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The archive comprises election ephemera, including election addresses, posters, drafts of election material, mostly for Plaid Cymru candidates for UK Parliament and local elections, along with some ephemera related to anti-nuclear weapons and anti-nuclear power campaigns and Plaid Cymru publications.

Deeds and documents, 1728-1988, relating to the Trewern Hall estate, including the Plough and Harrow Inn. They include documents relating to proposed improvements to cottages, 1937-1938, and the restoration of Trewern Hall, 1983-1988; farm and household accounts, with miscellaneous financial papers and vouchers, 1952-1986; correspondence and papers concerning agricultural improvements and grant applications, 1977-1985; correspondence concerning the tenancy of Plas Newydd, Trewern, 1982-1984; personal and family papers, 1949-1984, relating to William Herbert Chapman (1955-1982) and to Murray Lloyd Chapman, including the latter's research notes and papers, on the history of Trewern and Montgomeryshire families and his work in civil engineering, 1973-1986. Plans of the estate and proposed improvements to the farm buildings accompanied some of the papers. Papers relating to Phase 2 Restoration of Trewern Hall, 1990-1993; were received in 2007, including a diary of events in two volumes; papers relating to Ivor William Lloyd Chapman and Margaret Eleanor Chapman; and Gregory-Allen papers. Four further collections were received in August 2014, 2017, September 2018 and September 2019. The 2014 group remains uncatalogued.

Student notes on petrology, 1903; university lectures and notes for lectures given at Aberystwyth and Manchester, 1919-[1930], and at Cambridge, 1931-1938; other lectures and addresses on geological subjects, 1925-1939; material relating to academic and consultative research, undertaken mainy in Wales, 1884-[1942], including material relating to the mineral mining industries and river drainage in Mid Wales; files of personal papers and correspondence, 1913-1943; copies of letters to his wife, 1909-1966; pocket notebooks, [1920s]-[1930s]; theses and papers by other individuals, 1931-1943; photographs and slides, [c. 1903]-[1949]; portfolios containing plans, sections, maps and graphs relating to mines, collieries and power stations in Wales and England, [c. 1871]-1935; miscellaneous papers and research notes, 1904-1966.

Personal correspondence, 1916-1954; study notes, 1902-1952; biographical material, 1903-1954; notebooks entitled 'Tennyson Biography'; sermons and addresses, 1932-1952; orders of service for Victory, 1945, the United Nations 1946, Human Rights Day, 1951-1954, the Coronation and other occasions, 1931-1954; religious and international affairs, 1944-1945; Welsh Book Festivals, 1935-1938; Welsh School of Social Service, 1911-1940; The Gregynog Conferences on International Education, 1922-1937; Advisory Education Committee minutes, 1926-1929; international co-operation, 1933-1937; Welsh nationalism, 1910-1943, including nationalists' attitudes towards World War II, 1939-1941; broadcasting materials mostly of Marconi and Kemp, 1931-1953; Welsh broadcasting, 1923-1948; the Welsh Children's Peace Message, Pageant, and Wales and the Peace Movement, 1923-1955; BBC staff changes and administration in Wales, 1934-1952; the League of Nations, 1923-1952; the Welsh National Council of the League of Nations Union, 1923-1945; United Nations, 1942-1954; UNESCO, 1925-1947; addresses, radio talks and notebooks on the international situation, 1930-1954; Council for Education in World Citizenship, 1940-1950; London International Assembly, 1941-1944; Welsh Committee of the UNESCO, 1949-1953 and human rights materials, 1945-1953.

Papers of W. Llewelyn Williams, KC, MP, 1861-2005, comprising diaries, letters, professional papers, printed material, personal papers, and papers accumulated by his family after his death. The collection also includes the research papers of Neville C. Masterman relating to the life and political career of W. Llewelyn Williams.

The archive comprises the records of Messrs J. and A. Davies, Llanidloes, including account books, 1927-1972, a bill book, 1957-1965, and a letter book, 1958-1962; and miscellaneous office records, 1872-1964, of Williams, Gittins and Tomley.

The fonds comprises manuscript, typescript and printed material, including copies of acts or bills, correspondence, reports, etc., relating to Aberystwyth Borough and Rural District Councils Water Supplies.

The fonds comprises minutes books of the Society, 1952-1997, and files of correspondence and papers, 1960-2001, together with a file of correspondence with the Inland Revenue, 1960-1961.

Papers of Aneirin Talfan Davies, 1911-1980, consisting of diaries, 1956-1980; papers relating to his work with the BBC, including letters and scripts, [1940s]-[1970]; correspondence, drafts and notes reflecting his literary activities, including his lectures, books, articles, libretti and his editorial duties on Barn (there is comparatively little of his poetry present), 1941-[1979]; material such as letters, radio scripts and articles relating to literary figures such as Dylan Thomas, David Jones and T. Rowland Hughes, 1937-1973; correspondence and minutes of meetings, in connection with Llyfrau'r Dryw / Christopher Davies (Publishers) Ltd., Yr Academi Gymreig, The Guild for the Promotion of Welsh Music, the Welsh Arts Council, and a number of bodies within the Anglican Church in Wales, 1971-1977; letters from various prominent Welsh literary figures and successive Archbishops of Wales, 1972-1980; several volumes of press cuttings, 1911-1977; and personal papers, 1963-1974.