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Poetical compositions, 1824-1827, submitted for competition at 'Eisteddfod y Fottas' (the Boot Eisteddfod), held by Cymdeithas Cadair Merthyr Tydfil at the Boot Inn (Arwydd y Fottas), Merthyr Tydfil, together with some adjudications (T9/1, 2 folders). Also included are copies, 1823-1827, of posters advertising the eisteddfodau (T9/2).
Taliesin Williams was secretary to Cymdeithas Cadair Merthyr Tydfil. Some of the compositions were printed in Awenyddion Morganwg; neu, Farddoniaeth Cadair Merthyr Tudful (Merthyr Tydfil, [1826]).

Miscellaneous papers of Iolo Morganwg, collected in seven bundles with little or no unity (E9/1-7). Included is a bundle of fragments found amongst the papers of his son Taliesin (E9/7).

A collection of psalm-tunes ('erddiganau salmau') by Edward Williams (Iolo Morganwg).

Twenty-two notebooks and bundles, 1817-[1839], containing notes and memoranda by Taliesin on a variety of subjects. The volumes comprise notebooks, 1817-[1839] (T2/8, 10) and undated (T2/1-6, 12-15); bundles of miscellaneous loose papers (kept in old covers) (T2/7, 9, 11); old covers with no contents (T2/16-17); and notebooks relating to Welsh Triads (T2/18-22, as well as parts of T2/10).

Miscellaneous notes and papers of Iolo Morganwg, [18 cent., last ¼]-[1830s], on a variety of subjects, including (mainly Welsh) history (E8/1), religion (E8/2), Welsh and English literature, including Dr Johnson (E8/3), Bardism (E8/4) and biography and genealogy (E8/5); together with further bundles of miscellaneous notes and papers, retained in original order (E8/6-9), with subjects including politics, printing and Poems Lyric and Pastoral, 1784-[c. 1809] (E8/6), patriarchal religion, priestcraft and Lewis Morris (E8/7), poetry and monumental inscriptions (E8/8) and salmau (E8/9); and a case containing notes on Welsh manuscripts in the British Museum and at Jesus College, Oxford (E8/10).

Papers, [16 cent., second ½]-[1830s], of Iolo Morganwg, including manuscript music, [18 cent., last ¼]-[19 cent., first ¼], and printed sheet music, [17 cent., second ½]-[late 18 cent.]; hymns, [19 cent., first ¼]; travel journals, 1796-1815; Welsh and English poetry, 1776-[1826]; notes and notebooks, [18 cent., last ¼]-[1830s]; financial papers, 1782-1826; old covers, [18 cent., last ¼]-[19 cent., first ¼]; financial papers of Iolo's grandfather Edward Matthew, 1705-1736; and miscellaneous collected deeds and documents, [16 cent., second ½]-1824.

Manuscripts, [16 cent.]-[?1841], mostly collected or written by Iolo Morganwg. They include transcripts of Welsh poetry, pedigrees, grammars, and manuscripts belonging to Robert Vaughan of Hengwrt, Lewis Morris, Gwallter Mechain, Ieuan Brydydd Hir, Thomas Glyn Cothi, Richard Morris and others; literary papers of Iolo Morganwg, including hymns and psalm-tunes, English and Welsh poetry and Bardic papers; other papers including diaries, memorandum books and notebooks; and accounts of his father, Edward Williams, senior.

Bills, receipts and other financial papers of Taliesin Williams, 1811-1820 (T11/1), 1821-1844 and undated (T11/2); and day books, etc., 1811-1819 (T11/3-5).
Some of the papers apparently relate to Taliesin's school.

Letters (surnames Davies-Hall) addressed mostly to Taliesin Williams (Taliesin ab Iolo).
The correspondents include Walter Davies (Gwallter Mechain), [1812]-1837 (Nos 130-135), David Davis, Neath, 1810-1841 (Nos 137-148), John Davis (Brychan), 1829-1841 (Nos 149-157), Lady Charlotte Guest, 1837-1843 (Nos 191-202), and Augusta Hall, 1834-1841 (Nos 206-250).

Correspondence and other papers broadly relating to various aspects of Taliesin's public life and work in Merthyr Tydfil and elsewhere. The file contains: some fifty-four draft and copy letters, or parts of letters, written by Taliesin Williams, including many letters to newspapers, 1831-1845, some twenty-seven letters and envelopes addressed to Taliesin and others, 1808-1843, and miscellaneous calling cards and addresses (T10/1); miscellaneous papers relating to his work as a schoolmaster in Neath and Merthyr Tydfil (T10/2); papers relating mostly to various aspects of public life in Merthyr Tydfil, including papers apparently relating to his service as special constable, various petitions to the Crown, the Marquess of Bute and others, and a few items relating to the Merthyr Tydfil Sympathetic Society, 1831-1839 (T10/3); and various papers relating to his activities with groups such as Cymreigyddion y Fenni and Cymreigyddion yr Alarch, being mainly lists of competition subjects, entries and adjudications by him (T10/4).
Of particular note is the beginning (2 pp.) of a draft, in Taliesin's hand, of a petition sent by the people of Merthyr Tydfil to Lord Melbourne, the Home Secretary, in July 1831 pleading for clemency for Lewis Lewis (Lewsyn yr Heliwr) and Richard Lewis (Dic Penderyn) (the final petition is apparently lost, see Gwyn A. Williams, The Merthyr Rising (Cardiff, 1988), p. 184) (in T10/3).

