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Manuscripts of William Thomas (Islwyn, 1832-1878), Calvinistic Methodist minister, poet and hymnwriter.

Papers of Ithel Davies, 1884-1983, relating mainly to his imprisonment as a conscientious objector, 1916-1919; and personal papers, 1884-1983, including poetry and prose.

Deeds, 1583-1772, relating to properties in the parishes of Llangynfelyn and Llanfihangel Genau'r-glyn, and in Trefeurig, parish of Llanbadarn Fawr, Cardiganshire.

Papers accumulated by Ivan Monckton relating to his trade union activities in Wales, including papers of the Agricultural and Allied Workers National Trade Group Committee, 1918-1990; correspondence relating to the General Executive Committee of the TGWU and AAW, 1988-1989; correspondence relating to cruel sports, 1984-1993; correspondence and other papers relating to his work with the Forestry Commission, including union activities, 1983-1990; and reports, minutes and other documents relating to the Labour Party and the Health and Safety Executive Subcommittee, 1984-1992.

Papers of, or accumulated by, Ivor James in the course of his studies of the history of Wales during the late sixteenth and the seventeenth centuries.

Papers of the Rev. Ivor T. Rees, comprising mainly printed political material, 1928-1997, including election literature and candidates' addresses for British elections from Wales, England, Scotland and Northern Ireland and election literature, newsletters and press cuttings relating to minority parties such as the Socialist Party of Great Britain, 1951-1970; National Democratic Party/National Front/British National Party, [c. 1970's]-[1990's], and papers relating to Lt Commander W. G. Boaks, who stood as an independent candidate in many elections between 1951 and 1982, [c. 1970s-1980s]; articles and obituaries relating to politicians and other prominent individuals, [c. 1970s-1990s]; index cards containing details of British Parliamentary candidates who stood in British Parliamentary elections, 1910-1983; together with miscellaneous papers, 1948-1985; newspaper cuttings, 1931-1999 relating to Welsh politics, including the first election for the National Assembly for Wales and electoral candidates in Wales; and election leaflets mostly for the county council elections, 6 May 1999, in Swansea, Sketty, Anglesey, Vale of Glamorgan and Rhonda Cynon Taf.
Additional donations also include papers, 1999-2017, consisting mainly of printed material from web pages, press cuttings, and campaign material and election addresses relating to prominent Welsh politicians both in the Welsh Assembly and UK Parliament; papers, 1885-2018, relating to elections held in Wales and Welsh constituencies from the 19th to the 21st centuries and politicians who have stood as candidates, including in UK Parliamentary elections, Welsh Assembly elections, and European Parliament Elections; a large number of candidates' and politicians' biographies (1885-2018), and questionnaires for candidates standing in various 20th- and 21st- century elections (1997-2017; 2019); and a large number of papers including press cuttings and printed material from web pages relating to UK Parliamentary, Welsh Assembly, and European Parliament elections (1892-2018), including campaign material and election addresses relating to candidates standing in Welsh constituencies; and some typescript copies of Ivor T. Rees' works.

Manuscripts of the Reverend J. C. Jones, including material of Montgomeryshire and Caernarvonshire Congregationalist interest and autograph sermons.

Papers donated in 1933 by J. C. Owen, 1859-1921, dealing with tithes, rates, rent-charges, other parish accounts and miscellaneous ecclesiastical matters in various parishes in Cardiganshire and Brecknockshire with which the donor was connected. A second donation made in 1936 (listed elsewhere) comprises papers relating to J. C. Owen's ordination, 1883; a letter and other papers concerning the church and parish of Llanafan Fawr [1910]-1911; a copy of Y Dyddiadur Methodistaidd, 1864, with manuscript entries of preaching and other engagements, disbursements, etc.; miscellaneous papers including a list of vicars of Llanafan Fawr, 1486-1883; and items relating to the work of J. C. Owen.

Minute books relating to various Cambridge University societies, Llanelli Committee of Social Service for the Unemployed, Llanelli Park Lodge, Borough Road Chapel, London, etc., 1870-1933; undergraduate notes on history, English literature, Latin, and psychology, and miscellaneous papers relating to history and politics including 'Baronial opposition to Edward II', 1918; papers relating to Monmouthshire archives, 1937-1955; 'The Welsh assize roll 1277-1284: assize roll no. 1147', 1940; reports and preliminary reports, notes etc., on archives acquired by or to be acquired by NLW, 1941-1945; notes, drafts, proofs etc., of articles for the National Library of Wales Journal and items relating to archives in NLW, 1944; papers relating to the Committee on Welsh Calendar Customs, 1944-1947; papers relating to his post as lecturer in palaeography and diplomatic in the University of Cambridge, 1945-1947, and as reader in the same in the University of Durham, 1948-1962, including lectures notes; reports and notes on Welsh Church Commission documents to be deposited in NLW and items on Welsh church history, 1944-1963; episcopal and chapter records of the Welsh dioceses, including notes, drafts and proofs for 'Episcopal acts... Welsh dioceses 1066-1272' (2 vols, 1946 and 1948), and vol. III (Bangor and St Asaph) which was never published; papers as honorary editor of the Journal of the Historical Society of the Church in Wales, 1946-1952; papers relating to Giraldus Cambrensis; notes, photostats, transcripts and typescript of 'Professions of obedience to Canterbury c. 793-1420', proposed to be published by the Camden Society, 1947; miscellaneous papers on history and archives; 'Welsh and Marcher cases coram rege 1272-1307'; papers relating to indexing records at PRO, including transcripts and extracts from documents; notes for reports on the Exchequer records in the PRO; summaries and extracts from Assize Rolls; papers used in the preparation of 'Records of the court of augmentations relating to Wales and Monmouthshire', 1954, and 'The cartae antiquae rolls 11-20', 1960, and the unpublished 'Cartae antiquae rolls 21-30'; typescript and proof articles for 'Studies presented to Sir Hilary Jenkinson', 1957, together with correspondence between contributors and printers; papers relating to the Severn fisheries dispute and the seignory of Gower, 1957-1962; papers used in cataloguing the records of Guernsey, 1959-1969, and in the preparation of 'Catalogue of manuscripts in the library of the honourable society of the Inner Temple', 1972; miscellaneous papers relating to the history of Wales, 1908-1945; film script entitled 'The Black Prince'; diaries, 1946-1971; curricula vitae and papers relating to his personal life and career together with political articles by Prof. Curt Wachtel; photocopies of documents, personal photographs, plaster casts of seals etc.; papers received from Canon E. T. Davies, 1853-1940; uncatalogued correspondence bundles arranged by year, 1909-1971. Copies of his Welsh revolts of Edward II (Llanelli, 1912) and Medieval Northumberland (Llanelli, 1918), journals and offprints; documents relating to the manor of Swavesey, Cambridgeshire, 1623-1833; documents relating to Monmouthshire, 1616-late 19th century; miscellaneous documents relating to England and Wales, 1458-1848; papers and correspondence of Nathan Laski (1863-1941), Harold J. Laski, Professor of Political Science, University of London (1893-1950), Neville J. Laski, Q.C. (1890-1969), John L. Paton, High Master of Manchester Grammar School (1863-1946), Thomas F. Tout, Professor of History, Manchester University (1855-1929), and others including an autographed album.

