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Records relating mainly to the industrial concerns of the Crawshay family of Cyfarthfa, Merthyr Tydfil, Glamorgan, [1706]-1878, including leters and letter books of William Crawshay I and II and Robert Crawshay, 1806-1877; cash books, ledgers and bankers drafts, 1834-1888; deeds, [1706]-1885; wills, deeds and miscellaneous material, 1801-1838; balance sheets for ironworks, 1810-1867; will, valuation and probate for William Crawshay II, 1865-1869; shares and bills of exchange, 1870-1878; and Hilston Park estate papers, 1838-1862 and Caversham Park estate papers, 1826-1864. The archive represents the working papers of a major ironworking dynasty.

Political correspondence and papers accumulated by Godfrey Lee, 1968-1988, relating to Plaid Cymru activities in Newport, 1968-1978, Plaid Cymru's Montgomeryshire branch, 1977-1988, and Welshpool branch, 1978-1980; the work of Gwent Regional Council [of Plaid Cymru], 1969-1977; together with Plaid Cymru Conference Programmes, 1969-1988; and literature concerning the Merthyr Tydfil by-election, 1972.

Papers of Harri Webb, [c. 1919]-1995, including poetry, 1942-1989; reviews and reader's reports, 1974-1986; correspondence with publishers, broadcasters and editors relating to Webb's work, 1949-1995; correspondence from literary and artistic figures, [1940s]-1983; political correspondence, 1964-1974; political press cuttings, 1952-1981; papers relating to Plaid Cymru, 1961-1978, and Scottish politics, 1967-1969; and personal papers, [c. 1919]-1984.

A collection of Harri Webb's diaries. This group remains uncatalogued.