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Records of the Gregynog Press, 1902-1963, mainly 1922-1940, including accounts, 1922-1963; correspondence, 1924-1954; documents relating to published works, 1923-1940; documents relating to books printed for private circulation, 1929-1938, documents relating to unpublished works, 1932-1936; ephemera, 1927-1962; prospectuses and catalogues of printing firms, exhibitions, booksellers, 1926-1940; miscellaneous papers, 1917-1954, and photographs, 1902-1924; and draft designs and illustrations, [c. 1930s].

Deeds, relating to properties in the following counties: Anglesey, 1737-1871; Cardiganshire, 1736-1780; Carmarthenshire, 1684-1838; Caernarfonshire, 1831-1878; Denbighshire, 1591-1837; Flintshire, 1465-1855; Glamorgan, 1597-1883; Merionethshire, 1793; Pembrokeshire, 1683-1857; and Radnorshire 1623-1816.

Deeds relating mainly to Carmarthenshire, 1531-1857, and to other Welsh counties including Brecknockshire, 1655-1800, Cardiganshire, 1628-1819, Glamorgan, 1673-1792, Monmouthshire, 1636-1795, Montgomeryshire, 1675-1702, Pembrokeshire, 1724-1811, and Radnorshire, 1689-1773. There is no apparent connection between the deeds.

Deeds relating to the Maesnewydd estate in the parish of Llanfihangel Genau'r-glyn,Cardiganshire, together with account books, 1819-1969, and diaries, 19th cent., mainly of J. T. Morgan.

Deeds, 1557-1808, relating to premises mainly in Carmarthenshire, with some in Montgomeryshire, Cardiganshire and Flintshire, and a small number in other Welsh counties.

The collection consists of election addresses, leaflets, circulars and other printed matter, 1837-1991, generally acquired before the establishment of the Welsh Political Archive; election addresses, leaflets etc., 1905-2019, collected by the WPA; and printed materials, 1887-2019, concerning the political parties in Wales, various pressure groups and organisations, subject files, and other miscellaneous papers.

The records deposited in 1934 included two major groups, the 'Trevecka Group' and the 'Bala College Group'. The former, which represents the largely autonomous 18th-century development of Methodism in Wales, beginning in the 1730s, is centred on the archives of the founding father of Welsh Methodism, Howell Harris, and of the religious community which he established, the 'Trevecka Family'. Besides the 290 volumes of Howell Harris's diaries (for 1735-73), it comprises some 3000 letters, accounts of Societies (individual groups of adherents) and records of Associations. The 'Bala College Group' represents the development of Methodism during the 19th century, its spread in North Wales, the separation from the Established Church in 1811 and the formation of the Confession of Faith in 1823. The accessions of the years 1934 to 1974 include the records of the Sasiwn [the Association], district meetings, colleges, some individual chapels and churches, personal archives (both those of ministers and laymen), and those of the Foreign Mission. In content, the accessions of the years 1974-83 are distinguished from those of the earlier period by the high proportion of records of individual churches, many of them deposited because of the closure of the church. A third series, following a classification similar to that of the second, lists accessions from July 1983 onwards. The records of the North Cardiganshire Presbytery, detailed in a schedule [c.1940], have been withdrawn. Particular mention should be made of the archives of the Foreign Mission, which cover the missionary work of the Church in North East India from its beginning in the 1840s.

Records from the office of D. T. M Jones & Co., solicitors, 1775-[?1940], including office correspondence, 1775-1840, of Edward Jones senior, 1775-1820, Edward Jones junior, [c. 1790]-1840, Thomas Lewis, 1793-1800, John Jones, 1805-1852 (predominantly 1845-1848), Thomas Jones, 1860-1897, and D. T. M. Jones, 1898-1933; manuscript books, 1744-1925, including letter books, 1859-1917; depositions of witnesses, 1736-1768; deeds and records of lands in Cardiganshire, Carmarthenshire, Glamorgan, Pembrokeshire and Radnorshire, [16th century]-1949, including the estates of Dinas, Brecknockshire, 1756-1949, the Gwynne family of Glanbran and Buckland, 1679-1882, Cynghordy, Carmarthenshire, 1843-1945, Abermarlais, Carmarthenshire, 1712-1923, the Lloyd family of Briwnant, Carmarthenshire, 1544-1927, Glansevin, Carmarthenshire, 1678-1914, the Herbert Lloyd estate, Carmarthen, 1805-1884, Jones Family of Ystrad estate, Carmarthen and district, 1776-1865, and Llandeilo and district, 1785-1882, Glanyrannell estate, Carmarthenshire, 1692-1919, and Honeyborough, Pembrokeshire, 1783-1923; accounts, 1782-[?1940]; manorial records, [c. 1830]-1887; papers of Roger Jones, attorney, 1565-1867, including correspondence, [c. 1750]-1772, deeds and documents relating to the practice and estate, 1565-1867, and correspondence of Rev. John Jones, 1738-1790.

