cheltenham in aid of GCHQ workers, anti nuclear bunker protests in Carmarthen, anti-nuclear and anti UCW cutback rallies in Aberystwyth, events at Greenham Common, a 40th birthday party for the NHS in Aberystwyth and some family photos.

Two volumes containing manuscript music, 1809-1828, one inscribed within by 'Mary Madocks, alias Williams, Vron-Iw, October 1809', and two volumes of printed music, one of which belonged to Mrs Henry Laird, inscribed within by 'Jessie Laird, 1879', and bearing the initials 'J.L.', and the other bearing the bookplate of Mrs Mevekson-Sandbach. One manuscript copy and a printed copy has 'Mrs Williams, 1822' written on their covers.

Deeds relating to the parishes of Llanbadarn Fawr, 1548-1597, and Llangynfelyn, 1841-1848, Cardiganshire.

Deeds purchased from W. A. Evans, relating to Denbighshire, Flintshire and Anglesey, 1310-1795.

Deeds relating to properties at Deep Dean, Walford, Herefordshire, 1799-1816, and in Merthyr Tydfil, Glamorgan, 1788-1859.

Deeds and documents relating to Cardiganshire, 1590-1751; and Montgomeryshire, 1517-1770; deeds and documents relating to the Hughes family of Gogarth, 1669-1910; and miscellaneous items, 1692-1825.

A notebook containing notes on the history and practice of the Courts of Great Sessions in Wales accumulated by W. Llewelyn Williams, K.C., M.P. (1867-1922) (see Y Cymmrodor, XVI, pp. 1-87). Many of the extracts are taken from the Llwynwormwood MS, i.e. NLW MS 4492D.

The reminiscences of William Robert Hall (1849-1937), written in forty exercise books and published serially in The Cambrian News, 1920-1921.

Correspondence and other papers used in preparation towards the Wales Assembly of Women's report for the United Nations Fourth World Conference on the status of women, Beijing, 1995.

Particulars, in the autograph of Walter Davies (Gwallter Mechain) (1761-1849), of wages paid to agricultural workers in Wales c. 1800.

Deeds, wills and other documents relating to Monmouthshire, 1568-1825.

A typescript copy of an unpublished work by Richard Anthony entitled 'Water over Wales's Valleys', 1985.

Deeds and documents relating to properties mainly in Montgomeryshire, 1615-1910.

Account book, mainly in Welsh, 1867-1907, of Thomas Jones (d. 1897), Brynmeheryn, Ystradmeurig, co. Cardigan, containing customers' accounts for weaving, sometimes with details of patterns; also included are a few veterinary recipes. Later entries are in the hand of Evan W. Jones, possibly the son of Thomas Jones.

Account book, 1887-1916, of Thomas Jones, Pant-teg, Bronnant, co. Cardigan, weaver, with a few later memoranda, 1921-1924, mostly concerning machinery, by his son E. D. Jones. Note on 'Patrwn Carthen Felinfach' inside back cover.

A manuscript containing an account of money gifts received by Richard and Elizabeth Davies (probably of Carmarthen) on their wedding day, November 19th, 1811, and of gifts 'repaid' by them.

A volume containing a transcript of Griffith Jones, Welch Piety for 1751-1752 (London, 1753) and of part of the Welch Piety for 1753-1754 (London, 1755) and 1756-1757 (London, 1757) (ff. 1-138); extracts relating to the history of religion in Wales (ff. 139-232v) mainly from published works but a few extracts from manuscripts of H. T. Edwards, dean of Bangor (see ff. 149v, 168v-9v, 171v-2, 188. 201v); and extracts from Panton MSS 41 and 57 (ff. 234-343). Most of the volume appears to be in the hand of the Reverend David Jones, biographer of Dean Edwards and author of Life and Times of Griffith Jones sometime Rector of Llanddowror (London, 1902) and the dates 1889 (ff. 198, 201, 202v) and 1891 (ff. 332, 343, 'Copied by me D. J. ...') occur.