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A typescript essay entitled 'Casgliad o weithiau Sion Brwynog, gyda nodiadau hanesyddol a beirniadol' by the late the Reverend Gilwym H[ywel] Jones, Welsh Presbyterian minister, Blaenclydach, co. Glamorgan. The essay, under the pseudonym of 'Emrys', was awarded the prize at the National Eisteddfod at Holyhead, 1927, and pasted into the volume is a typescript copy of the adjudication of Professor Sir John Morris Jones and Professor Henry Lewis.

Three copybooks of lecture notes, 1902-1904, compiled by John Tudor of Hebron, Pembrokeshire, whilst an undergraduate at the University College of North Wales, Bangor.
The volumes include notes on Welsh poetry (1450-1600) and exercises in Hebrew grammar (NLW MS 16192iB); notes on Welsh poetry (1300-1450), notes on Welsh and Irish philology and a comparative list of Irish and Welsh words (NLW MS 16192iiB); and notes on Welsh poets of the fifteenth century (NLW MS 16192iiiB). A note from the donor is included (with NLW MS 16192iB)

A commonplace book of prose and verse, including a fragment on husbandry, recipes, a charm, astronomical and tide tables, 'Ystori Peilatvs', 'Ystori Adda', 'Ystori Noe Hen', 'Ystori Suddas', 'Araith Gwgan', an extract from Y Ffydd Ddi-ffvant, interpretations of dreams, a calendar for 1695, and poetry by Aneirin Gwawdrydd (fl. second half 6 cent.), Taliesin (fl. end 6 cent.), Hywel Cilan (fl. c. end 15 cent.), Sion Cent (c. 1400-15 cent.), Dafydd Nanmor (fl. 15 cent.), Dafydd ab Edmwnd (fl. 1450-1490), Dafydd ap Gwilym (fl. 1315/20-1350/70), Iolo Goch (c. 1320-1398), Morys ap Hywel (fl. c. 1530), Gruffudd ab Ieuan (c. 1485-1553), Sion Brwynog (d. ?1567), Sion Tudur (c. 1522-1602), Huw Morys (1622-1709), Dafydd ap Rhys (fl. c. 1550), Lewys Morganwg (fl. 1520-1565), Robert Leiaf, Guto'r Glyn (c. 1435-c. 1493), Gruffudd Gryg (fl. 1357-1370), Maredudd ap Rhys (fl. 1440-1483), Tudur Aled (c. 1465-c. 1525), Gruffudd ap Dafydd ap Hywel (fl. 1480-1520), Syr Dafydd, Rhys Cain (d. 1614), Gruffudd Llwyd ab Einion (fl. c. 1380-1410), Wiliam ap Sion ap Dafydd, and Thomas Prys (1564?-1634). Some 'englynion' and memoranda have been written in the margins by Evan Thomas, Cwmhwylfod (d. 1781).

Manuscripts, [late 12 cent.]-[early 20 cent.], formerly part of the library of the Mostyn family of Mostyn Hall, Flintshire, comprising transcripts and extracts from Giraldus Cambrensis, Geoffrey of Monmouth, Dares Phrygius, Nennius, Gildas, David Jenkins (Judge Jenkins), Sir John Wynn of Gwydir, Lydgate's 'Life of Our Lady', Leland's Itinerary, 'Chroniques de France', historical manuscripts such as Brut y Tywysiogion and Brut y Brenhinoedd, Welsh romances and the Mabinogion; collections of mainly Welsh poetry, among them the seventeenth-century volumes Llyfr Coch Nannau and Llyfr Gwyn Corsygedol, containing poems by Dafydd ap Gwilym, Guto'r Glyn, Tudur Aled, Siôn Cent and others; genealogies, pedigrees and histories; official papers relating to Caernarvonshire; catalogues of the Mostyn and Gloddaeth libraries, 1692-1842; etc.

