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The fonds comprises minutes books of the Society, 1952-1997, and files of correspondence and papers, 1960-2001, together with a file of correspondence with the Inland Revenue, 1960-1961.

Notes for a guided tour of the commote Uwch Aled, Denbighshire written by Robin Gwyndaf, 2011.

Records of Vale of Glamorgan Liberal Association and Barry Constituency Liberal Association, comprising minutes of Annual General Meetings, 1974-1982; Executive Committee minutes, 1975-1987, papers relating to the Welsh Liberal Party, 1982-1987; Barry Town Liberal Association accounts, 1975-1984; correspondence concerning Prospective Parliamentary Candidate, 1981-1982 and with Vale of Glamorgan SDP, 1981-1985; notes on environment and planning in South Glamorgan, 1981-1982; general correspondence and papers, 1982-1987, including the proposed amalgamation with the SDP, 1987; election literature, 1983-1987; and papers relating to Sully and Wenvoe branches, 1983-1986.

Records of the Vale of Neath Brewery, 1844-1913, including ledgers, 1894-1897; pay books, 1882-1912; purchase abstract books, 1896-1908; beer sales books, 1896-1913; spirit sales books, 1897-1912; and printed books, 1863-1913.

A vesting assent dated 17 December 1953, bound in book form, relating to the Llysnewydd Estate in the counties of Carmarthen and Cardigan, 1953-1981, including an estate map.

Two volumes containing manuscript music, 1809-1828, one inscribed within by 'Mary Madocks, alias Williams, Vron-Iw, October 1809', and two volumes of printed music, one of which belonged to Mrs Henry Laird, inscribed within by 'Jessie Laird, 1879', and bearing the initials 'J.L.', and the other bearing the bookplate of Mrs Mevekson-Sandbach. One manuscript copy and a printed copy has 'Mrs Williams, 1822' written on their covers.

Deeds relating to the parishes of Llanbadarn Fawr, 1548-1597, and Llangynfelyn, 1841-1848, Cardiganshire.

Deeds purchased from W. A. Evans, relating to Denbighshire, Flintshire and Anglesey, 1310-1795.

Deeds relating to properties at Deep Dean, Walford, Herefordshire, 1799-1816, and in Merthyr Tydfil, Glamorgan, 1788-1859.

Deeds and documents relating to Cardiganshire, 1590-1751; and Montgomeryshire, 1517-1770; deeds and documents relating to the Hughes family of Gogarth, 1669-1910; and miscellaneous items, 1692-1825.

A notebook containing notes on the history and practice of the Courts of Great Sessions in Wales accumulated by W. Llewelyn Williams, K.C., M.P. (1867-1922) (see Y Cymmrodor, XVI, pp. 1-87). Many of the extracts are taken from the Llwynwormwood MS, i.e. NLW MS 4492D.

The reminiscences of William Robert Hall (1849-1937), written in forty exercise books and published serially in The Cambrian News, 1920-1921.

Correspondence and other papers used in preparation towards the Wales Assembly of Women's report for the United Nations Fourth World Conference on the status of women, Beijing, 1995.

Particulars, in the autograph of Walter Davies (Gwallter Mechain) (1761-1849), of wages paid to agricultural workers in Wales c. 1800.

Deeds, wills and other documents relating to Monmouthshire, 1568-1825.

A typescript copy of an unpublished work by Richard Anthony entitled 'Water over Wales's Valleys', 1985.

Deeds and documents relating to properties mainly in Montgomeryshire, 1615-1910.

Account book, mainly in Welsh, 1867-1907, of Thomas Jones (d. 1897), Brynmeheryn, Ystradmeurig, co. Cardigan, containing customers' accounts for weaving, sometimes with details of patterns; also included are a few veterinary recipes. Later entries are in the hand of Evan W. Jones, possibly the son of Thomas Jones.

Account book, 1887-1916, of Thomas Jones, Pant-teg, Bronnant, co. Cardigan, weaver, with a few later memoranda, 1921-1924, mostly concerning machinery, by his son E. D. Jones. Note on 'Patrwn Carthen Felinfach' inside back cover.

A manuscript containing an account of money gifts received by Richard and Elizabeth Davies (probably of Carmarthen) on their wedding day, November 19th, 1811, and of gifts 'repaid' by them.