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Gohebiaeth, barddoniaeth, rhyddiaith a phapurau teuluol, yn ymwneud â J. W. Jones, 1878-1954, a'i dad, 'Glan Barlwyd', 1866-1917; deunydd a gasglwyd gan J. W. Jones yn ymnweud ag unigolion a sefydliadau yn ardal Blaenau Ffestiniog, gan gynnwys gohebiaeth, barddoniaeth a phapurau eraill o eiddo 'Gwilym Deudraeth', 1917-1939, 'Elfyn', 1874-1917, Y Parch. R. R. Morris, 1883-1933, 'Alafon', 1875-1915, 'Llifon', 1899-1916, 'Isallt', 1887-1913, a 'Glyn Myfyr', 1893-1937; llythyrau at John Daniel Davies yn rhinwedd ei swydd fel golygydd Y Rhedegydd, 1930-1942; barddoniaeth a phapurau eraill o eiddo T. Gwynn Jones, 1910-1944; barddoniaeth, [1840]-1940, gan amryw feirdd, yn cynnwys Hedd Wyn ac R. Williams Parry; deunydd rhyddiaith amrywiol, peth ohono wedi'i gyhoeddi yn Y Drysorfa ac yn Y Rhedegydd, 1879-1954; llawysgrifau cerddorol, 1876-[c. 1934]; beirniadaethau eisteddfodol, 1870-1939; llyfrau lloffion yn cynnwys torion o'r wasg, [c. 1879]-1940; dyddiaduron, 1864-1935; cofnodion chwareli llechi Blaenau Ffestiniog, 1868-1951; amryw gyfrifon a llyfrau cyfrifon yn ymwneud â gwahanol fusnesau a sefydliadau, 1784-1932; cofnodion yn ymwneud ag eglwysi'r Methodistiaid Calfinaidd, 1840-1951, gan gynnwys rhai Bethel, Tanygrisiau, [1840x1945]; pregethau a nodiadau crefyddol,1846-1952; deunydd printiedig yn cynnwys effemera etholiadol, marwnadau, baledi, carolau ac emynau, 1820-1948; a gweithredoedd a dogfennau yn ymwneud â siroedd Caernarfon, Meirionnydd a Dinbych, 1759-1947. = Correspondence, poetry, prose and family papers, relating to J. W. Jones, 1878-1954, and to his father, 'Glan Barlwyd', 1866-1917; material collected by J. W. Jones relating to individuals and organizations in the Blaenau Ffestiniog area, including correspondence, poetry and other papers of 'Gwilym Deudraeth', 1917-1939, 'Elfyn', 1874-1917, Rev. R. R. Morris, 1883-1933, 'Alafon', 1875-1915, 'Llifon', 1899-1916, 'Isallt', 1887-1913, and 'Glyn Myfyr', 1893-1937; letters to John Daniel Davies as editor of Y Rhedegydd, 1930-1942; poetry and other papers of T. Gwynn Jones, 1910-1944; poetry, [1840]-1940, by various poets, including Hedd Wyn and R. Williams Parry; various prose material, some of which was published in Y Drysorfa and Y Rhedegydd, 1879-1954; musical manuscripts, 1876-[c. 1934]; eisteddfod adjudications, 1870-1939; scrapbooks containing press cuttings, [c. 1879]-1940; diaries, 1864-1935; records of Blaenau Ffestiniog slate quarries, 1868-1951; various accounts and account books relating to various trades and organisations, 1784-1932; records relating to Calvinistic Methodist churches, 1840-1951, including those of Bethel, Tanygrisiau, [1840x1945]; sermons and religious notes, 1846-1952; printed material including electoral ephemera, elegies, ballads, carols and hymns, 1820-1948; and deeds and documents relating to Caernarfonshire, Merionethshire and Denbighshire, 1759-1947.

Estate and family records of the Chirk Castle estate, mainly in Denbighshire, comprising deeds from 1284; manorial records, mainly of the lordship of Chirk and Chirkland, 1322-1853, including receiver's accounts, ministers' accounts, court rolls, etc.; records of the estate's involvement in the coal, iron and lead industries in Denbighshire from 17 cent.; Denbighshire Quarter Sessions records, including order books, 1647-1675, rolls, 1643-1699, and a book of indictments, 1670-1690; Denbighshire militia records, 1602-1797, and related local government records, 1602-1811; business papers of Sir Thomas Myddelton (1550-1631); personal and estate correspondence from c.1600; literary manuscripts, c.1630-1887; and parliamentary election papers for Denbighshire and Denbigh boroughs, 1681-1852, including papers relating to quo warranto proceedings against the mayor and burgeses of Holt, 1739-1743.

