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The archive includes papers and letters of members of the Anwyl family of Chester, 1848-1983, including letters to Sir Edward Anwyl, Welsh scholar.

Personal archive of material relating to Gwasg Gregynog accumulated by the donor during his time as a director and trustee of the Press, 1998-2018.

Sub-fond A comprises papers related to Ann Jones's campaign for domestic fire safety measures in Wales, centering on the devolution of powers to the National Assembly for Wales for this purpose and the resulting legislation; the Domestic Fire Safety (Wales) Measure, 2011, which required sprinkler systems to be fitted to all newly built or substantially converted domestic residences in Wales. Sub-fond B comprises material related to Ann Jones' campaign against the closure of the North Wales Fire and Rescue Service control room in Rhyl. Sub-fonds C comprises material related to the Children's Society's decision to withdraw from Wales, and Ann Jones' efforts in the the subsequent establishment of Tros Gynnal Plant to continue that work. Sub-fonds D relates to the restructure of the National Health Service in Wales.

A visitors book and two 'rotation books' (session lists) relating to the studio of the photographer Angus McBean, 1945-1987.

Records relating to the Anglo-Welsh Review, mainly typescripts of material published in the magazine, 1957-1988, including editor's correspondence files, printer's copies and galley proofs, 1957-1988; and subscription lists, 1957-1975. The archive also includes correspondence and papers relating to the publication's demise and closure, 1981-2000 (November 2021 deposit).

Deeds, 1490-1977, including deeds and documents mainly relating to properties on Anglesey, Caernarfonshire, Merionethshire and Middlesex, 1675-1977; and deeds relating to properties in Finchley, Middlesex, 1490-1796.

Deeds, 1704-1912, relating to properties in the town of Denbigh and the parishes of Henllan and Eglwys-bach, Denbighshire.

Papers, 1966-2015, relating to the filming and production of Under Milk Wood (1972), directed by Andrew Sinclair, together with papers relating to the financing and distribution of the film and to other Dylan Thomas projects.

Personal papers of the photographer Alvin Langdon Coburn consisting mainly of correspondence concerning his association with several orders of freemasonry, 1903-1966. There is also a small amount of correspondence relating to his work as a photographer, 1913-1965, mainly concerning lectures broadcast by the BBC, but also including letters relating to the sale, by Coburn, of a small collection of letters from the American writer Henry James. The fonds also consists of lectures and associated notes, again mainly concerning Coburn's interest in freemasonry, 1937-[1966], dealing particularly with its history and origins; a few lectures reflecting particular aspects of his career as a photographer, and on his approach to photography, 1924-[1966]; together with some printed material, 1924-1966, primarily circulars from various Masonic lodges concerning forthcoming events. Given Coburn's important contributions to photography there is surprisingly little material which is of direct relevance to this aspect of his life within the archive. The additional group of material consists mainly of correspondence and papers relating to the administration of the estate of Alvin Langdon Coburn following his death and includes copies of his will and codicil and a Probate document proved at Bangor.

Papers of Alun-Oldfield Davies, 1928-1988, relating mainly to the artist and writer David Jones, including an original water-colour inscription, 1954; photographs of inscriptions, personalised and sent as greetings cards , 1958-1961; letters from David Jones to Alun Oldfield-Davies, 1954-1962; papers concerning the fate of David Jones's manuscripts and pictures, 1971-1976; miscellaneous items including lists of works by David Jones for exhibitions, 1972-1976, a radio talk broadcast in 1954 and articles on his life and work, 1954-1988. The additional papers comprise a copy of John Morris-Jones, Penillion Omar Khayyam (Gregynog Press, 1928), formerly in the possession of Colonel Richard C. Ruck (1887-1973), containing his manuscript annotations in Persian, Welsh and English, with letters from his widow concerning the bequest of the volume to Alun Oldfield-Davies, 1973-1974; and a notebook containing reminiscences in Welsh ('Stori fy mywyd') of the Reverend Jonathan Oldfield-Davies (1876-1960), Congregationalist minister and father of Alun Oldfield-Davies.

Papers of Alun Lewis, 1919-1996, including family correspondence and letters from Robert Graves; autograph and typescript copies of published and unpublished poems; typescript copies of published and unpublished prose; personalia; an unpublished autobiographical novella of college life; memorial tributes to Alun Lewis in poetry form; and notebooks containing poetry and other writings by him.

Deeds, mainly relating to the Alltlwyd estate, 1617-1869, chiefly in the parishes of Llanrhystud and Llansanffraid, Cardiganshire.

A large collection of Alistair Crawford's papers relating to his academic and artistic career in Wales.

Literary papers, 1964-1995, juvenilia, 1939-1942, and journals, 1966-1994, of Alison Bielski, together with her work journals, 1995-2002 .

Papers of Alfred T. Davies, 1875-1965, including family and personal correspondence, 1887-1949; papers relating to the British Prisoners of War Book Scheme, 1914-1918; and papers relating to his works, including Student captives, I (1917), Student captives, II, Robert Owen... a memoir (1948), The Lloyd George I knew (1948), and intended books Light through prison bars and Owned of God: or Moody and Sankey, 1875 and 1883: some memoirs and a tribute, with a Welsh translation by Rev. E. K. Jones, 1945. Also three bound volumes of the printed magazine produced by civilian prisoners at Ruhleben Camp near Berlin.

Manuscripts, [1850]-[1915], of Alcwyn C. Evans, mainly comprising antiquarian and historical material relating to Carmarthenshire and other places in Wales and including transcripts from parish registers, public records and other sources, and Welsh pedigrees and genealogical records compiled by Alcwyn C. Evans.

Deeds, 1815-1931, relating to the manor of Llanfihangel Talyllyn and other properties in Brecknockshire, together with a court book, 1859-1908, of the manor of Llanfihangel Talyllyn; notebooks and exercise books, containing notes on historical, genealogical, and heraldic material mainly about the town and county of Brecon, taken from various printed and manuscript sources; notes and sketches relating to the armorial bearings of Brecknockshire families, and extensive transcripts of parish registers and of monumental inscriptions; a file of typescript notes concerning the Breconshire Agricultural Society; some notes in the hand of John Lloyd compiled in pursuance of his historical researches; a file of notes, transcripts, and correspondence relating to the parish of Llanfeugan; a manuscript volume, compiled c. 1880, of transcripts of inscriptions, sometimes with additional notes and sketches, of tablets and monuments in Brecknockshire churches and a few Nonconformist chapels, drawings of archaeological remains, etc.; a further file of transcripts of monumental inscriptions in several Breconshire churches and churchyards; a scrap- book of newspaper cuttings relating to the Turco-Greek war of 1897; and a group of eleven deeds, mainly of Brecknockshire interest, 17th-19th cent.

A collection, 1804-1908, which includes parochial and financial returns, reports and correspondence relating to the diocese of Bangor.

This collections comprises minutes of meetings and subscriptions relating to Aberystwyth Baptist College, college note books, sermons, lectures and correspondence.