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Notebooks, 1920-1923, copy of thesis entitled 'Daearyddiaeth Hanesyddol ac Economig Cymru'; drafts of published works, including Saints, seaways and settlements in the Celtic lands (1969), Dewi Sant. Nawdd Sant Cymru / Saint David. Patron Saint of Wales (1983) and 'Distribution of the Crown Livings in England and Wales . . . 1539' (?unpublished); lecture notes when he was Gregynog Professor of Geography and Anthropology at UCW, Aberystwyth, 1947-1968; papers relating to United Theological College, 1976-1983; papers relating to the University of Wales, Aberystwyth, 1978-1983; correspondence addressed to him, 1925-1982; maps, diagrams and posters prepared by him [20th century]; and miscellaneous papers, 1924-1981.

Personal papers of Elwyn Davies, Margaret Davies and Ben Davies, 1878-1986; academic research notes, theses and publications concerning historic stock farming and field systems, [post-1902]-1985; papers relating to the University of Wales, 1937-1982, the Milford Haven Conservance Board, 1958-1982, the national parks, 1960-1983, the Countryside Commission, 1967-1982, and papers relating to the University of Wales, Aberystwyth, the National Library of Wales and the National Museum of Wales, 1962-1985; printed matter, 1937-1986; and papers relating to Alun Davies and the Historical Association, 1965-1977.

Papers of Merfyn Jones relating to the Liberal Party, 1964-1989, comprising papers and correspondence of the National Liberal Association, 1964-1988; papers, correspondence and minutes relating to the Welsh Liberal Party, 1965-1987, and on subjects including policy, 1969-1986, devolution, 1976-1979, and European Elections, 1977-1984; correspondence and minutes relating to Ceredigion and Ceredigion and Pembroke North Liberal Associations, 1966-1988, and papers relating to general and local elections, 1973-1987; papers relating to Aberystwyth Liberal Association, 1968-1988, to University College of Wales, Aberystwyth, 1977-1989, and to the Association of University Teachers, 1979-1988; newspaper cuttings, 1964-1988; personal papers of Merfyn Jones and correspondence with Liberal politicians, 1965-1988; printed material, [1968]-1987; papers relating to Young Liberals at national and local levels, 1966-1976; papers relating to the Social and Liberal Democrats, 1984-1988.