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One of eleven volumes containing sermons, addresses, notes, etc., 1834-1886, mainly by David Davies of Penmachno, afterwards of Barmouth.

A sermon on Habakkuk ii, 4 written in 1791 by Dafydd Ellis [David Ellis (1736-1795)], Criccieth, a well-known transcriber of manuscripts.

A collection comprising Cribyn Unitarian Church register with records dating from 1826 to 1899, and including church accounts, 1851-1852, and a brief history of the church and a list of ministers, 1790-1877; together with papers of the Rev. John Islan Jones, Cribyn, Unitarian minister, which include letters, 1915-1918, whilst Jones was on active service, and a journal containing an account of tours taken by Jones, 1915-1916.

Papers of the Rev David Evans, [1851]-1993, comprising papers relating to Cribyn Unitarian Chapel, Cardiganshire, including notebooks and volumes containing various chapel accounts, 1851-1927; papers relating to Cribyn Day school, 1888-1942, including account books, 1888-1909, one of which contains the Cwmiago household and farming accounts, 1904-42, and class attendance registers, 1890-1905; volumes of David Evans' sermon notes, [1893x1946]; addresses, [1880x1950]; plays, [1880x1950]; poetry [not written by David Evans], [1880x1950]; prose works, [1880x1950]; religious material, [1880x1950]; miscellaneous papers, [1880x1993], including recollections of Rev. David Evans by his great-great niece Gwenlyn E. Thornton; and printed material, 1865-1950.

Papers of David Evans, 1894-1942, mostly relating to his biographical work on Viscount Rhondda, including source materials, 1894-1918; together with source material relating to Sir David Richard Llewellyn, [1879x1951]; papers relating to the work of the Committee on Commercial and Industrial Policy, 1916; administrative records relating to the South Wales Journal of Commerce, 1926-1935; and miscellaneous material, 1917-1942.

Papers of the composer and musician Prof. David Evans, [c. 1896]-[c. 1934], comprising full and fragment scores of choral music, including orchestral and vocal scores, cantatas, anthems, hymn tunes, carols and other sacred music, arrangements of welsh airs, miscellaneous compositions, compositions by other composers, together with miscellaneous material.

Newsletters, programmes, publicity material and ephemera connected with Welsh societies in America, 1939-1985; in Canada, 1968-1985; miscellaneous North American Welsh societies, 1970-1985, including the Welsh National Gymanfa Ganu Association, 1970-1985; Women's Welsh Club of America, 1977-1984; Welsh Associated Youth of America and Canada, 1982-1985; Cymdeithas Madog, 1980-1985; and National Welsh-American Foundation, 1982-1984.
Further papers donated in 2005.

The music manuscripts of the composer David Harries, 1952-1995, comprising mainly drafts and scores of chamber and instrumental music, orchestral music, choral and organ, and voice and piano arrangements.
A second donation made in August 2021 contains further music manuscripts of David Harries, 1953-1993, and includes works by Harries' contemporary William Mathias (1934-1992) in addition to Harries' own compositions of chamber and instrumental music, orchestral music, choral and organ, and voice and piano arrangements.

Account books, 1864-1932, of Richard Watkins, Trecastle, Breconshire, and an account book and manuscript roll, 1867-1923, relating to Trecastle Calvinistic Methodist church, of which the Reverend David Henry Williams, son-in-law of Richard Watkins, was minister from 1912 to 1933.

The collection comprises business records of David Hughes & Sons, Aberdyfi, namely ledgers, 1878-1946, day books, 1888-1913, account books of receipts, 1870-1905, a bank account book, 1937-1943, and a file of bills and invoices, 1927. There is also a notebook containing minutes and other records of the Sunday school of Tabernacl C.M. church Aberdyfi, 1892-1893, and a notebook containing brief details relating to the Aberdyfi Burial Board, 1909.

Manuscript oratorios, operas, orchestral pieces, choruses, melodies and other musical compositions (including the four Welsh Airs arranged for choir and full orchestra premiered at the Crystal Palace, 1896); an autographed notebook containing solfa versions of Welsh melodies arranged for male voices, 1915; correspondence, 1934-1935, relating to the proposed publication of a memorial volume to Jenkins by nine of his contemporaries ('Er Cof am yr Athro David Jenkins Gan Naw o'i Gyfoedion'); music exercise books, 1877-1881, and a volume containing blacksmith's accounts, Trecastell, and particulars of payments to preachers, 1796-1810.

'A Collection of Materials to assist in writing a History of Glamorganshire. Copied from old Manuscripts, and Compiled from other Sources, by David Jenkin Senr. Swanea 1839'.

'Ychydig o Hanes Morganwg, allan o Lyfr Ysgrifen y diweddar Barchedig Edward Gamage, Offeiriad Sant Athan, yn awr ymherchenogaeth Mr. John Spencer, o'r un Plwyf', with other Glamorgan material, including 'Cambrian Pedigrees, Together with An Account of the Different Manors within the County of Glamorgan and the names of the Proprietors thereof', etc.

'The Glamorganshire Pedigrees copied from old Manuscripts, and compiled from various other Sources, by David Jenkin, Swansea, August, 1838'.

Two account books, 1959-61 and 1968-72, of David John George (1885-1972) of Scleddau Park, Fishguard, co Pembroke (see Annual Report 1972-73, p 38).

An autograph letter, 1955, from David Jones, artist and writer, enclosing proof corrections to his article 'History and pre-history' to be published in the literary magazine Dock Leaves.

Literary manuscripts of David Jones, with manuscript drafts of In Parenthesis: Seinnyessit e gledyf ym penn mameu; The Anathemata: Fragments of an attempted writing; Epoch and Artist: Selected writings by David Jones; The Sleeping Lord and other fragments; The Dying Gaul and other writings, and The Roman Quarry and other sequences. There is a substantial body of letters to David Jones from friends, editors and others, 1910-1976; draft letters from David Jones to friends, newspaper editors and others, 1929-1982; and letters by David Jones, 1919-1985, published in Dai Greatcoat: A self-portrait of David Jones in his letters. There are some examples of David Jones' art, and material relating to David Jones as an artist, as well as personal documents, financial papers, family papers, photographs, and accumulated research material.

'Carolau', 'cerddi', 'englynion', etc. composed c. 1767-1783 by David Jones ('Dafydd Sion Siams'), bookbinder, Penrhyndeudraeth, and in his autograph. On pp. 110-11 is 'Hymn a Gyfansoddwyd gan ... Evan Hughes ffeiriad llanfihangel [y Traethau]'.

Poetry by David Jones, alias David John James (Dafydd ab Ioan or Dafydd Deudraeth), mostly awdlau for eisteddfodau.