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Records relating mainly to the industrial concerns of the Crawshay family of Cyfarthfa, Merthyr Tydfil, Glamorgan, [1706]-1878, including letters and letter books of William Crawshay I and II and Robert Crawshay, 1806-1877; cash books, ledgers and bankers drafts, 1834-1888; deeds, [1706]-1885; wills, deeds and miscellaneous material, 1801-1838; balance sheets for ironworks, 1810-1867; will, valuation and probate for William Crawshay II, 1865-1869; shares and bills of exchange, 1870-1878; and Hilston Park estate papers, 1838-1862 and Caversham Park estate papers, 1826-1864. The archive represents the working papers of a major ironworking dynasty.

The collection consists of election addresses, leaflets, circulars and other printed matter, 1837-1991, generally acquired before the establishment of the Welsh Political Archive; election addresses, leaflets etc., 1905-2019, collected by the WPA; and printed materials, 1887-2019, concerning the political parties in Wales, various pressure groups and organisations, subject files, and other miscellaneous papers.

Papers relating to the Liberal Party of Wales, 1961-1962, mainly pertaining to appointing a national organiser for the Party.