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Autograph letters from a large number of people to Thomas and others, mainly relating to archaeology, Welsh history, literature and ecclesiastical affairs. The correspondents include B. Beedham, William Buckland, W. Boyd Dawkins, Walter Davies ('Gwallter Mechain'), J. P. Earwaker, D. Silvan Evans, R. W. Eyton, E. A. Freeman, Margaret Gatty, Reginald Heber, Felicia Hemans, H. Longueville Jones, John Keble, Sir Theodore Martin, Sydney (Lady) Morgan, Lord Mostyn, Samuel Rogers, W. F. Skene, Sir Arthur Sullivan, John Williams ('Ab Ithel'), Morris Williams ('Nicander') and Robert Williams (Rhydycroesau); an English poem entitled 'The Sixth Centenary of Dante's Beatrice 1890' by T. Tudno Jones; and a number of 'cut-out' autographs.

Seventeen letters, 1859-79, to D. Silvan Evans from the Reverend Robert Williams (1810-81), sixteen of which are written from Rhydycroesau (rectory), Oswestry and one from Culmington Rectory, Bromfield (the writer's Cornish dictionary, advice, words and their meanings, re translations for Mr Skene, 'these English Bishops', the 'Celtic Remains', the 'Greal', etc., the death of Henry Parry, r[ector] of Bylchau (mention of his father's library), interest in the addressee's preferment, he has been making a catalogue of the books in St Asaph cathedral library, reference to the death of Professor Evander Evans and Professor Ebel, the slowness of so many of his subscribers to pay, the writer's health, sympathy, his removal to Culmington).

Extensive material relating to Welsh bibliography accumulated by, and mainly in the hand of, D. Silvan Evans. It includes a volume entitled 'Bibliotheca Cambrensis. Llyfrofyddiaeth Cymru' ('A[u]ctore Dan. Silvano Evans, Cereticense') (pasted on to the inside lower cover is a holograph letter from the Reverend David Williams, Llanedy Rectory, 1868, giving the entry of baptism of John, son of John Walter, cleric and lexicographer, on 22 August 1721); a home-made notebook entitled 'Llyvryddiaeth Gymreig' (pasted on to the inside lower cover is a note in the hand of Benjamin Williams, ('Gwynionydd')); another home-made notebook entitled 'Emynau detholedig at Wasanaeth yr Eglwys. Rhag. 29, 1862', being a bibliography of Welsh hymnals and relevant source material; copious unbound leaves containing book titles (one of the titles is written on the dorse of a letter from M. A. Lewis, Tredegar Post Office, 1868, requesting the return of the writer's copy of 'Dr. J. D. Rees's Old Grammar'); and letters from John Peter ('Ioan Pedr'), Bala to [Henri] Gaidoz, 1870 (publications not contained in Rowland's work [Llyfryddiaeth y Cymry]), to D. Silvan Evans from W[illia]m Price, Llanffwyst, Abergavenny, 1869 (an addition to Llyfryddiaeth y Cymry), [Robert John Pryse] 'Gweirydd ap Rhys', Bangor, [18]78 (the title of Llyfer Plygain, 1618, transcribed by the writer from a volume examined at the Pengwern [Mostyn] sale in 1874), W[illiam] Rowlands ('Gwilym Lleyn'), Machynlleth, 1862-4 (4) (additions and corrections to [Llyfryddiaeth y Cymru], with references to Evan Evans ('Ieuan Brydydd Hir'), to [Jane] Davies, Penmaen, to W. F. Skene, etc., a request by a local printer to be allowed to print the recipient's edition of the works of [Walter Davies] Gwallter Mechain', the writer's removal from the manse to another house in Machynlleth and subsequently to Oswestry, the reported cataloguing of 'Llyfrfa Coleg Dewi' [the library of St. David's College, Lampeter], the illness and voyage to Australia of the writer's son), and from W[illiam] Spurrell, Carmarthen to [William] Rowlands ('Gwilym Lleyn') at Brynmawr, 1851-2 (2) (the writer's copy of Sion Dafydd Rhys's Welsh Grammar, biography of John Daniel, printer of Carmarthen). Some of the unbound titles are in the hand of Richard Williams (1835-1906), Celynog, Newtown and there is some later and additional material in the hand of J. H. Davies.