A collection of holograph manuscripts of musical compositions by Joseph David Jones (1827-1870).

The 1939 deposit consists of deeds and documents, 1549-1887, relating to properties in Montgomeryshire, Merionethshire, Breconshire and Shropshire. The 1973 deposit mainly contains deeds and documents, 1564-1932, relating to properties in Montgomeryshire, many relating to the Lloyd family of Montgomery. The 1979 deposit comprises materials gathered by J. D. K. Lloyd for a History of Montgomery; a bundle of deeds and documents, [19 cent.]-[20 cent.], relating to the family of Lloyd of Plas Trefaldwyn, Montgomery, and Castell Forwyn, Abermule; photographic albums, 1898-1978, comprising mainly family photographs; a collection of over 1000 postcards and photographs of historic buildings throughout Europe; and seven manuscript maps of land in Montgomeryshire, 1772-1858.

Records of J. D. Lloyd and Sons, Aeron Monumental Works, 1877-1947, consisting mainly of day books, 1877-1946; ledgers, 1898-1947; records of raw material costs, 1921-1928; account book, 1934; and loose receipts, 1922-1936.

Papers, [1897x1927], from the library of John Dyer Richards. They include autograph poetry by Richards, many of which was written for competition at eisteddfodau; autograph sermon notes; material relating to Ellis Humphrey Evans ('Hedd Wyn') comprising transcripts by Richards of letters and poetry, 1917, by 'Hedd Wyn' and an essay and biographical notes on 'Hedd Wyn'; together with an autograph letter, 1917, from R. Williams Parry.

Papers, 1927-1952, of the Rev. J. Dyfnallt Owen relating to the imprisonment of Breton nationalists and the alleged suppression of Breton language and culture by the French state following the Second World War, consisting of correspondence, written accounts of the treatment of individual nationalists, papers relating to the visit of the Welsh delegation to Brittany in 1947, a typescript draft of Yann Fouéré, Breton Nationalism (Cardiff, [1946]), and other general papers.

Manuscripts of, or collected by, John Edwards Griffith, [c. 1715]-1929, including pedigrees, memoranda and genealogical notes relating mainly to Anglesey and Caernarvonshire; a volume of pedigrees by John Ellis, Tai Croesion, 1723; manuscripts of William Williams, Llandygái; and some 350 letters, [c. 1892]-1929, to J. E. Griffith relating to botany and genealogy and to his publications.

The fonds contains the business and personal papers of J. E. Powell.

Deeds of the Myfod family of Tremeirchion, Flintshire, 1657-1727, and of their successors by marriage, the Jones family of Ffynnon Feuno, Tremeirchion, 1746-1781, and the sale of Ffynnon Feuno to Thomas Pennant of Downing, 1784. Deeds relating to New Inn and Tanybryn, 1793-1796, Tynyrafon in Tremeirchion, 1810-1821, and properties, including Gadlys, in the parish of Holywell, 1813-1873.

Papers of J. Glyn Davies, mainly letters, many relating to antiquarian, academic and library interests, including 400 from Robert Scourfield Mills ('Owen Rhoscomyl'), 1903-1919, almost 200 from Jennie Thomas relating to Llyfr mawr y plant, 1920-1950, and 150 from T. Gwynn Jones, 1908-1947; papers of his family, including the Tanycastell Collection, 1821-1858; and manuscripts collected by him, including the Henblas manuscript (Welsh poems by various authors, 1664-1685) and the Gwallter Mechain manuscripts.

Papers of J. Glyn Picton, 1949-1991, mainly papers concerned with his researches into General Sir Thomas Picton (1758-1815) and the Picton family, 1951-1991, including correspondence, 1949-1977; notes, 1951-1975; copies and transcripts of probate record and Pembrokeshire plea rolls; photographs and news cuttings, 1975-1984; and copies of printed sources; with also records, articles and lectures reflecting J. Glyn Picton's public service in the fields of national health and industrial relations, 1951-1977.