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A collection which includes Welsh and Irish poetry; a translation of the psalms from Latin into Welsh; Welsh sermons; papers relating to the founding and early days of the University College of Wales, Aberystwyth; material relating to Ann Griffiths and to Richard Robert Jones ('Dic Aberdaron'); original literary manuscripts; notebooks and journals; miscellaneous transcripts; etc.

A volume containing sermons written by John Prichard, Amlwch (1821-1889).

A volume containing pedigrees of British saints copied by Sir Samuel Rush Meyrick [1783-1848] from transcripts made by Edward Williams ('Iolo Morganwg') [1747-1826] from the books of Thomas ab Ieuan [Thomas Evan James] ('o Dre'r Bryn') [1824-1870].

Transcripts of 'cywyddau' by Sion Cent, Dafydd Gorlech, Robin Ddu, Dafydd Llwyd ap Llywelyn, Lewis Powys, Gwilym Telyn, Maredudd ap Rhys, Owain Twna, [Sir] Gruffudd Fychan, Syr Huw Pennant, Edwart Owain and Ieuan Brydydd Hir (Ieuan Fardd).

A volume containing a collection of tunes and anthems, mainly with Welsh words.

A transcript by John Thomas ('Sion Wyn o Eifion') of cywyddau and other poems by Robin Ddu, Rhys Goch Eryri, Iolo Goch, Tudur Aled, Dafydd Gorlech, Dafydd Llwyd ap Llywelyn ap Gruffudd, Dafydd ap Hwlcyn ap Madog, Rhys Llwyd ap Rhys, Maredudd ap Rhys, Mathew Owen, Edward Morus and Sion Lleyn; the manuscript also contains triads, genealogies, 'Breiniau Gwŷr Arfon', 'Meddygon Myddfai', 'geirlyfr William Lleyn', etc.

The original manuscript, 1877, of 'Caneuon y Gwynfydau' by Richard Davies ('Mynyddog').

Autographs of various Welsh ministers and writers; an autograph sermon by Morgan Howells [1794-1852]; a poem on the Vale of Glamorgan by Lt-Colonel Morgan, 1834; poems by Robert Davies ('Bardd Nantglyn') [1769-1835].

A transcript, 1763, made by Evan Thomas [d. 1781], Cwmchwylfod, near Bala, of a sixteenth century herbal attributed to William Salesbury [1520?-1600?].

Autograph sermons in the hand of Richard Jones, Wern, Llanfrothen, 1798; hymns based on the Psalms; poems; notes on Calvinistic Methodist Association meetings, 1806-1807; miscellaneous notes.

Sermons by John Parry (1775-1846), Chester (author of Rhodd Mam, etc.).

Sermons, 1838, in the hand of William Ambrose ('Emrys') [1813-1873].

Printed, manuscript and graphic material relating to Richard Robert Jones ('Dic Aberdaron').

A metrical translation of the psalms from Latin into Welsh by George Parry, son of James Parry ['Eos Ewias'] of Ewyas Lacy.

Sermons written by Christmas Evans (1766-1838).

A transcript by William Jones ('Bleddyn'), Llangollen of 'cywyddau' and 'englynion', etc. by Gwerful Mechain, Hywel Dafi [Hywel ap Dafydd ab Ieuan ap Rhys], Sion ap Philpot, Robert ap Dafydd Llwyd, Gruffudd Leiaf, Iorwerth Fynglwyd, Dafydd Llwyd ap Llywelyn ap Gruffudd, Sion ap Hywel ap Tudur, Huw Cae Llwyd, Lewis Daron, Bedo Brwynllys, Syr Rhys o Gar[no], 'Twm o'r Nant' [Thomas Edwards], 'Person Llangwm', Tudur Aled, Morys ap Hywel ap Tudur, Gruffudd Hiraethog, Huw Llwyd Cynfal, Ieuan Dew Brydydd, Dafydd ap Gwilym, Richard Cynwal, Huw Machno, Syr John [Sion] Leiaf, [Sir] Huw Pennant, Rhys Nanmor, Sion Dafydd Lâs [John Davies], Syr Dafydd Owain, Gruffudd ab Ieuan ap Llywelyn Fychan, Hywel Cilan, Sion Tudur, Lewis Môn, Hywel Gethin, Ieuan ap Gruffudd Leiaf, Watcyn ap Rhisiart, Hywel ap Rheinallt, Mathew Brwmffild, Guto'r Glyn, Watcyn Clywedog, Wiliam Llŷn, Wiliam Cynwal, Simwnt Fychan, Ieuan Llafar, Thomas Prys, William Vaughan, Huw Arwystli, Sion Phylip, Richard Phylip, Ieuan Dyfi, Lewis Menai, Rhys Goch Glyndyfrdwy, Llywelyn ap Gutun, Madog Leiaf and Ieuan ap Rhydderch, with 'englynion' by Dafydd Nanmor, Cadwaladr Ces[ai]l, Huw Ifan ap Huw ('o'r Brynbychan') and Siôn Ifan.

A volume containing notes of sermons by Enoch Williams (Llansamlet), John Michael (Y Berth, Llanfaethlu), Micah Thomas (Y Fenni), Henry Rees, Roger Edwards, Joseph Thomas (Carno), Lewis Edwards, Edward Morgan (Dyffryn), R. A. Jones (Swansea) and Dr Thomas Price (Aberdare); miscellaneous poems; a printed translation into Tahitian, by John Davies, of the first portion of the Gospel of St John.

Letters relating to the work of the University College of Wales Welsh library committee and lists of subscriptions and gifts received by that committee 1896-1899; letters concerning the College entrance scholarship examination, 1887; a letter, 1909, containing notes of the pedigree of Charles Comstock Betts, Richmond, Mass. and Brooklyn, USA.

A volume containing documents relating to the family of Ann Griffiths (née Thomas) [1776-1805], Dolwar Fechan, hymnist.