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Letters, 1835-1840, from David Owen ('Dewi Wyn o Eifion') to Richard Humphreys (Faerdref) , Ellis Owen and James Spooner (Tremadog), together with drafts of letters by David Owen relating to Welsh literary matters.

Nearly two hundred autograph letters, 1855-1891, relating mainly to Welsh literary matters, and especially to Glamorgan, 1855-1899, to Jonathan Reynolds ('Nathan Dyfed') from contemporary Welsh poets and authors; miscellaneous poems; printed broadsides; press cuttings; etc.

Autograph letters from a large number of people to Thomas and others, mainly relating to archaeology, Welsh history, literature and ecclesiastical affairs. The correspondents include B. Beedham, William Buckland, W. Boyd Dawkins, Walter Davies ('Gwallter Mechain'), J. P. Earwaker, D. Silvan Evans, R. W. Eyton, E. A. Freeman, Margaret Gatty, Reginald Heber, Felicia Hemans, H. Longueville Jones, John Keble, Sir Theodore Martin, Sydney (Lady) Morgan, Lord Mostyn, Samuel Rogers, W. F. Skene, Sir Arthur Sullivan, John Williams ('Ab Ithel'), Morris Williams ('Nicander') and Robert Williams (Rhydycroesau); an English poem entitled 'The Sixth Centenary of Dante's Beatrice 1890' by T. Tudno Jones; and a number of 'cut-out' autographs.

A letter, 1855, from John Williams ('Ab Ithel') to [Evan Davies ('Myfyr Morganwg')].

A manuscript containing a transcript of a lecture on The Influence of the Literature of Wales on that of other countries, given by Teilo at Llandilo, 16 March 1864; a note on Thomas Jones (Twm Sion Catti); material relating to the late Rev. John Evans, Llwynffortun, 1865.

Drafts and notes in the hand of Taliesin Williams for the volume Iolo Manuscripts, A Selection of Ancient Welsh Manuscripts, in prose and verse, from the collection made by the late Edward Williams, Iolo Morganwg,… with English translations and notes by his son, the late Taliesin Williams (Ab Iolo) of Merthyr Tydfil (Liverpool: Welsh MSS Society, 1848).
Included are manuscript drafts of the Welsh texts on pp. 3-328 passim (T4/1), drafts of the English translations on pp. 341-496 passim (T4/2), drafts for the footnotes on pp. 332-489 passim (T4/3), a draft of pp. 331-507 passim combining text and footnotes (T4/4), and notebooks containing notes and memoranda relating to the volume (T4/5-11). Also included is a bundle of draft texts, relating mostly to Welsh saints in a format similar to T4/1 but which were either omitted from the volume or intended for another book on Bonedd y Saint (T4/12).

An account of the early history of Wales and notes on Welsh place-names, literature, etc.

Some three hundred and fifty letters, 1945-1969, from Gilbert Turner to John Cowper Powys and Phyllis Playter, which include references to the novelist Elena Puw Morgan, Welsh language and literature, visits to North Wales, the writer's procurement of library books for the recipients and the preparation of typescript copies of Powys's Dostoievsky (1947) and Rabelais (1948). Turner continued corresponding with Phyllis Playter after John Cowper Powys's death in 1963.

Articles and addresses by David Samuel mainly on Welsh literature, history and education, 1890-1909, and an account of his tour in the United States of America, 1889.

Press cuttings relating to Wales and Welsh culture, such as religion, politics, literature, music, education, St. David's Day celebrations and the Eisteddfod Genedlaethol, individuals, and the National Library of Wales [1895]-[1939].

Addresses by Meredith J. Hughes on 'Myth and legend in the literature of Wales', 1914, and 'Democratic Theory and Institutions', 1919; a hymn 'Ymwel a mi o Arglwydd da', and a poem entitled 'Afon Alun', 1924.

A Latin vocabulary, notes for the study of the Mabinogion, extracts from printed sources, notes on 'Y Gogynfeirdd' and their vocabulary, etc.