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The catalogued portion of the archive contains records of the family of Owen, later Humphreys-Owen, of Glansevern, and Johnes of Garthmyl, mainly comprising title deeds and documents, [late 12 cent.]-1929, mainly relating to property in Montgomeryshire; estate papers, 1767-1924, including rentals, accounts and surveys; records relating to Campobello island, New Brunswick, Canada, 1767-1902; substantial family correspondence, 1633-1926, political correspondence of Arthur Charles Humphreys-Owen, 1856-1905, including letters from Lord Rendel; naval papers of Captain William Owen, 1746-1778, [c. 1797]. The uncatalogued part of the archive includes correspondence of the Owen and Humphreys-Owen families, 1754-1905; pedigree of the Owen family, 1839; and material relating to S. P. F. Humphreys Owen, [c. mid 20 cent].

Papers of Stuart Rendel and family members, including papers relating to the University College of Wales, Aberystwyth, and the proposal to establish the National Library of Wales and its development during the early years of its existence, 1883-1916; speeches, addresses and political papers relating to disestablishment of the church in Wales and the 1889 Intermediate Education Act, 1882-1909; press cuttings, 1881-1913; photographs, 1892; miscellaneous letters, 1878-1912; letters to Stuart Rendel, 1853-1912, including letters from A. C. Humphreys Owen, 1877-1905, family letters, 1853-1902, and letters from prominent political figures and Welsh public figures; letters and copies of letters from Rendel, 1880-1912; diaries, mainly recording details of Stuart Rendel's business activities, 1863-1869; notes of conversations with W. E. Gladstone, John Morley and H. H. Asquith, 1888-1910; papers relating to Chinese affairs and French and Chinese peace talks, 1884-1886; papers of James Meadows Rendel, including letters, 1828-1856, and papers relating to his estate, 1856-1859; letters of Catherine Jane Rendel, 1845-1855; letters and papers of George Wightwick Rendel, 1871-1902; papers relating to Rendel's other brothers, 1841-1889, and his daughters, 1882-1910; letters and papers of Harry Stuart Goodhart-Rendel, 1898-1959, and other papers concerning him, 1963-1977; papers, mainly letters, of the Goodhart family, 1819-1957; papers of Miss Rosemary Rendel, 1986-1996; papers of Sir George William Rendel, including: Foreign Office papers, 1917-1967, correspondence, 1912-1973, papers relating to the Catholic Union of Great Britain, 1942-1979, lectures, diaries and notes, 1915-1954, personal and family papers, 1908-1980, and material relating to the book The Sword and the Olive (1957), 1954-1986.