An incomplete miscellany, in the form of three unbound volumes, of free- and strict-metre poetry (including illustrative extracts), compiled by David Thomas ('Dafydd Ddu Eryri') under the title of 'Golwg a'r Parnassus, a Helicon, Sef, Casgliad neulltuol, neu Bigion Dewisol Allan o Waith Prif feirdd neu Brydyddion yr oesoedd, sef y Rhannau hyny o'u Gwaith na ymddangosodd yn argraphedig Hyd yn hyn ond mewn hen Sgrifeniadau, yn Englynion A chywyddau. yn Ddwy Rann; un yn Ddigrifol ar llall yn ddifrifol. O Gascliad, Dewi, ab Thomas, Waunfawr. A Sgrifenwyd yn y flwyddyn 1781'. The preface ('Rhagymadrodd at y Darllenydd') indicates both the period and partly the source of the volume: 'Y Darnau canlynol o Brydyddiaeth a Sgrifennwyd Gennyf yn fy Ieuenctyd, Pan ddechreuais Gyntaf Gael blas, ar farddoniaeth Reolaidd Ac yn ol fy nhŷb i, y Pryd hwnnw, maent yn Brif orchestwaith, Pigion, neu oreuon, Gwaith yr hen Feirdd ... Yr a adsgrifennais wrth ymdeithi[o] yn ddamweiniol, heibio'r lleoedd yr oeddynt iw gweled fel y Gwelwch yn Enwau'r Eglwysydd'. The poets represented include Rhichard Phylip; Maredudd ap Rhys; David Thomas ('Dafydd Ddu Eryri'); Hugh Hughes ('Y Bardd Coch o Fôn') (1766); Huw Morys; Siôn Cent; William Phylip; Elis Roberts; Dafydd ap Gwilym; Siôn Phylip; Bedo Brwynllys; Tudur Aled; Gruffudd Hiraethog; Siôn Brwynog; Siôn Tudur; Edward Morys; Owen Gruffydd; and Siôn Mawddwy. The titles include 'Englynion i Sir feirionydd'; 'Englynion Iw gosod ar fedd Huw Jones o Langwm ...'; and 'Englyn i Hugh Lloyd Cynfel'. Additions in other hands include some music scores of carol tunes and calligraphic exercises.

A volume of transcripts of poetry, mainly 'cywyddau' and 'englynion', by Iowerth Fynglwyd, William Llŷn, Huw Cae Llwyd, Gwilym ap Sefnyn, Dafydd Nanmor, Thomas Prys, Syr Dafydd Trefor, Aneurin Gwawdrudd ('Anearan Gwowdrudd'), Rhys Pennardd, Iolo Goch, Gutun Ceiriog, Siôn Mawddwy, Dio ap Ifan Du, Rhys Goch Glyndyfrdwy, Dafydd ap Edmwnd, Dafydd Ddu o Hiraddug, Philip John Philip, Siôn Philip, Owain Gwynedd, Ieuan Brydydd Hir, Siôn Cent, David Jones, Rhys Wynn, Siôn Tudur, Dafydd ap Gwilym, Dafydd Llwyd ap Llywelyn ap Gruffudd, Meredydd ap Rees, Llywelyn ap Gutun, Syr Owain ap Gwilym, Griffith Philip, Rowland Vaughan, Richard Philip, Edmwnd Prys, Robin Ragett, Tudur Aled, John Prichard Prys, Robert Klidro, Ellis Rowland 'o Harlech', Hugh Llwyd 'o Gynfal', Huw Morris, Lewis Morris, Mr. David Roberts, Rice Lloyd, Moris ap Robert, Bala, and Thomas Jones, Orsedd Las. The greater part of the volume was written in the early eighteenth century. Among slightly later hands at the end of the volume is that of William Jones of Orsedd Las. At the end of the volume is a letter from a Welsh emigrant, written from Delaware, 21 September, 1828.

Llangibby Castle estate records, including court rolls of manors in Monmouthshire, 1262-1911, Glamorgan, 1675-1739, Gloucestershire, 1427-1595, and Somerset, 1609-1691; title deeds, mainly Monmouthshire, 1217-1930, and correspondence, mainly 18-19 cent.; important letters and papers relating to the civil war in Monmouthshire; and manuscripts aquired by the family, including drafts and copies of Modus Tenendi Parliamentarum and Observata Parliamentaria by Henry Elsynge, junior (1598-1654), clerk to the House of Commons, together with minutes of the House of Commons, 1624-1626, calendar of the Journal of the House of Lords, 1647-1768, copies of the Journals of the House of Commons, 1547-1701, index to parliamentary proceedings, temp. Edward III-Edward IV, and, 1724-1743, civil war tracts, the journal of the missionary Dr Joseph Wolff, 1832, 'Prif Achae holh Gymru Benbaladr' in the autograph of Sir Thomas Wiliams, Trefriw, 1578-1609, a seventeenth-century collection of Welsh poetry by the principal 'cywyddwyr'; a memoir of Richard Robert Jones ('Dic Aberdaron', 1780-1843) in his own autograph; English sermons and miscellaneous notes by Rev. Edmund Jones, Pontypool, a sermon notebook of Rev. Philip Henry (1631-1696), the eminent Nonconformist divine, a survey of the lands of Henry, earl of Pembroke, in Glamorgan and Monmouthshire, 1570, and a survey of lands in the lordship of Usk, 1619; pedigree rolls of Sir Roger Williams of Penrhos, Monmouthshire, compiled by Thomas Jones ('Twm Siôn Catti'), 1591, and of the Williams family of Llangibby Castle, probably compiled by Sylvanus Morgan.

A volume of popular Welsh poems on religious and scriptural themes written c. 1673-1674 by James Phillipp(es), with additions made a generation later by Phillipp James. The poems belong to the type of verse known in Cardiganshire as 'halsingod'. Linguistic evidence suggests that the authors were natives of East Carmarthenshire.