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Papers of François Jaffrennou (Taldir), 1771-1955, including a five volume autobiographical work entitled 'Le Matricule 315', [1920s]-1946; press cuttings, 1899-1955; manuscript poetry and prose works, 1944-1953; papers and notes relating to the German Occupation and Taldir's subsequent incarceration, 1938-1955; family documents and papers, 1771-1925; copies of works by Loeiz ar Floc'h (Stourmer), 1910-1915, and Georges Floc'h (Yann Tanig), 1945-1951; and papers relating to the Pan-Celtic Congress of 1904 and other Pan-Celtic activities, 1904-1949.

Papers, 1772-1990, mainly comprising correspondence and papers of George Crawshay of Haughton Castle, Northumberland, which include letters, 1840-1874, from George Crawshay to his mother Louise Crawshay, his wife Eliza, and other family members; letters, 1840-1890, to George Crawshay from political figures, which reflect Crawshay's active political rôle; a journal, 1836-1837, of George Crawshay whilst in Freiburg under the care of a German tutor; miscellaneous papers, [1830s]-1890, of George and Eliza Crawshay; and letters and papers, 1772-1950, of Florence and James Kennedy Esdaile, daughter and son-in-law of George Crawshay.

Miscellaneous papers relating mainly to Thomas Charles, Bala, and to his grandson David Charles, Trefeca.

Diaries and journals of tours of William Dillwyn, 1774-1775, 1777, 1781-1790, recording his departure from Pennsylvania for England, tours of parts of England and south Wales, his religious, political and business activities, the anti-slavery committee, and family business.

Papers, 1774-1947, of Lady Eleanor Butler and Sarah Ponsonby, popularly known as the 'Ladies of Llangollen', comprising diaries and correspondence, together with related papers.

Papers of and relating to the novelist John Cowper Powys (1872-1963) and other members of his family, including his correspondence with family, friends and associates, as well as published and unpublished literary works, diaries, lectures, essays, and material relating to his estate and literary executorship. Also included are correspondence and literary and personal papers of Powys's companion Phyllis Playter (1893-1982), as well as personal and estate papers of members of the Powys family including his father, Charles Francis Powys, his paternal grandfather, Littleton Charles Powys, his uncle, Littleton Alfred Powys, his aunts, the Johnson sisters, and his nephew, Francis Llewellyn Powys.

This collection is from the library of Robert Davies Roberts and relates principally to family history and to the antiquities of Denbighshire.

Papers of Henry Robertson, comprising personal and estate papers, 1829-1907; records of a very large number of Welsh railway undertakings, 1786-1911, comprising books of reference, surveryors' notebooks, acts of parlimaent, bills and estimates, conveyances and other title deeds, specifications and tenders, prospectuses and miscellaneous papers; office papers, correspondence and miscellaneous professional papers, 1824-1903; papers relating to several clubs and societies, 1888-1907; and printed books and papers, 1786-[c.late 19th cent.].

The papers consist of the personal papers and letters of, and acquired by, Evan Richards of Nanthenfoel, 1823-1872; family correspondence, 1826-1891; unproved Cardiganshire wills, 1805-1847; and miscellaneous documents of Cardiganshire interest, 1787-1853.

Deeds and documents of the Williams family of Bodelwyddan, Flintshire, relating to the Bodelwyddan, Bodidris and Pengwern estates in Flintshire and Denbighshire, 1788-1898.

Papers of David Davies, the first Baron Davies of Llandinam (1880-1944), along with papers of other members of the family, David Davies (1818-1890), Edward Davies (1852–1898), Revd. Gwilym Davies (1879-1955), Gwendoline Elizabeth Davies (1882-1951) and Mary Sidney Davies (1884-1963). They reflect Lord Davies varied business and political interests and include the records of the New Commonwealth Society, papers related to the League of Nations Union Welsh National Council, the first and second world wars, the Temple of Peace, the King Edward VII Welsh National Memorial Institute, the National Library of Wales, the Royal Welsh Agricultural Show, University of Wales Aberystwyth, Davies’s coal and railway interests, international affairs, drafts and copies of Davies’s publications mainly on international relations, papers of the David Davies Memorial Institute and papers related to Gregynog Press.

Poetical compositions by Daniel Jones, together with miscellaneous papers including transcripts, correspondence, newspaper cuttings and a note relating to the births of his children. The transcribed material is largely by David Jones of Llan-non, son of Daniel Jones.

Papers, 1790-1914, of, or relating to, Nassau William Senior and his family. They include family correspondence, including transcripts, 1800-1912; correspondence, 1818-1863, of Nassau William Senior with various individuals, including Lord Lansdowne, [?1831]-[c. 1860], and John Murray Forbes, 1855-1863; letters to Senior from Alexis de Tocqueville, Edward Everett and George Sumner, 1842-1863, mainly relating to contemporary political events in France and the United States; papers, 1834-1837, concerning Poor Law legislation, social and religious issues in Ireland and factory regulation in the cotton industry; letters, 1855-1876, to Jane Elizabeth Senior; a journal of Senior's tour in Scotland, Ireland and Wales, [?1819]; and miscellaneous papers, including letters from statesmen and ecclesiastical dignitaries, 1790-1887, collected by Walter Nassau Senior.

Manuscripts, [1790x1937], by or belonging to, the Reverend David Morgan Lewis. The material is largely of Congregational or Welsh literary/historical interest and includes sermons and sermon notes; volumes of hymn-tunes and material relating to Welsh hymn-writers (including Ann Griffiths) and their work; lecture notes and essays; tour journals, [1889]-1906, of David Morgan Lewis; and an album mainly of Congregational interest compiled by John Lloyd James ('Clwydwenfro').

The collection known as the Archdeacon A. O. Evans Manuscripts is a group of manuscripts given to the National Library by Albert Owen Evans. They include correspondence and papers relating to A. O. Evans.

Papers of Henry Richard and his family, [early 19 cent.]-1904, including correspondence, 1808-1904; travel journals, 1849-1886; a few items relating to education in Wales, 1870-1883; sermons by Ebenezer Richard, [early 19 cent.]-1834; a family register, 1809-1836; and papers of James Hughes (Iago Trichrug), [1800x1844].

Records of Davies Brothers, 1800-1896, and of the Cardigan branch of Swansea Old Brewery & Davies' (Cardigan) Bonded Stores Ltd., 1896-1921, including ledgers, 1872-1908, day books, 1872-1918, press letter books, 1878-1919, cash books, 1879-1912, bills, 1893-1913, order books, 1898-1921, receipts, 1904-1910, records relating to orders, 1904-1920, and letters from the company's Swansea and Pembroke branches, 1905-1920, together with a group of additional papers, [19 cent., last ¼]-[1930s], 1980. Papers of John Davies, solicitor, 1804-1883, including electoral registers for the Cardigan boroughs, 1834-1839, and papers relating to the business affairs of Daniel Davies of The Bonded Stores, Cardigan, 1878-1882.

Manuscripts once belonging to E. Penllyn Jones (d. 1902), Calvinistic Methodist minister and librarian of the University College of Wales, Aberystwyth, comprising notes on the psalms; transcripts by Thomas Charles Edwards (1837-1900) of miscellaneous correspondence; examination answers, 1871; and essays on education in Wales and on Welsh hymn writers.

A collection which includes poetry by Edward Evans (Iolo Gwyddelwern), Hugh Morris (1830-1908) and David Roberts (Dewi Havhesp), together with a fragment of a sermon by David Owen (Dewi Wyn o Eifion).

A collection of notebooks and collectanea of David Harris Williams (d. 1927).