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Papers of David Thomas Guy, 1912-1975, including papers relating to the Workers' Educational Association, 1920-1973, in particular of the South Wales District; minute book of Cardiff Printers Ltd, 1946-1973; papers relating to the University of Wales, 1973-1975, and Coleg Harlech, 1971-1975; papers of the Welsh Advisory Committee of the British Council, 1971-1973; appointment diaries, 1939-1973; and bibliographical notes, press cuttings, photographs and personal memorabilia, 1948-1970.

Administrative records of the University of Wales from its establishment in 1893 comprising papers relating to the foundation of the University; records of the University Court, Guild of Graduates, the Senate, Academic Board, University Council, Board of Celtic Studies, University of Wales Press Board, The Committee of Principals, Registrar's papers; records of committees, sub-committees and ad hoc committees created by, or answerable to, the Court, the Council, the Academic Board, etc., and printed materials. The archive is a fundamental source for the history of the University and for University education in Wales; to the development and provision of bilingual education in higher education in Wales, and, to a lesser extent to education in general in twentieth-century Wales.

Papers relating to the University of Wales comprising correspondence, minutes of meetings of the Council and the University Extension board, reports of extra-mural and tutorial classes, etc.