Ten designs for stained glass panels, with armorial pedigree of the Myddelton family attributed to A. W. N. Pugin and John Hardman Powell; three hundred and thirty-two volumes relating to the Chirk Castle estates; a collection of miscellaneous volumes and documents relating to the Chirk Castle estates, including an account book of the Nangwrud Slate Quarry, rentals books, account books, volumes relating to the Black Park Colliery, a rabbit account book, and other papers; and an indenture, 1812, relating to Bodlith, Llansilin, part of the Chirk Castle estate were acquired. These remain uncatalogued.

A manuscript account book for Sir Richard Myddelton's properties at Chirk Castle and Soho Square, London, 1686-1700 and 1748-1752.

A manuscript Steward's letter-book relating to Chirk Castle, 183501838.

Cofnodion Plaid Cymru, 1915-1999, yn cynnwys cofnodion, agenda and gohebiaeth y pwyllgor gwaith a phwyllgorau eraill, 1925-1997; gohebiaeth gyffredinol, 1925-1998, gyda nifer o aelodau a swyddogion blaenllaw y blaid; cofnodion, gohebiaeth a phapurau eraill y gwahanol bwyllgorau rhanbarthol, 1925-1997, a changhennau,1930-1992; cofnodion a dogfennaeth y Cyngor Cenedlaethol, 1967-1997; cofnodion ariannol, yn cynnwys rhai papur newydd misol y blaid Y Ddraig Goch a Welsh Nation a Chronfa Gŵyl Ddewi, 1927-1996; rhaglenni a threfniadau ar gyfer cynadleddau ac Ysgolion Haf, 1933-1998; cofnodion aelodaeth, 1930-1996; papurau y Grŵp Ymchwil, [c.1960]-1995; papurau, yn cynnwys areithiau ac effemera, yn ymwneud ag etholiadau, 1929-1999; papurau yn ymwneud ag Adran y Menywod, 1924-1996, a'r Mudiad Ieuenctid, 1964-1998; papurau yn ymwneud â refferendwm datganoli 1979,1969-1983, a refferendwm 1997, a Chynulliad Cymru,1992-1998; papurau yn ymwneud â Y Ddraig Goch, Welsh Nation a chyhoeddiadau eraill, 1932-1996; deunydd printiedig gan Blaid Cymru ac eraill yn cynnwys llyfrau, cyfnodolion a phamffledi,1913-1996; torion o'r wasg, 1924-1996; cylchlythyron, 1938-1992; papurau yn ymwneud â'r Blaid Seneddol,1980-1996; papurau unigolion ac rhai ar wahanol bynciau amrywiol, 1926-1998 = Records of Plaid Cymru, 1915-1999, including minutes, agendas and correspondence of the executive and other committees, 1925-1997; general correspondence, 1925-1998, with many prominent party members and officials; minutes, correspondence and other papers of the various regional committees, 1925-1997, and branches, 1930-1992; minutes and records of the National Council, 1967-1997; financial records, including those of the party's monthly newspaper Y Ddraig Goch and Welsh Nation and Cronfa Gwyl Dewi, 1927-1996; arrangements for and programmes of conferences and Summer Schools, 1933-1998; membership records, 1930-1996; papers of the Grŵp Ymchwil (research group), [c.1960]-1995; papers, including speeches and ephemera, relating to elections, 1929-1999; papers relating to the Adran Menywod (Women's Section), 1934-1996, and the Mudiad Ieuenctid (Youth Movement), 1964-1998; papers relating to the 1979 devolution referendum, 1969-1983, and the 1997 referendum and Welsh Assembly, 1992-1998; papers relating to Y Ddraig Goch, Welsh Nation and other publications, 1932-1996; printed matter by Plaid Cymru and others including books, periodicals and pamphlets, 1913-1996; press cuttings, 1924-1996; circulars, 1938-1992; papers relating to the Parliamentary Party, 1980-1996; papers of individuals and to various miscellaneous topics, 1926-1998.