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Mae'r casgliad yn cynnwys cerddi eisteddfodol, cerddi coffa ac englynion gan Dofwy, ei ddyddiadur am 1888, traethodau ganddo, ynghyd â thorion o'i erthyglau o Y Cymro. = The collection includes eisteddfodic poems, memorial poems and englynion by Dofwy, his diary for 1888, essays by him, together with cuttings of his articles from Y Cymro.

Records of the Dolgelley Aiding Society, 1828-1856, comprising financial records, 1828-1845; minute books, 1830-1835; rules, 1829-1856; medical certificates, 1831-1833; and correspondence, 1833.

Estate records, almost all title deeds, of the Dolforgan and Llynlleoedd estates, Montgomeryshire, 1570-1879, together with papers, mainly rentals, accounts, and particulars, of the following manors belonging to the Powis Castle estate: Kerry, Cydewain and Halcetor, 1579-1745, Starta Marcella, 1623-1702, and Tirymynech, 1650-[mid-18 cent.].

Deeds relating to the Dolobran estate in the parishes of Meifod and Llanfihangel-yng-Ngwynfa, Montgomertyshire. The deeds date from the time of Charles Lloyd (1662-1747), and are records of mortgages, transfers of mortgages and creations of trusts, of the sale of the estate by the Lloyd family to Joseph Jones, and of the repurchase in 1873 of a portion of the old estate (Dolobran Fach) by Henry Lloyd. Two documents dated 1878 refer to the acquisition of the other part of the estate by Sampson Samuel Lloyd, MP. The part played by Dolobran in the history of the Quakers in Montgomeryshire is reflected in letters, 1813-1829 relating to transactions for the sale of the Quaker Meeting House and Burial Ground at Dolobran.

Estate records of the Dolaucothi estate, Carmarthenshire, and family papers, [16-20 cent.], of the Johnes and Hills-Johnes families of including extensive correspondence comprising over 15,000 letters, 1688-[20 cent.], and military papers of Lieutenant-Colonel Sir James Hill-Johnes (d. 1919).

Deeds and documents, 1598-1856, mostly assignments of mortgage and related bonds, concerning Dôl y Cae and other premises in the parish of Tal-y-llyn, including a lease from William Owen Pughe and his brother Richard to his son Aneurin Owen Pughe.

Political papers, 1944-1991, of Donald Richard Coleman, including correspondence files, 1964-1991, mainly of political interest; papers concerning the Labour Party, 1964-1990, many relating to the Labour Party Wales; and files, 1944-1990, relating to various subjects.

The papers comprise research papers and notes relating to the Celtic verb and syntax (see Donald G. Howells, 'The Gaelic of Carloway, Isle of Lewis: prepositions with verbal nouns' in James Carney and David Greene (editors), Celtic Studies. Essays in memory of Angus Matheson 1912- 1962 (London, 1968), and D. Gwyon Howells, 'Absolute and conjunct again', Studia Celtica, 22/23 (1987/88)); notes in the form of index cards relating to the origin of Welsh phrases and idioms (boxes 15-16); translation and grammatical points on 'Y Gododdin' (box 6) and comments on the syntax of 'Breuddwyd Rhonabwy' (box 10); and photocopies of articles relating to syntax in other languages, in particular French and Indo- European (box 14).

Original deposit of Dora Thatcher papers, comprising material accumulated during preparation for her published books, 1955-1977. Additional deposit of Dora Thatcher papers, comprising material accumulated during preparation for her short stories, plays and articles, 1948-1985.

Papers, 1920-1989, of Dorothy Sylvester, including notebooks and lecture notes, 1920-1972; research papers, including notes, card indexes and press cuttings, relating mainly to her study of the historical geography of England and Wales, with special reference to the Welsh borderland; material relating to published works, 1957-1983; addresses and articles, 1928-1988; literary papers, and correspondence, 1926-1989.

Records of the campaign to secure to top level domain .cym for the Wales mainly comprising correspondence, letters of support, policy documents and press coverage. The campaign later supported .cymru and .wales as domains for Wales.

Research papers of Douglas B. Hague, including general correspondence relating to research work on lighthouses, 1960-1988; typescript drafts, correspondence, 1967-1975, and notes relating to the publication of Lighthouses: their Architecture, History and Archaeology; notes relating to the publication of Lighthouses of Wales; and miscellaneous papers, 1965-1987.

The collection comprises deeds and documents, 1587-1861, relating mainly to the Mackworth family of Gnoll and to the Gnoll estate; miscellaneous documents, 1801-[1865], mainly relating to Neath; and miscellaneous documents, extracts taken from documents made by Donald H. Jones, mainly of Neath interest; papers relating to meetings, 1923-1933, of the Neath Antiquarian Society; notes made by Donald Jones of tours of north and south Wales; historical and archaeological notes by Donald Jones; a file of letters, 1931-1939, received by Jones; files of press cuttings relating to Neath antiquities, 1925-1935; and many other miscellaneous papers and documents of Neath interest.

Deeds and papers collected by Douglas J. Elliott, mainly relating to the Jones of Glanyrafon-ddu family and to properties in Llansadwrn, Pencarreg, and Talley, Carmarthenshire, 1767-1869; and typescript copy of the parish register of Gwaenysgor, Flintshire, 1713-1760, [20th century].

Notebooks and other papers of Dr Douglas Houston, including drafts of poems, notes, diary entries, correspondence and drafts of articles.

Records relating to David Owen & Son, 1860-1958,including account books, 1860-1958, time sheets, 1945-1958, letter books, 1921-1943, and business papers and correspondence, 1916-1957.

Deeds relating to the estates in Denbighshire and Flintshire, of the Pennant families of Bychton and Downing, 1352-1802, and a small number of draft letters from, and letters to, Thomas Pennant, [c.1765]-1769, together with some of his notes and a notebook, [c.1764-1765] and undated.

Records accumulated by D. Peter Garbett Edwards, 1951-1993, including records relating to the Mid-Wales Industrial Development Association, 1957-1977; records relating to the Mid-Wales Development Corporation, 1973-1977; records relating to the Development Board for Rural Wales, 1978-1987; miscellanea, 1951-1996; and related printed material, 1966-1997.

Scrapbooks containing press cuttings etc., 1900-1982, relating largely to Welsh drama, theatrical activities and popular entertainment in Wales and amongst Welsh communities in English cities, including material on dramatists of Wales, 1932-1953; drama in Wales, 1922-1982; Welsh actors, 1932-1946; theatre cuttings, 1931-1953; fairs, folklore and folk-dancing in Wales, 1936-1938; children's theatre, 1959-1967; Welsh National Theatre, 1900-1978; and information on theatre in Ireland, Scotland, France, Spain, Germany, Italy, Greece, Russia, America, and other countries.

Papurau D. R. Evans, yn cynnwys ei atgofion am fywyd ar y môr, [c. 1917], ei anerchiadau a nodiadau ar bynciau amrywiol, a dyddiaduron Hugh H. Hughes, 1913-1914, ynghyd â dau draethawd gan Jones, [c. 1906] = Papers of D. R. Evans, comprising his memoirs of life at sea, [c.1917], his addresses and notes on miscellaneous subjects, and diaries of Hugh H. Jones, 1913-1914, together with two essays by Jones, [c.1906].