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Records of the Peterwell and Falcondale estates of the Harford family, in Cardiganshire and Carmarthenshire, including Peterwell estate papers, 1696-1963, including deeds, accounts, surveys and valuations; Lampeter Town estate papers, 1868-1954, Tresaith estate papers, 1886-1975, Blaise Castle estate papers, 1834-1938; and manorial records relating to the borough of Lampeter, 1741-1848.

Records of the Esgair and Pantperthog estates, Merionethshire, and of the Ruck family, comprising deeds and documents relating to lands in Merioneth, Cardiganshire, and Kent, 1509-1939, letters and papers relating to the Plas Gwyn estate, Anglesey, 1659-1822, and Welsh manuscripts of more than one Oliver Morris of Esgair Lleferin, Merioneth, 17 cent.-18 cent.

Papers of the Rev David Evans, [1851]-1993, comprising papers relating to Cribyn Unitarian Chapel, Cardiganshire, including notebooks and volumes containing various chapel accounts, 1851-1927; papers relating to Cribyn Day school, 1888-1942, including account books, 1888-1909, one of which contains the Cwmiago household and farming accounts, 1904-42, and class attendance registers, 1890-1905; volumes of David Evans' sermon notes, [1893x1946]; addresses, [1880x1950]; plays, [1880x1950]; poetry [not written by David Evans], [1880x1950]; prose works, [1880x1950]; religious material, [1880x1950]; miscellaneous papers, [1880x1993], including recollections of Rev. David Evans by his great-great niece Gwenlyn E. Thornton; and printed material, 1865-1950.

Papers of the South Wales Women's Temperance Union, including correspondence, 1911-1965; minute books and accounts of meetings, 1931-1957; account books, 1916-1966; printed material, 1948-1957; hymn sheets, 1839-1966; and posters, 1932-1957.

The fonds comprises papers, [1936]-2002, reflecting the diverse interests and actvities of Dr Goronwy Alun Hughes such as minority languages, anthropology, genealogy, libraries and the voluntary services in Wales, including personal and business correspondence and microfiche of Pacific interest; together with the papers of Brenda Hughes, his second wife, relating to Romanian life; and of his late wife Dr Zuzana Hughes relating to social work.

A collection of miscellaneous letters and papers, 1757-1993, purchased or received by donation from various sources by the National Library of Wales during the period June 2008-May 2013 and boxed as one volume.

Papers of and acquired by R. Bryn Williams, mainly relating to the Welsh settlement in Patagonia, including a diary of Joseph Seth Jones, one of the first wave of emigrants on the Mimosa to Patagonia, 1865, and correspondence, 1865-1868; correspondence of his brother, Robert Charles Jones, 1867-1877; copy records of the Welsh courts in Y Wladfa, 1872-1881; letters and minute books relating to Vrondeg Baptist Chapel, 1875-1887, Gaiman, 1877-1891, Eglwys Llanddewi, 1891, Eglwys Bryn Gwyn and Cyfarfod Misol Y Wladfa (Calvinistic Methodists), 1881-1955; papers relating to the Centenary Celebrations of the Welsh settlement in Patagonia, 1952-1962; letters from the founders of the Welsh colony, 1866, and from others who had experienced life there; letters to R. Bryn Williams from Patagonia and from Wales relating to Patagonia, [c. 1941-1961]; research notes and manuscripts of books and radio plays by R. Bryn Williams, 1942-1962; miscellaneous records relating to Wales and elsewhere collected by Williams, 1865-1962; papers relating to John S. Williams, 1901-1962; papers and press cuttings on the history, culture and industry of Patagonia, 1869-1962; and typescripts of published and unpublished works, lectures, scripts, etc.

Deeds and documents, [c. 1753]-1927, relating to properties in the counties of Brecknockshire, 1815-1834, Cardiganshire, [c. 1753]-[c. 1853, Glamorgan, 1851, Montgomeryshire, 1803-1857, Monmouthshire, 1843, and Pembrokeshire, 1819-1927, referred to the Treasury Solicitor for advice or litigation.

A collection of deeds relating to various Welsh counties, 1626-1830, including a group relating to the Parry family of Llanrhaiadr Hall, Denbighshire, 1698-1830.

Literary, family and business papers, 1732-1982, of Lewis Lewis ('Awenfab o Wynfe', 1837-1906), poet, of Gwynfe, Carmarthenshire, his son, Dr Ivor Lewis, St Asaph, and other members of his family, including drafts of poetry by Lewis Lewis; denominational diaries, 1848-1908; and letters, including correspondence, 1854-1947, between Lewis Lewis and relatives and friends in the United States and Canada.

