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The original typescript of '"Hapus Dyrfa": nefoedd oes Victoria', the Islwyn memorial lecture delivered by Dr. R. Tudur Jones at University College, Cardiff, and published in Llen Cymru, 13, pp. 236-77.

The origin, character and development of Accentual verse in Welsh with special reference to Rhys Goch ap Rhicert by D. Lloyd-Jenkins, Llanddewibrefi (later Tregaron). English. Boards. Donated by Professor J. E. Caerwyn Williams, December 1967.

An autograph essay entitled 'The Origin of Moral Evil' by Thomas Gee, signed and dated 12 February 1837.

The origin and history of the Old Meeting House, Aberdare by Rees Jenkin Jones. (Formerly Rees Jenkin Jones MS.) English. In boards. Donated by Dr Goronwy Jones, Swansea.

A typescript volume on the history of the Oriel family of Pembrokeshire, written by O. J. Vaughan in 1983, and updated in 2001.

A collection comprising of 'articles' dating from 1780, with revised rules dated 1881, and further copies of articles; minutes; accounts, balance sheets, a bank pass book and financial statements; and correspondence relating to the 'Old Social Club', Aberystwyth.

The Old Eisteddfodau of Caernarvon by W. E. Davies (1851-1927). English. Between boards. Donated by Professor C. W. Davies, Aberystwyth, August 1960.

A copy of The Oddfellows' Magazine, vol. XLV, No. 475 (July 1914), containing a full account of The Annual Movable Conference of the Manchester Unity held at Aberystwyth, 1914.

The Normal College for Wales, Swansea: reports, and a biography of Evan Davies. English. Leather. Donated by D. T. Morgan, Barmouth, June 1960.

A copy of the second edition of Clement Moody: The New Eton Latin Grammar ... (London, 1840) containing a short note in the autograph of Richard Robert Jones (Dic Aberdaron) (1780-1843).

Letters, 1907-1908, mainly to W. B. Halhed, relating to the proposed formation in North Wales of a branch of the National Vigilance Association.

A booklet, [2010], produced for advertising purposes detailing the history of collecting photographs as specifed by the Royal Charter awarded to the National Library of Wales in 1907 and including examples of photography, 1841-1945.

The National Library of Wales Building Fund: London Welsh Committee minutes in the hand of R. H. Parry. English. Boards. Donated by the London Welsh Committee.

Mounted press cuttings, mainly from The Cambria Daily Leader, The Carmarthen Chronicle, The Carmarthen Journal, The Carmarthen Weekly Reporter, The Times, and The Welshman, consisting of reports on, and copies of correspondence relating to, the National Eisteddfod of Wales, held at Carmarthen, 2-6 September 1867, and copies of two letters, October 1867, addressed to the editor of the Welshman, relating to opinions, alleged by reviewers to have been expressed in Matthew Arnold: On the Study of Celtic Literature [(London, 1867)], p. 11, concerning the attitude of [Connop Thirlwall], bishop of St. David's, towards the Welsh language.

Balance sheets of National Eisteddfodau, 1880-1932, compiled by Isaac Davies, Birkenhead, with instructions for eisteddfod secretaries.

The National Diary of Wales, with MS notes by William Pugh, Argoed. (Formerly Bontddu MS.) Welsh, English. Cloth. Donated by Mrs Anne Pugh, Bontddu, March 1940.

A note on Cwpan Nanteos, the so-called healing cup kept at Nanteos, near Aberystwyth.

The Mystery of Elizabeth Canning, a story by Arthur Machen. (Formerly Caradoc Evans MS 6.) English. Unbound. Donated by Mrs M. Caradoc Evans, Penrhyncoch, 1946/1947.

Letters re. the Myddfai 'S. Paul inscription' by H. T. Payne, John Jenkins, Kerry, Thomas Beynon, etc. English, Welsh. Donated by W. Isaac Williams, London, 1948.