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Notebooks and loose papers containing drafts and notes by Taliesin Williams relating to various books and essays, especially to his unpublished works on Merthyr Tydfil (T5/1-5), Llandaff (T5/6-13) and Sion Cent (T5/14-16).
Also included are papers relating to Coelben y Beirdd, Cyfrinach Beirdd Ynys Prydain and possibly other publications (T5/17-18, see also T5/4) and fragments relating to his essay on the Neath Valley (T5/19).

Notebooks and other volumes containing Welsh poetry, including drafts, fragments and notes, mostly by or in the hand of Taliesin ab Iolo (T6/1-22).
Seven volumes (T6/16-22) appear to been used by school pupils to copy out English poetry, later re-purposed by Taliesin for his own Welsh poetry.

Welsh poetry, including drafts, fragments and notes, mostly by or in the hand of Taliesin ab Iolo, comprising: loose poems which are either complete or relatively substantial (T7/1), with two further bundles of more fragmentary poems, drafts and notes (T7/2-3); three bundles of loose poetry retained in original order (T7/4-6); and items in hands other than that of Taliesin ab Iolo (T7/7).

English poems and fragments, drafts and notes, mainly in the hand of Taliesin Williams, comprising poems generally of a more substantial or complete nature (T8/1), a bundle of smaller notes and fragments (T8/2), a bundle of poems in a generally poor condition (T8/3), notebooks containing poetry (T8/4-5), and notebooks and loose papers containing drafts and notes for Taliesin's poem The Doom of Colyn Dolphyn (London, 1837) (T8/6-11).

Poetical compositions, 1824-1827, submitted for competition at 'Eisteddfod y Fottas' (the Boot Eisteddfod), held by Cymdeithas Cadair Merthyr Tydfil at the Boot Inn (Arwydd y Fottas), Merthyr Tydfil, together with some adjudications (T9/1, 2 folders). Also included are copies, 1823-1827, of posters advertising the eisteddfodau (T9/2).
Taliesin Williams was secretary to Cymdeithas Cadair Merthyr Tydfil. Some of the compositions were printed in Awenyddion Morganwg; neu, Farddoniaeth Cadair Merthyr Tudful (Merthyr Tydfil, [1826]).