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Papers of Arthur John Williams, 1881-1943, including political papers comprising letters, 1868-1911; papers relating to legal, electoral and land reforms, 1867-1911; papers relating to his parliamentary elections in Birkenhead and Glamorgan, 1880-1895; papers relating to South Glamorgan politics, 1886-1924; material concerning the National Liberal Club, 1883-1951; diaries, 1864-1911; diaries of Rose Harriette Thompson Crawshay 1868-1943; and family and financial papers, 1767-1943.

Clement Davies's papers, [c.1884]-1967, mainly Liberal Party papers, 1928-1962, Clement Davies's political career, 1929-1965, Welsh affairs, 1936-1962, peace movements, 1940-1962, foreign affairs, 1944-1962, constituency papers, 1951-1962, and home affairs, 1953-1963; and papers and correspondence of Jano Clement-Davies, 1873-1969, and papers of Stanley Clement-Davies, 1920-1963.

Personal and political papers of E. T. John, 1881-1931, including correspondence, 1886-1931; personal and family papers, 1882-1930; political papers, 1907-1930; papers relating to Welsh and Celtic cultural movements, 1912-1930; posters and programmes, 1881-1927; and miscellaneous papers and publications, [c. 1894]-1930.

The fonds comprises a substantial group of letters and papers, 1911-1972, acquired by Frances as private secretary to Lloyd George, including some business papers, notebooks of reminiscences and printed items. There are letters from a number of prominent politicians and public figures. There is also a small group of letters and papers, 1912-1965, concerning Lloyd George himself, papers, 1933-1946, relating to Jennifer Longford's schooldays, and a few papers relating to other members of the Stevenson family, notably Frances's sister Muriel and brother Paul. The material in sub-fonds G was loaned by Mrs Ruth Nixon of Camberwell to the National Library of Wales to be digitised in March 2013 and subsequently returned to her a few months later. Some of this material was subsequently purchased by NLW in 2017 and catalogued as sub-fonds H. The 2017 purchase includes various articles about Lloyd George, a draft memorandum partly in the hand of Lloyd George and partly in the hand of Frances Stevenson regarding the early part of the First World War, letters from Frances Stevenson to her family, including some from the Versailles Peace Conference, notes following Lloyd George's speeches and papers relating to Jennifer Longford including letters between her and Lloyd George.

Papers of Stuart Rendel and family members, including papers relating to the University College of Wales, Aberystwyth, and the proposal to establish the National Library of Wales and its development during the early years of its existence, 1883-1916; speeches, addresses and political papers relating to disestablishment of the church in Wales and the 1889 Intermediate Education Act, 1882-1909; press cuttings, 1881-1913; photographs, 1892; miscellaneous letters, 1878-1912; letters to Stuart Rendel, 1853-1912, including letters from A. C. Humphreys Owen, 1877-1905, family letters, 1853-1902, and letters from prominent political figures and Welsh public figures; letters and copies of letters from Rendel, 1880-1912; diaries, mainly recording details of Stuart Rendel's business activities, 1863-1869; notes of conversations with W. E. Gladstone, John Morley and H. H. Asquith, 1888-1910; papers relating to Chinese affairs and French and Chinese peace talks, 1884-1886; papers of James Meadows Rendel, including letters, 1828-1856, and papers relating to his estate, 1856-1859; letters of Catherine Jane Rendel, 1845-1855; letters and papers of George Wightwick Rendel, 1871-1902; papers relating to Rendel's other brothers, 1841-1889, and his daughters, 1882-1910; letters and papers of Harry Stuart Goodhart-Rendel, 1898-1959, and other papers concerning him, 1963-1977; papers, mainly letters, of the Goodhart family, 1819-1957; papers of Miss Rosemary Rendel, 1986-1996; papers of Sir George William Rendel, including: Foreign Office papers, 1917-1967, correspondence, 1912-1973, papers relating to the Catholic Union of Great Britain, 1942-1979, lectures, diaries and notes, 1915-1954, personal and family papers, 1908-1980, and material relating to the book The Sword and the Olive (1957), 1954-1986.