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Papers, 1844-1941, of the Williams family of Acre House, Acrefair, mainly comprising letters, including family correspondence and letters received from relatives in Glamorgan, from the Pugh family, and from relatives in the USA, [late 19th cent.]-[early 20th cent.]; letters to the Rev. Ebenezer John Williams, mostly relating to his duties as minister and the chapel and water works in Llanwddyn, 1882-1889; and letters to John Williams, [late 19th cent.], mostly relating to the iron industry. The archive also includes diaries of John Williams, 1844-1897; notebooks, accounts and other documents, 1856-1893, relating to the ironworks in Ruabon and South Wales; diaries and notebooks of the Rev. Ebenezer John Williams, 1869-1935 (including chapel committee notes, accounts, Sunday School registers, and sermon notes); diaries and notebooks of Rev. John Pugh, 1849-1890, (including one containing his autobiography); papers relating to Liberal Party election campaigns in Montgomeryshire and Denbighshire, [late 19th cent.]; deeds, 1842-1921, mostly relating to property in Dowlais; papers relating to schools, [late 19th cent.]-[early 20th cent.], including school notebooks, prospectuses of schools including Holt Academy, and papers relating to the founding of British schools in the Cefn Mawr district and elsewhere.

Deeds and documents relating to Trimsaran Coal, Iron and Steel Company, [c. 1861]-1872; Ynisarwed Resolven Colliery Company, 1866-1875; and Yniscedwyn Iron, Steel, and Coal Company, 1837-1875; and copies of Court Rolls of the Manor of Evenjobb, Radnorshire, 1798-1851.

Papers of John Bedford, 1762-1791, largely relating to his time in South Wales, and deal with iron-making techniques, his interests in experimenting with and improving these techniques, and the state of his own business ventures in forging and quarrying. The papers include notes on iron-making techniques, 1763-1788; management and business papers, 1766-1791; correspondence, petitions and miscellaneous notes, 1766-1789; and quarry notes, 1762-1789.

Papers of W. Emrys Pride, 1936-1987, comprising correspondence and other papers relating to devolution and economic policy, 1969-1978; papers relating to his work as a civil servant, mainly on economic topics, 1940-1978; research papers for his publications, including 'Tinman's progress' (1966), 'Rhondda my valley brave' (1975), 'Why Lloyd George met Hitler' (1981), and 'Pride in Britain's High-Tech Progress' (1985), 1966-1985; personal papers and miscellaneous correspondence, 1936-1977; financial papers, 1949-1977; and offprints and typescripts of articles and booklets, 1949-1987.