Letters, 1910-1944; scrapbooks, 1893-1948; poetry, 1910-1952; manuscripts and typescripts of prose compositions, essays, articles and addresses, [1909]-1918; sermons, undated, [1897x1953]. None of her major works are represented among the papers.

Deeds relating to Pencrug and other properties in the parishes of Llanafan Fawr and Llanafan Fechan, Breconshire, 1587-1863.

The collection consists of the Goodwyn of Dorking deeds, 1573-1754; Coke of Holkham deeds, 1671-1786; Montagu, duke of Montagu deeds, 1690-1735; Berenger of Iver deeds, 1693; Macro family deeds, 1711-1739; Boucherett of Lincolnshire deeds, 1720-1738; Brancaster Great Malthouse deeds, 1722-1729; Hooper of London deeds, 1723-1747; Spencer, duke of Marlborough deeds, 1735; Lamb of Lincoln's Inn deeds, 1737-1815; Southampton Street deeds, 1760; Waldo of Clapham deeds, 1769-1796; Edmunds of Grays Inn deeds, 1776-1788; miscellaneous deeds: Cardiganshire, 1672-1810; and miscellaneous deeds: England, 1699-1811.

Records collected by the United Reformed Church in Wales, 1868-1973, including Wood Street English Congregational Church, Cardiff, registers, 1891-1959, and roll books, minute books and accounts, 1868-1972; St John's English Congregational Church, Flint, subscription books, 1970-1973; English Congregational Union of North Wales, minutes and other papers, 1882-1970; Flintshire District English Congregational Union, minutes and other papers, 1935-1972; Montgomeryshire English Congregational Union, minutes, 1928-1973; trust deeds and legal papers, 1948-1968; Pembrokeshire English Congregational Union, meeting attendance book, 1952-1972; and miscellaneous correspondence, printed material and addresses, 1954-1972. ; church accounts, 1930-1949 ; minute book of Wood Street Congregational Church, Cardiff, 1868-1873; attendance book of Association and executive committee meetings of the Pembrokeshire English Congregational Union, 1952-1972.

Papers of, or accumulated by, [1700x1915], D. Lleufer Thomas, comprising material relating to the Welsh Land Commission, miscellaneous prose and verse, correspondence and other papers.

Family papers and estate records of the Williams family of Cwmcynfelyn, Cardiganshire, comprising rentals, 1833-[1885], valuations, [1849]-1879, financial papers, 1826-1899, deeds of the Cwmcynfelyn estate in north Cardiganshire, and in the parish of Machynlleth, Montgomeryshire 1773-1886, deeds relating to Penpompren in Llanfihangel Genau'r-glyn, 1724-1791 (including a schedule of deeds dating back to 1694), which probably found their way to Cwmcynfelyn through the marriage of Matthew Davies Williams of Cwmcynfelyn and Susanna Griffith in 1828; papers relating to the Donisthorpe and Mapperley collieries, Leicestershire, 1874-1899; papers relating to the Gogerddan estate, Cardiganshire, accumulated by George Griffiths Williams as agent until his retirement, 1852-1895; and personal papers of Mathew Davies Williams, 1821-1864.

Papers of Gwyn Griffiths, 1970-1988, including various Liberal Party pamphlets, 1970-1981; papers concerning the Welsh League of Young Liberals, 1975-1977; correspondence and papers concerning the Liberal Ecology Group, 1978-1984; correspondence and papers concerning the Liberal Parliamentary Association, 1986-1988.

The fonds contains the business and personal papers of J. E. Powell.

Collection of deeds and other papers, [1310]-[1958], of Gwendoline Elizabeth Davies and Margaret Davies, including printed books, 1478-1844, papers concerning the Gregynog Press, 1922-1960, copies of books, 1923-1940, ephemera, 1927-1962, designs and drawings, n.d.; and deeds relating to properties in Montgomeryshire, 1597-1832.

Correspondence and papers of T.G.G. Herbert together with historical records acquired by him, 1736-1899, general and political correspondence, 1953-1986, much of it relating to the work of the Ceredigion District Council; papers relating to the Cardiganshire County Council elections, 1955-1972; personal papers, 1936-1988; and papers relating to his son Rhodri Herbert, 1954-1972.

An additional five boxes of papers were donated February 2006. This group remains uncatalogued. A collection of photographs, slides and postcards were received at the same time, which also remain uncatalogued.