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Estate and family records of Mansel, later Talbot, of Penrice, and its estates in Gower, Glamorgan, from the 16th cent.; including records of Margam Abbey, 12-19th cent., including charters from its foundation in c. 1147, together with royal charters, charter rolls and papal bulls, which form one of the most complete series of archives of any medieval abbey in Great Britain; substantial early archives for Penrice, and other estates, mostly in Glamorgan; manorial records for the manor of Margam Abbey and others; early records of the coal industry in Glamorgan; a large group of Mansel correspondence, 1568-1848, along with some papers relating to Williams of Plas Dyffryn Clydach, largely literary, 17th cent.-18 cent.

Papers of Wynford Vaughan Thomas, 1850-1986, including war despatches, 1943-1945; papers relating to Indian independence, 1947; scripts of radio programmes on the Middle East, 1956; papers relating to state occasions, 1950-1956; notes for a proposed book on the river Niger, 1961-1963; manuscript and typescript copies of stories, articles, lectures, etc., 1947-1964; scripts of radio and TV programmes and proposed programmes, 1946-[1980s]; notes for proposed works on autobiography, 'Journeys', the River Niger, and Welsh history, [1950s]-1984; manuscripts, notes and typescripts for the published works Anzio, Madly in all directions, Shell Guide to Wales, Portrait of Gower, and Trust to talk, 1958-1980; travel journals, 1947-1964, recording visits to India, West Indies, Europe, Middle East, Africa and Hong Kong and Singapore; notebooks containing notes, drawings and miscellanea, [1947]-[1960s]; financial papers, 1945-1973; correspondence, 1936-1986; papers relating to wine, 1980-1984; papers relating to Dylan Thomas and his literary estate, 1955-1974; family papers, 1895-1950; press cuttings relating to his broadcasting career, 1937-1978; papers relating to Botticelli's painting, 'Primavera', 1945-1988; and miscellaneous papers, mainly printed, 1850-1974.

Rev. William Griffiths's journals, 1816-1855; printed diaries, 1837, 1843-1845, 1850-1851; a 'day book' or diary, 1854-1861, with additional entries at the end by his son; a notebook of autobiographical data upon which his book Gower memories of William Griffiths (Aberaeron, 1957) is based; personal letters, 1825-1849; miscellaneous letters, 1840-1860; printed copies of reports and notices of general meetings of the Glamorgan Banking Co., 1845-1858; sermon notes, 1817-1861; notebooks relating to subscriptions for Bethesda Church, Gower, 1838-1843; translation of Robert Jones, Drych yr Amseroedd; letters, 1851-1882, addressed mainly to William Griffiths [junior] at Aberaeron, and an account book, 1849-1855, relating to his business at Aberaeron; and correspondence of Miss A. G. Jones relating to the Rev. William Griffiths, 1948.

Papers of J. Mansel Thomas, Swansea, 1912-1979, with over a hundred typescript copies of plays, sketches, radio scripts and short stories. In a few cases the files contain manuscript drafts, and correspondence from the BBC and various publishers. There are notebooks containing ideas for plays and short stories, research notes used in preparing lectures, and also correspondence and papers relating to the history of Gower.