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Papers, 1743-1994, of or relating to Margaret Mostyn Jones of Wern House, Mostyn, Flintshire, and to members of her family, and including a journal, 1861-1864, kept by her while employed by Augusta Hall, Lady Llanover; correspondence, 1876-1932, to and from Margaret Mostyn Jones, including letters, 1890-1894, written to members of her family while living in Ohio; an autobiographical essay, 1929-1932, by Margaret Mostyn Jones; together with papers, 1743-1874, mainly of Flintshire interest.

Letters addressed to Huw T. Edwards, 1929-1970, and carbon copies of letters sent by him, 1945-1969, concerning politics, literature, and the Council for Wales and Monmouthshire, including letters to and from political figures in the Labour Party and Plaid Cymru, and Welsh literary figures; pocket diaries, 1929-1968; minute books of the North Wales Labour Federation, 1923-1930; reports and memoranda concerning the activities of the Council for Wales and Monmouthshire, political life in North Wales, and the activities of TWW, 1935-1966; press cuttings relating to Edwards' political career and the activities of the Council for Wales and Monmouthshire, 1930-1968; illuminated addresses and distinctions presented to him, 1933-1969; miscellaneous printed items, 1912-1967; poems by him, 1950-1958; and other personal papers, 1926-1967; and acquired papers, notably letters from Sir Owen M. Edwards to Hughes and Son, Wrexham, printers, 1894-1895.

Deeds, 1507-[1839], mainly relating to Flintshire, and to a lesser extent to Denbighshire and Anglesey.

Deeds and documents (1668-1882) relating to properties mainly in in co. Flint (Axton, Bistre, Caergwrle, Coleshill, Cwm, Cwm Uwchglan, Diserth, Estyn or Hope, Hawarden, Holywell, Hope, Hope Owen, Huriathicke, Kilken, Kinnerton, Mould, Newmarket, Northop, St Asaph, Shordley, Skeiviog, and Whitford), but also in cos Denbigh (Denbigh, Henllan, Llanrwst and Lleweny), Chester (Chester and Dodleston), Brecknock (Devynnock), Anglesey (Amlwch, Coedana, Llanerchymedd, Llanbadrug, Llanddyfnan, Llanfechell and Llanfihangel Tre'r Beurdd), Montgomery (Berth Lloyd) and Pembroke (Amroth). The main families were Mostyn of Mostyn Hall and Hope of Broughton and Hope.

Deeds purchased from W. A. Evans, relating to Denbighshire, Flintshire and Anglesey, 1310-1795.

Papers relating to families and estates in north Wales, including the West family, the Chirk Castle estate, the Hengwrt, Rug and Nannau estate, the Wynnstay estate, the Penbedw estate, the estate of Richard Willding of Llanrhaeadr Hall, Denbighshire, and the Whitehall-Davies family of Broughton Hall, Flintshire, and Llannerch, Denbighshire. Records and correspondence, including relating to abstracts of title, chapels, churches, conveyances, inclosures, industrial activity, law suits, mining, parliamentary elections, probate, railways, schools and tithe commutation. Office records, including cash journals, bill books and letter books, [19th century]-[20th century].

Deeds and documents, 1280-1797, relating to Shropshire, Cheshire, Denbighshire, Flintshire, Montgomeryshire and Staffordshire, together with genealogical, heraldic and antiquarian notes, compiled c. 1745-c.1766 and [mid 19th cent.].