Records and papers, 1647-1872, relating to the manors of Llanelidan, Llanfair Dyffryn Clwyd, Rhos, Llanhychan, Rhiwbebyll, Llech, Llan and Meifod, Denbighshire, 1647-1872; miscellaneous documents including papers relating to Llanelidan enclosures, 1797-1832; miscellaneous papers relating to the Bishop of Bangor's estate in Llanelidan, 1828-1836; and posters issued by the Ruthin Association for the Prosecution of Felons, 1846-1851.

Deeds and other documents, 1630-1886, relating mainly to the Powell family of Maesgwyn and to the parishes of Diserth, Llansanffraid-yn-Elfael, Llandegla and Glasgwm, Radnorshire, 1630-1886; and to properties of the Jones family of Bryncynfelyn in the parish of Llanfechain, 1651-1782.

Papers of the family of Jones and Pughe-Jones of Ynysgain, Cricieth, Caernarfonshire, 1501-[c. 1955], including deeds, mostly relating to the Cricieth area and to Merionethshire, 1501-1890; and an account book, 1614-1918.

Records mainly of the manor of Monmouth, 1549-1919, including a survey of the manor, 1612; entry books of surrenders of customary properties, 1673-1919; transcripts of papers relating to heriots and alienations, 1606-1628; conveyances, 1610-1774, of the manors of Monmouth, Ebboth and Longstocke, and the lordships of Kidwelly, Carnwyllion and Iscennen; and transcripts of documents relating to the borough and corporation of Monmouth, 1549-1716.

Papers of Leslie Wynne Evans, [1846x1985], including correspondence, 1931-1974, many of which relating to his research work; research papers and source materials, [1846x1985], including papers of Sir John Herbert Lewis, 1916-1923 and Sir Alfred T. Davies [1904x1949], correspondence of O. M. Edwards, 1907-1911, and xerox copies of Board of Education records, 1880-[c. 1920]; drafts and fragments of articles, chapters etc, [1930x1985]; miscellaneous papers including papers relating to University College, Cardiff, 1962-1977, notes, articles, maps and photographs, [1937]-[1977].

Deeds and documents, 1672-1872, relating mainly to properties in the parish of Llanfihangel Cwm Du, Brecknockshire. They also include some probate documents, extracts from parish registers and financial papers.

Deeds, mainly relating to Cardiganshire and Carmarthenshire, 1668-1757.

Deeds acquired by E. Williams of Hove, relating to premises in Brecknockshire, 1564-1823; Cardiganshire, 1663-1778; Carmarthenshire, 1437-1790; Caernarfonshire, 1437-1822; Denbighshire, 1507-1743; Flintshire, 1469-1761; Glamorgan, 1612-1775; Merionethshire, 1616-1762; Monmouthshire, 1491-1795; Montgomeryshire, 1636-1773; Pembrokeshire, 1645-1797; and Radnorshire and Herefordshire, 1543-1786.

Deeds and other documents mainly relating to families and estates in the St Davids area, Pembrokeshire, 1694-1896, including manuscript maps relating to the parishes of Llanrheithan and Mathri, Pembrokeshire, and Llanwinio, Carmarthenshire, 1812-1821. The families involved include Howells of Llysyfran, Ford of Stonehall, Owen of Orielton, James of Llandeloy and St Edrins, Parry of Porthiddy (Llanrian), Laugharne of Orlandon, and Mathias of Lochmeyler and Castle Cenlas. The Mathias family include Rev. John Matthias (d. 1805) of Lochmeyler, vicar of Llandeloy, who bought Castle Cenlas, c.1792.

Deeds and documents relating to the estates of the Jones family of Pen y Bryn, Ruabon, Denbighshire,1534-1808, and of the Maddocks family of Prees Henlle, Whittington, Shropshire, 1441-1786.

Documents collected by Col. Sir John Conway Lloyd, including over a thousand deeds, 1323-1870, relating to properties in the counties of Brecon, Glamorgan, Hereford, Monmouth, Radnor, Cardigan, Carmarthen, Gloucester, and London; together with various documents, including letters and papers relating to the Lloyd family and other estates. In addition, the archive consists of deeds and documents, 1588-1864, mainly of industrial interest accumulated by John Lloyd (1833-1915), pertaining to the New Weare ironworks, Goodrich, Hereford; the Hirwaun ironworks; the Beaufort Iron Company, the Clydach ironworks; the Dowlais Iron Company; and the Bute Works. A substantial group of Dinas Estate records has been transferred to the Maybery Collection.

Deeds, wills and other documents relating to Monmouthshire, 1568-1825.