Thirty-six notebooks, 1806-1846, containing notes and memoranda by Ab Iolo on a variety of subjects.

Miscellaneous printed items found among the papers of Taliesin ab Iolo, including pamphlets, offprints, handbills, newspaper cuttings, maps, engravings, posters and a copy of The Cardiff Guide and Directory (Cardiff, 1829).

Drafts and notes in the hand of Taliesin Williams for the volume Iolo Manuscripts, A Selection of Ancient Welsh Manuscripts, in prose and verse, from the collection made by the late Edward Williams, Iolo Morganwg,… with English translations and notes by his son, the late Taliesin Williams (Ab Iolo) of Merthyr Tydfil (Liverpool: Welsh MSS Society, 1848).
Included are manuscript drafts of the Welsh texts on pp. 3-328 passim (T4/1), drafts of the English translations on pp. 341-496 passim (T4/2), drafts for the footnotes on pp. 332-489 passim (T4/3), a draft of pp. 331-507 passim combining text and footnotes (T4/4), and notebooks containing notes and memoranda relating to the volume (T4/5-11). Also included is a bundle of draft texts, relating mostly to Welsh saints in a format similar to T4/1 but which were either omitted from the volume or intended for another book on Bonedd y Saint (T4/12).

Notebooks and loose papers containing drafts and notes by Taliesin Williams relating to various books and essays, especially to his unpublished works on Merthyr Tydfil (T5/1-5), Llandaff (T5/6-13) and Sion Cent (T5/14-16).
Also included are papers relating to Coelben y Beirdd, Cyfrinach Beirdd Ynys Prydain and possibly other publications (T5/17-18, see also T5/4) and fragments relating to his essay on the Neath Valley (T5/19).

Notebooks and other volumes containing Welsh poetry, including drafts, fragments and notes, mostly by or in the hand of Taliesin ab Iolo (T6/1-22).
Seven volumes (T6/16-22) appear to been used by school pupils to copy out English poetry, later re-purposed by Taliesin for his own Welsh poetry.

Welsh poetry, including drafts, fragments and notes, mostly by or in the hand of Taliesin ab Iolo, comprising: loose poems which are either complete or relatively substantial (T7/1), with two further bundles of more fragmentary poems, drafts and notes (T7/2-3); three bundles of loose poetry retained in original order (T7/4-6); and items in hands other than that of Taliesin ab Iolo (T7/7).

English poems and fragments, drafts and notes, mainly in the hand of Taliesin Williams, comprising poems generally of a more substantial or complete nature (T8/1), a bundle of smaller notes and fragments (T8/2), a bundle of poems in a generally poor condition (T8/3), notebooks containing poetry (T8/4-5), and notebooks and loose papers containing drafts and notes for Taliesin's poem The Doom of Colyn Dolphyn (London, 1837) (T8/6-11).

Miscellaneous notes broadly relating to Welsh and Glamorgan history, Welsh literature and related subjects. They comprise: bundles of loose papers (T3/1-2) and notebooks (T3/3-14) containing notes and memoranda on a variety of historical subjects, including Bonedd y Saint; notebooks and loose notes on Welsh poetry and poets (T3/15-18); miscellaneous notes on sayings, idioms, etc. (T3/19); a few recipes for ink and toothache (T3/20); miscellaneous fragments, together with three maps drawn on tissue paper (T3/21); a bundle of annotated wrappers used by Taliesin to sort some of his and his father's papers (T3/22 – see also T13/7); six booklets, 1838-1839, containing extracts from manuscripts relating to Wales at the British Museum and Bodleian Library (T3/23); a bundle of foolscap sheets containing mostly genealogical texts relating to Welsh saints and legendary figures (T3/24); and a transcript of a lecture on Oriental languages 'Delivered by Professor [Duncan] Forbes at K[ing's] C[ollege] London', November 1837 (T3/25).

Letters, 1809-1864, addressed mainly to Taliesin Williams (Taliesin ab Iolo), Glebe land, Merthyr Tydfil, along with some letters, copy letters and draft letters from Williams, 1813-1847.

One hundred and twenty-two letters, 1879-1885, from Edward Williams, Middlesbrough, to his second son Aneurin Williams.